A method for detecting whether vertical deviation of an optical disc occurs is provided. First, before a pickup head is successfully focused on the optical disc, a pickup head is actuated based on an input control signal so as to generate a focus error signal with a plurality of S-curves. Then, a plurality of zero crossing points of the S-curves in the focus error signal is identified and a plurality of input control values respectively corresponding to the zero crossing points is obtained. A variation of the input control values is then calculated. Whether vertical deviation of the optical disc occurs can be determined according to the variation of the input control values.