An overclocking control method cooperates with an overclocking application of a computer system when the overclocking application is started. The overclocking control method includes the steps as follows. A BIOS enters an overclocking mode according to an executing state of the overclocking application. The BIOS receives a first triggering signal outputted from a south bridge chip, and the first triggering signal is generated by the south bridge chip according to a first button of the computer system. The BIOS selects a piece of corresponding overclocking information from a look-up table and loads the overclocking information into a register of the BIOS according to the first triggering signal to control the overclocking of the computer system.