The invention described herein details flexible, high-efficiency photovoltaic cells with nano-enhanced absorbers and ultra-low dark current. By extending infrared absorption, power conversion efficiencies in single-junction, nano-enhanced solar cells can potentially meet or even exceed the Shockley-Queisser limit. Novel device designs utilizing advanced band gap engineering are employed to suppress non-radiative recombination and expose the limiting radiative component of the dark current. Light trapping structures and new nanostructured absorber designs are also considered to maximize the creation and collection of photogenerated carriers. Flexible photovoltaic devices are fabricated using established full-wafer epitaxial liftoff processes. The innovative design described herein provides for light-weight and flexible photovoltaic sheets capable of achieving ultra-high conversion efficiencies over a wide range of operating conditions.