A design method for optimization of a transient control law of the aero-engine is disclosed, and performs the transient schedule optimization for the aero-engine by adopting an SQP algorithm, to realize the design of the transient control law along a constrained boundary condition. The fuel flow rate value is adjusted, other constraints remain unchanged, and the transient control law is designed under different limits. The transient time under each transient control law is calculated by constructing the transient time evaluation function. A lookuptable interpolation table is established by using the calculated transient time and corresponding fuel flow, to realize the fuel flow scheduling under different transient time. The fuel flow obtained by scheduling in the expected time is taken as an acceleration and deceleration control schedule of the closed-loop control of the aero-engine, and the output thereof is taken as the reference instruction of an acceleration process.