In a method of manufacturing a liquid discharge head, the liquid discharge head has a flow-path unit having a liquid flow path, and a piezoelectric actuator unit. The liquid flow path has discharge openings and corresponding pressure chambers. The actuator unit has actuators which apply pressure to liquid in the pressure chambers. The method includes positioning the actuator unit to oppose the surface of the flow-path unit while extending on the plurality of pressure chambers, forming a particular film that is impermeable to the liquid on a supporting member. The particular film is secured to the surface of the flow-path unit by placing the supporting member on the flow-path unit, and aligning the supporting member such that a surface of the particular film opposes the surface of the flow-path unit while the openings of the plurality of pressure chambers are covered.