Disclosed are a method and a device for intercepting a call for a service by an application in an operating system of an electronic apparatus. The method comprises: loading an interception dynamic link library to a process where the service is located; replacing the address of an input/output control function in the process with a first address of the interception dynamic link library; when the application is calling the service, executing the interception dynamic link library based on the first address so as to obtain the name and information of the application as well as the information of the call, and replacing the address of the service to be called comprised in the information of the call with a second address of the interception dynamic link library; and executing processing based on the second address according to the name and/or information of the application. The invention increases the security of the operating system of the electronic apparatus.