The present invention provides a color adjustment device, a method of adjusting color and a display device for the same. It measures a plurality of tristimulus sets at various white grayscales on a LCD panel, converts the multiple tristimulus sets into a plurality of chromatic sets (xn, yn). Among the plurality of chromatic sets (xn, yn), it recognizes the Pth chromatic set (xp, yp), the break point, and based on the pth chromatic set (xp, yp), determines a plurality of target chromatic sets (Nxn, Nyn) at from the grayscale 0 to the grayscale p, where Nx n = x 0 + ( x 255 - x 0 ) · [ 1 - exp ⁡ ( 1 - p n ) ] , ⁢ Ny n = y 0 + ( y 255 - y 0 ) · [ 1 - exp ⁡ ( 1 - p n ) ] . By this method, an exponential function instead of a linear function is adopted to depict the chromatic variation at low grayscales. Thus the grayscale variation appears more smooth and without any obvious break point in human's perception.