Methods for applying a coating to a substrate in rolled form, the substrate including a first edge face and a second edge face opposite the first edge face, the substrate further having a first major surface and a second major surface opposite the first major surface, the first and second major surfaces extending between the first edge face and the second edge face, the methods including applying a coating to at least one edge face and optionally at least a portion of one or both major surfaces of the substrate in rolled form. Articles in rolled form prepared according to the foregoing methods are also disclosed.