A method of evenly using a plurality of blocks of a Flash memory comprises: providing at least one threshold value, which is utilized for sieving out blocks suitable for use from the plurality of blocks according to erase counts of the plurality of blocks; and by comparing erase counts of at least a portion of the plurality of blocks with the threshold value, sieving out a specific block for use from the plurality of blocks according to a purpose of use. An associated memory device and a controller thereof are also provided, where the controller comprises: a ROM arranged to store a program code, wherein the controller is provided with the at least one threshold value through the program code; and a microprocessor arranged to execute the program code to control the access to the Flash memory. The controller sieves out the specific block according to the purpose of use.