A method of forming a light sheet includes printing a layer of inorganic LEDs on a first conductive surface of a substrate, depositing a first dielectric layer, and depositing a second conductor layer over the LEDs so that the LEDs are connected in parallel. At least one of the first conductive surface or the second conductor layer is transparent to allow light to escape. A phosphor layer may be formed over the light sheet so that the LED light mixed with the phosphor light creates white light. The flat light sheet is then folded, such as by molding, to form a three-dimensional structure with angled light emitting walls and reflective surfaces to control a directionality of the emitted light and improve the mixing of light. The folds may form rows of angled walls or polygons.