A powertrain control system is provided for a vertical take-off and landing aerial vehicle for urban air mobility. A powertrain of the vertical take-off and landing aerial vehicle is a hybrid type powertrain, in which the output shaft of a rotor driving motor is directly connected to a rotor, a battery is connected to the rotor driving motor to supply power thereto, and an engine and a generator are connected to a battery to charge and discharge the battery. The driving of the engine and the generator is controlled based on required power of the motor and the SOC of the battery in each flight step of the vertical take-off and landing aerial vehicle, and the SOC of the battery is constantly maintained at a predetermined level or higher.