A preparing method for coiled nano carbon material is provided and includes forming a noble metal catalyst crystallite nucleus layer on the surface of the substrate by displacement of a noble metal catalyst, forming a composited nano carbon material on the metal layer of the substrate by using TCVD; in which the composited nano carbon material includes coiled carbon nano tubes and coiled carbon nano fiber. The measured quantity of the total coiled nano carbon tubes and coiled nano carbon fiber in the total measured quantity of nano carbon material is greater than 30%. The coiled nano carbon material can be acquired by scraping it off from the substrate surface.