Electrodes, separators, half-cells, and full cells of electrical energy storage devices are made with electrospinning and isostatic compression. The electrical energy storage device may include electrochemical double layer capacitors (EDLCs, also known as “supercapacitors”), hybrid supercapacitors (“HSCs”), Li-ion capacitors and electrochemical storage devices, Na-ion capacitors and electrochemical storage devices, polymer electrolyte fuel cells, and still other capacitors and electrochemical storage cells.