The present disclosure provides an optimization method, a unit, and an electronic device of a shifted frequency (SF)-based electromagnetic transient simulation, comprising: determining a current amplitude and a voltage frequency based on a node voltage and a branch current calculated from a shifted frequency on a basis of a current time step; determining an optimal shifted frequency of the current time step based on the current amplitude and the voltage frequency; and updating the shifted frequency by adopting the optimal shifted frequency of the current time step for calculating a node voltage and a branch current of the next time step. The method, the unit, and the electronic device provided in the present disclosure may gradually update and optimize the shifted frequency in the simulation process so to enable the shifted frequency to reach the best, thus ensuring the accuracy of output current and voltage simulation results.