A method includes the production of a primary ingot, the production of a secondary ingot, and the removal of a flux layer. A CaO—CaF2 flux in a content of 3-20 mass % and obtained by mixing 35-95 mass % of CaF2 with CaO is added to a Ti—Al alloy material including a total of at least 0.1 mass % of oxygen and at least 40 mass % of Al, and the resultant substance is melted by a melting method using a water-cooled copper container in an atmosphere having a pressure of 1.33 Pa or higher and held to produce the primary ingot. The primary ingot is continuously drawn downwards while being melted by a melting method using a bottomless water-cooled copper casting mould in an atmosphere having a pressure of 1.33 Pa or higher to produce the secondary ingot. The flux layer deposited on the surface of the secondary ingot is mechanically removed.