A method for fabricating an organic light-emitting diode employing a mixed host is disclosed, which comprises the following steps: (A) providing a substrate with a first electrode formed thereon; (B) coating a mold with a light-emitting layer material, wherein the light-emitting layer material comprises: a mixed host, and dye molecule(s) (or dye-function-group-composing materials) etc.; (C) pressing the mold coated with the light-emitting layer material onto the substrate to transfer the light-emitting layer material to the first electrode of the substrate, to form a light-emitting layer; and (D) forming a second electrode over the light-emitting layer. The mixed host consists of host-function molecule(s) and auxiliary additives. In addition, the present invention also provides a light-emitting diode, which is prepared by the aforementioned method.