The present invention relates to an electrode for a non-aqueous electrolyte secondary battery, a non-aqueous electrolyte secondary battery using the electrode, and a method for manufacturing the non-aqueous electrolyte secondary battery. The electrode for a non-aqueous electrolyte secondary battery includes a material mixture layer containing an active material and a porous insulating layer. The insulating layer is formed on the material mixture layer. The insulating layer contains a resin having a cross-linked structure and inorganic particles. A mixed layer that includes components of the insulating layer and components of the material mixture layer is provided at the interface between the insulating layer and the material mixture layer.