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    Method for catalytic conversion of carbon monoxide in a hydrogen-containing gas mixture with improved cold start behavior
    21.
    发明授权
    Method for catalytic conversion of carbon monoxide in a hydrogen-containing gas mixture with improved cold start behavior 失效
    在具有改进的冷启动行为的含氢气体混合物中催化转化一氧化碳的方法

    公开(公告)号：US06555088B1

    公开(公告)日：2003-04-29

    申请号：US09566981

    申请日：2000-05-09

    Applicant: Frank Baumann ,  Stefan Wieland

    Inventor： Frank Baumann ,  Stefan Wieland

    IPC: C01B316

    CPC classification number: B01J23/56 ,  B01J23/38 ,  B01J23/89 ,  C01B3/16 ,  Y02P20/52

    Abstract: A method for conversion of carbon monoxide to carbon dioxide and hydrogen with water in a gas mixture containing hydrogen and other oxidizable components. An oxidation-active noble metal shift catalyst is the catalyst. The necessary operating temperature of the catalyst is established and optionally maintained by partial oxidation of the oxidizable components of the gas mixture.

    Abstract translation: 一种在含有氢气和其他可氧化组分的气体混合物中将一氧化碳转化为二氧化碳和氢气的方法。 氧化活性贵金属转移催化剂是催化剂。 催化剂的必要操作温度被建立，并且任选地通过气体混合物的可氧化组分的部分氧化来维持。

    Shaped organosiloxane polycondensates, process for their preparation and use
    23.
    发明授权
    Shaped organosiloxane polycondensates, process for their preparation and use 失效
    成型有机硅氧烷缩聚物，其制备和使用过程

    公开(公告)号：US5466767A

    公开(公告)日：1995-11-14

    申请号：US340877

    申请日：1994-11-15

    Applicant: Stefan Wieland ,  Peter Panster ,  Horst Grethe

    Inventor： Stefan Wieland ,  Peter Panster ,  Horst Grethe

    IPC: C08G77/48 ,  C08G77/54 ,  C08G77/58 ,  C08G77/26 ,  C08G77/22 ,  C08G77/30

    CPC classification number: C08G77/54 ,  C08G77/48 ,  C08G77/58

    Abstract: Disclosed are shaped organosiloxane polycondensates in the form of macroscopic spherical particles with a diameter of 0.01 to 2.5 mm, a specific surface area of 0.01 to 1000 m.sup.2 /g, a specific pore volume of 0.01 to 5 ml/g, and a bulk density of 50 to 1000 g/l, consisting of units of the formula (I):X--R.sup.1 (I)and/or the formula (II):R.sup.2 --Y--R.sup.3 (II)and the formula (III): ##STR1## as well as optionally, in addition, units of the formula ##STR2## wherein R.sup.1 to R.sup.3 are identical or different and represent a group of the formula (V): ##STR3## R.sup.4 being bonded directly to the X or Y group and representing a linear or branched, fully saturated or unsaturated alkylene group, a cycloalkylene group, a phenylene group or a unit of the formula ##STR4## and M corresponding to a Si, Ti or Zr atom. Also disclosed are a process for preparation and use.

    Abstract translation: 公开了直径为0.01〜2.5mm，比表面积为0.01〜1000m2 / g，比孔体积为0.01〜5ml / g的宏观球状颗粒形状的成型有机硅氧烷缩聚物，体积密度为 由式（I）：X-R1（I）和/或式（II）：R2-Y-R3（Ⅱ）和式（Ⅲ）组成的单位为50〜1000g / （III）的化合物，另外还有式（IV）的单元，其中R 1至R 3相同或不同并且表示式（Ⅴ）的基团：或Y基团，并且表示直链或支链的 完全饱和或不饱和的亚烷基，亚环烷基，亚苯基或下式的单元，即对应于Si，Ti或Zr原子的式“IMAGE”或“IMAGE”和M。 还公开了一种制备和使用的方法。

    Hydrating or oxidizing process using a metal-containing, shaped organosiloxane amine copolycondensate catalyst
    25.
    发明授权
    Hydrating or oxidizing process using a metal-containing, shaped organosiloxane amine copolycondensate catalyst 失效
    使用含金属的有机硅氧烷胺共缩合催化剂进行保湿或氧化处理

    公开(公告)号：US5352791A

    公开(公告)日：1994-10-04

    申请号：US121580

    申请日：1993-09-16

    Applicant: Peter Panster ,  Stefan Wieland

    Inventor： Peter Panster ,  Stefan Wieland

    IPC: B01J31/06 ,  B01J31/12 ,  B01J31/16 ,  B01J31/18 ,  C08G77/398 ,  C08G77/48 ,  C08G77/54 ,  C08G77/58 ,  C08K3/10 ,  C08L83/04 ,  C08L83/08 ,  C07D215/06 ,  C07C53/134 ,  C08G77/26

    CPC classification number: C08G77/58 ,  B01J31/124 ,  B01J31/1675 ,  B01J31/1805 ,  C08G77/398 ,  C08G77/54 ,  B01J2231/641 ,  B01J2531/821 ,  B01J2531/822 ,  B01J2531/824 ,  B01J2531/828

    Abstract: Shaped organosiloxane amine copolycondensates are described which contain Pd, Pt, Ru and/or Rh, as well as optional promotors and/or moderators. The shaped copolycondensate function as a carrier for metals and are made up of units of: ##STR1## and/or units of Y--R.sup.6. R.sup.2 to R.sup.6 are a group represented by the formula: ##STR2## wherein R.sup.7 is a group bound to N, X, or Y (for example, an alkylene group) and R.sup.1 is R.sup.7 --SiO.sub.3/2, H, CH.sub.3, C.sub.2 H.sub.5, or C.sub.3 H.sub.7. X stands for a double-bonded group such as --S--, --S.sub.2 --, --S.sub.3 --, --S.sub.4 --, --HN--CS--NH-- and Y stands for a monovalent groups such as --CN, --SCN, --SH, --S--CH.sub.3, --NH.sub.2, --NH--(CH.sub.2).sub.2 --NH.sub.2. The carrier substance may be cross-linked with cross-linking agents containing Si, Ti, Zr or Al. The metal-containing product is spherical in form and is defined by the parameters of sphere diameter, specific surface and pore volume as well as bulk density. Methods of production and use of the copolycondensates are also described.

    Abstract translation: 描述了含有Pd，Pt，Ru和/或Rh的有机硅氧烷胺共缩合物，以及任选的促进剂和/或调节剂。 成型的共缩聚物用作金属载体，由以下单元组成：＆lt; IMAGE＆gt;和/或Y-R6单元。 R2至R6是由下式表示的基团：其中R7是与N，X或Y结合的基团（例如亚烷基），R1是R7-SiO3/2，H，CH3 ，C 2 H 5或C 3 H 7。 X表示-S-，-S2-，-S3-，-S4-，-HN-CS-NH-和Y代表一价基团如-CN，-SCN，-SH ，-S-CH 3，-NH 2，-NH-（CH 2）2 -NH 2。 载体物质可以与含有Si，Ti，Zr或Al的交联剂交联。 含金属产品的形状为球形，由球体直径，比表面积和孔体积以及堆积密度的参数定义。 还描述了共缩聚物的生产和使用方法。

    Process for preparing glycide by epoxidation using polymeric organosiloxane ammonium salts of oxoacids of the elements V, Nb, Ta, Mo, and W
    26.
    发明授权
    Process for preparing glycide by epoxidation using polymeric organosiloxane ammonium salts of oxoacids of the elements V, Nb, Ta, Mo, and W 失效
    使用元素V，Nb，Ta，Mo和W的含氧酸的聚合有机硅氧烷铵盐通过环氧化制备糖苷的方法

    公开(公告)号：US5286885A

    公开(公告)日：1994-02-15

    申请号：US53248

    申请日：1993-04-28

    Applicant: Peter Goetz ,  Stefan Wieland ,  Peter Panster ,  Gustaaf Goor ,  Rainer Siegmeier

    Inventor： Peter Goetz ,  Stefan Wieland ,  Peter Panster ,  Gustaaf Goor ,  Rainer Siegmeier

    IPC: C08G77/54 ,  C08G77/58 ,  C07D301/12 ,  C07D303/14

    CPC classification number: C08G77/54 ,  C08G77/58

    Abstract: The invention relates to polymeric organosiloxane ammonium salts having a silica-like skeleton and including units of Formula (I): ##STR1## wherein R.sup.1 and R.sup.2 are identical or different and signify a group of Formula (II): ##STR2## wherein R.sup.5 is an alkylene group and the oxygen atoms are saturated by silicon atoms of additional groups corresponding to Formula (II), optionally with the insertion of cross-linking agents; R.sup.3 represents groups corresponding to R.sup.1 or R.sup.2, or hydrogen or an alkyl group; R.sup.4 represents hydrogen or an alkyl group; x is the charge number of an oxo anion of a monooxo-, isopolyoxo- or heteropolyoxo acid of the elements vanadium, niobium, tantalum, molybdenum or tungsten; and oxo groups of the X anion also may be replaced by peroxo groups. The invention also includes methods of preparing the salts of Formula (I) from salts of the type (R.sup.1 R.sup.2 R.sup.3 R.sup.4 N.sup.+).sub.y Y wherein Y is different from X. The invention further includes the use of the salts of Formula (I) as catalyst for oxidation reactions using peroxo compounds as an oxidation agent.

    Abstract translation: 本发明涉及具有二氧化硅样骨架并包括式（I）的单元的聚合有机硅氧烷铵盐：（*化学结构*）（I）其中R1和R2相同或不同并且表示式（II）的基团： （*化学结构*）（II）其中R5是亚烷基并且氧原子被对应于式（II）的另外的基团的硅原子饱和，任选地插入交联剂; R3表示对应于R1或R2的基团，或氢或烷基; R4表示氢或烷基; x是元素钒，铌，钽，钼或钨元素的单氧，异羟基或杂多酸的氧阴离子的电荷数; X阴离子的氧基也可以被过氧基取代。 本发明还包括从其中Y不同于X的类型（R 1 R 2 R 3 R 4 N +）y Y的盐制备式（I）的盐的方法。本发明还包括使用式（I）的盐作为氧化反应的催化剂，其使用 过氧化合物作为氧化剂。

    Catalyst for autothermal reforming of hydrocarbons with increased water gas shift activity
    27.
    发明授权
    Catalyst for autothermal reforming of hydrocarbons with increased water gas shift activity 失效
    具有增加的水煤气变换活性的烃的自热重整催化剂

    公开(公告)号：US07150866B2

    公开(公告)日：2006-12-19

    申请号：US10644377

    申请日：2003-08-20

    Applicant: Stefan Wieland ,  Frank Baumann

    Inventor： Stefan Wieland ,  Frank Baumann

    IPC: C01B3/40 ,  B01J23/40 ,  B01J23/42 ,  B01J23/46

    CPC classification number: B01J23/464 ,  B01J23/40 ,  B01J37/0244 ,  C01B3/382 ,  C01B3/40 ,  C01B2203/0244 ,  C01B2203/0283 ,  C01B2203/0844 ,  C01B2203/1005 ,  C01B2203/1047 ,  C01B2203/1064 ,  C01B2203/142 ,  C01B2203/82 ,  H01M8/0612 ,  Y02P20/52

    Abstract: The invention relates to a catalyst and a process for the autothermal, catalytic steam reforming of hydrocarbons using the catalyst. The catalyst has a multilayer structure and comprises a lower catalyst layer located directly on a support body and an upper catalyst layer located on the lower catalyst layer, with the lower catalyst layer preferentially catalysing the partial oxidation and the upper catalyst layer preferentially catalysing steam reforming. In a further embodiment, a three-layer catalyst having a further catalyst layer for the carbon monoxide conversion (water gas shift reaction) is described. Each catalyst layer comprises at least one platinum group metal on an oxidic support material.The steam reforming process is carried out in an adiabatic process by passing a feed mixture of hydrocarbons, oxygen and water or water vapour which has been heated to a preheating temperature over the multilayer catalyst.Catalyst and process are used for producing hydrogen-containing fuel gases in reformer systems, preferably for fuel cells.

    Abstract translation: 本发明涉及使用催化剂的烃的自热，催化蒸汽重整的催化剂和方法。 催化剂具有多层结构，并且包括直接位于支撑体上的下催化剂层和位于下催化剂层上的上催化剂层，下催化剂层优先催化部分氧化，上催化剂层优先催化蒸汽重整。 在另一个实施方案中，描述了具有用于一氧化碳转化的另一催化剂层（水煤气变换反应）的三层催化剂。 每个催化剂层在氧化载体材料上包含至少一种铂族金属。 蒸汽重整过程通过将已被加热到预热温度的烃，氧气和水或水蒸汽的进料混合物通过多层催化剂进行，在绝热过程中进行。 催化剂和方法用于在重整器系统中生产含氢燃料气体，优选用于燃料电池。

    Process for catalytic autothermal steam reforming of alcohols
    28.
    发明授权
    Process for catalytic autothermal steam reforming of alcohols 失效
    醇的催化自热蒸汽重整方法

    公开(公告)号：US06949683B2

    公开(公告)日：2005-09-27

    申请号：US10300173

    申请日：2002-11-20

    Applicant: Stefan Wieland ,  Frank Baumann

    Inventor： Stefan Wieland ,  Frank Baumann

    IPC: C01B3/26 ,  B01J23/63 ,  C01B3/32 ,  C01B3/40 ,  C07C27/16

    CPC classification number: C01B3/323 ,  C01B2203/0244 ,  C01B2203/0844 ,  C01B2203/1023 ,  C01B2203/1029 ,  C01B2203/1064 ,  C01B2203/1082 ,  C01B2203/1217 ,  C01B2203/1247 ,  C01B2203/82 ,  Y02P20/52

    Abstract: The invention relates to a process for catalytic autothermal steam reforming of alcohols having two or more carbon atoms by directing a preheated educt or reactant mixture of the alcohols, oxygen and water or steam over a catalyst. The process is conducted in an adiabatic manner wherein the catalyst comprises at least one platinum group metal on an oxidic support selected from the group consisting of aluminum oxide, silicon dioxide, titanium dioxide or mixed oxides thereof and zeolites, and that the educt or reactant mixture contains additional hydrocarbons, which are reformed at the same time as the alcohols.

    Abstract translation: 本发明涉及通过将催化剂上的醇，氧和水或蒸汽的预热的脱水或反应物混合物引入催化剂，从而对具有两个或多个碳原子的醇进行催化自热蒸汽重整的方法。 该方法以绝热方式进行，其中催化剂包含选自氧化铝，二氧化硅，二氧化钛或其混合氧化物的氧化物载体上的至少一种铂族金属和沸石，并且所述离子或反应物混合物 含有另外的烃，它们与醇同时重整。

    Method for catalytic conversion of carbon monoxide in a hydrogen-containing gas mixture
    29.
    发明授权
    Method for catalytic conversion of carbon monoxide in a hydrogen-containing gas mixture 失效
    在含氢气体混合物中催化转化一氧化碳的方法

    公开(公告)号：US06723298B1

    公开(公告)日：2004-04-20

    申请号：US09568814

    申请日：2000-05-11

    Applicant: Frank Baumann ,  Stefan Wieland

    Inventor： Frank Baumann ,  Stefan Wieland

    IPC: C01B316

    CPC classification number: B01J37/0205 ,  B01J23/894 ,  B01J35/04 ,  C01B3/16 ,  H01M8/0662 ,  Y02P20/52

    Abstract: A method for catalytic conversion of carbon monoxide with water to carbon dioxide and water in a hydrogen-containing gas mixture (carbon monoxide conversion) by passing the gas mixture over a shift catalyst that is at an operating temperature for the carbon monoxide conversion. The method is carried out with a shift catalyst based on noble metals that is applied to an inert support element in the form of a coating.

    Abstract translation: 通过使气体混合物通过在一氧化碳转化的工作温度下的变换催化剂将一氧化碳与水一起在含氢气体混合物（一氧化碳转化）中催化转化为二氧化碳和水的方法。 该方法使用基于以涂层形式施加到惰性支撑元件的贵金属的换档催化剂进行。

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