In one aspect, methods of detecting ice formation on an aircraft are described herein. In some implementations, a method of detecting ice formation on an aircraft comprises disposing an ice detector on an exterior surface of the aircraft, the ice detector comprising a probe surface and a pyroelectric material layer disposed on at least a portion of the probe surface. The method further comprises generating a charge on a surface of the pyroelectric material layer of the ice detector to increase the local freezing point of water on the surface of the pyroelectric material layer.