A frequency demultiplication adjustment method of PLL comprises obtaining a plurality of corresponding frequency demultiplication frequency points according to a default frequency demultiplication value of a phase-locked loop; obtaining a load state of the processor within a predetermined sampling period, and obtaining a target frequency point of the processor by the processor frequency adjustor; determining a frequency range of a virtual frequency point to be added according to the position of the target frequency point; performing calculation within the frequency range to obtain equivalent frequencies corresponding to virtual frequency points; judging whether the frequency of the target frequency point is equal to the equivalent frequency corresponding to the virtual frequency points; if not, switching the processor frequency adjustor to the corresponding frequency demultiplication frequency point; and adjusting the frequency demultiplication value of the phase-locked loop which outputs a clock source signal corresponding to the virtual frequency points to the processor.