Disclosed herein is a composition for use in the preparation of a Lacrosse sport ball, the composition comprising a prepolymer, the prepolymer comprising a multifunctional polyisocyanate and one or more polyols having a molecular weight of from about 1000 Daltons to about 5000 Daltons, and a curative comprising an amine or an additional polyol or a combination thereof. A Lacrosse ball formed from the composition exhibits a ball compression of from about 180 pounds to about 210 pounds or from about 90 pounds to about 210 pounds when tested in accordance with ND 049-12m12 Section 5.3 Ball Compression, and wherein the molded spherical ball exhibits a ball coefficient of restitution COR of from about 0.60 to about 0.70 or from about 0.50 to about 0.75 when tested in accordance with ND 049-12m12 Section 5.4 Ball Coefficient of Restitution COR.