Disclosed herein is system comprising a lighter-than-air (LTA) device and method of making the same. In an embodiment, the system includes the LTA device, which includes a membrane having a flexible substrate and an active material disposed thereon, wherein the active material is configured to controllably change the surface area of at least a portion of the substrate when an electrical stimulus is applied to the active material. In addition, the system may include a payload box; an altitude control vent mechanism; a meteorological data collection package; a communication unit; and an antenna.