The disclosure features methods that include obtaining a first calcium hydroxide solution that includes a first concentration of calcium ions and a second calcium hydroxide solution that includes a second concentration of calcium ions, adding a phosphoric acid solution to the first calcium hydroxide solution to generate a combined solution featuring an aqueous suspension of calcium dihydrogen phosphate particles, and adding the second calcium hydroxide solution to the combined solution to form a product solution that includes an aqueous suspension of particles of a calcium phosphate composition.