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公开(公告)号：KR1020140059540A
公开(公告)日：2014-05-16
申请号：KR1020120126106
申请日：2012-11-08
Applicant: 한국에너지기술연구원
Abstract: According to an embodiment of the present invention, there is provided a segment type solid oxide fuel cell module including a tubular type supporting body, a fuel electrode that is formed on the porous tubular type supporting body, an electrolyte layer, an air electrode, and a connection material, in which the air electrode has a multi-layer structure of LSCF-GDC layer, LSCF layer, LSCF-LSCo, and LSCo. According to another embodiment of the present invention, there is provided a method for manufacturing a segment type solid oxide fuel cell module including forming a flat tubular type supporting body; forming a fuel electrode on the flat tubular type supporting body; forming an electrolyte layer on the fuel electrode; forming an air electrode on the electrolyte layer; and forming a connection material that is positioned outside the air electrode and allows electrical communication between units cells by electrically connecting the fuel electrode of the unit cell to the air electrode of the other unit cell, in which the forming of the air electrode on the electrolyte layer has a step for forming paste by using SCF-GDC composite powder, LSCF, LSCF-LSCo composite powder, and LSCo, coating the paste onto the electrolyte layer, and heat-treating the coated paste.
Abstract translation: 根据本发明的实施例，提供了一种段式固体氧化物燃料电池模块，其包括管状支撑体，形成在多孔管状支撑体上的燃料电极，电解质层，空气电极和 连接材料，其中空气电极具有LSCF-GDC层的多层结构，LSCF层，LSCF-LSCo和LSCo。 根据本发明的另一实施例，提供了一种制造段型固体氧化物燃料电池模块的方法，包括形成扁平管状支撑体; 在扁平管状支撑体上形成燃料电极; 在燃料电极上形成电解质层; 在电解质层上形成空气电极; 并且形成位于空气电极外部的连接材料，并且通过将单元电池的燃料电极与另一个电池单元的空气电极电连接，从而允许单元电池之间的电连通，其中在电解质上形成空气电极 通过使用SCF-GDC复合粉末，LSCF，LSCF-LSCo复合粉末和LSCo形成糊料的步骤，将糊料涂覆到电解质层上，并对涂覆的糊料进行热处理。
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公开(公告)号：KR101395049B1
公开(公告)日：2014-05-16
申请号：KR1020120128936
申请日：2012-11-14
Applicant: 한국에너지기술연구원
Abstract: A fuel cell stack module according to an embodiment of a technical idea of the present invention includes: an air supplying system supplying air; a fuel supplying system supplying fuel; and multiple stack modules receiving the air and the fuel from the air supplying system and the fuel supplying system, and producing electric energy through an electrochemical reaction. The air supplying system comprises: multiple air branched pipes connected to each stack module; an air supplying pipe connected to one ends of the air branched pipes; and porous media located inside the multiple branched pipes, and uniformly distributing and supplying the air to each stack module.
Abstract translation: 根据本发明的技术思想的实施例的燃料电池堆组件包括：供给空气的空气供给系统; 供应燃料的燃料供应系统; 以及多个堆叠模块，其从空气供应系统和燃料供应系统接收空气和燃料，并通过电化学反应产生电能。 空气供给系统包括：连接到每个堆叠模块的多个空气分支管道; 连接到空气支管的一端的供气管; 位于多个分支管内的多孔介质，并且均匀地分配和供给每个堆叠模块的空气。
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公开(公告)号：KR1020140056544A
公开(公告)日：2014-05-12
申请号：KR1020120120434
申请日：2012-10-29
Applicant: 한국에너지기술연구원
CPC classification number: H01M4/9016 , H01M4/92 , H01M10/0568 , H01M10/0569 , H01M12/08 , H01M2300/0025 , H01M2300/0028 , Y02E60/128
Abstract: The present invention relates to a positive electrode catalyst which contains a sea urchin-shaped α-MnO_2 in which platinum (Pt), ruthenium (Ru), iridium (Ir), gold (Au), or palladium (Pd) nanoparticles are dipped, a method for manufacturing the same, and the lithium-air battery using the same. The method for manufacturing the positive electrode catalyst which contains the sea urchin-shaped α-MnO_2 according to the present invention includes: a first step in which sea urchin-shaped α-MnO_2 powder is formed by adding a first reaction activating agent to a manganese (Mn) precursor; a second step in which a mixture is manufactured by adding a second reaction activating agent used to dip one or more types of nanoparticle precursors which is selected form a group consisting of platinum (Pt), ruthenium (Ru), iridium (Ir), gold (Au), and palladium (Pd), and a reducing agent to the α-MnO_2 powder formed in the first step; a third step in which the mixture manufactured in the second step is mixed with the α-MnO_2 powder; and a fourth step in which the mixture manufactured in the third step is reduced. According to the lithium-air battery which adopts the positive electrode catalyst which is manufactured by the manufacturing method of the present invention, an oxygen reaction is accelerated in a positive electrode of the lithium-air battery so that charge and discharge overvoltage can be lowered and energy efficiency can be improved.
Abstract translation: 本发明涉及含有铂（Pt），钌（Ru），铱（Ir），金（Au）或钯（Pd）纳米粒子的海胆状α-MnO_2的正极催化剂， 其制造方法和使用其的锂空气电池。 根据本发明的含有海胆状α-MnO_2的正极催化剂的制造方法包括：第一步骤，其中通过向锰添加第一反应活化剂形成海胆状α-MnO 2粉末 （Mn）前体; 第二步，其中通过添加用于浸渍选自铂（Pt），钌（Ru），铱（Ir），金，铱，铱（Ir））的一种或多种类型的纳米颗粒前体的第二反应活化剂来制备混合物 （Au）和钯（Pd），还原剂与第一步中形成的α-MnO_2粉末的还原剂; 将第二步骤中制造的混合物与α-MnO_2粉末混合的第三步骤; 以及第三步骤中制造的混合物的第四步骤。 根据采用本发明的制造方法制造的正极催化剂的锂空气电池，在锂空气电池的正极中加速氧反应，能够降低充放电过电压， 能提高能效。
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公开(公告)号：KR101341979B1
公开(公告)日：2013-12-16
申请号：KR1020110059234
申请日：2011-06-17
Applicant: 한국에너지기술연구원
CPC classification number: Y02P70/56
Abstract: 본발명은전기화학반응을이용하여탄소연료가갖는화학에너지로부터직접전기를고효율로생산할수 있는원통형연료극지지체를이용하여구성된직접탄소연료전지및 이의제조방법에관한것이다. 본발명의직접탄소연료전지에따르면, 일단면은폐쇄되고타단면은개방된구조의원통형연료극지지체상에전극을형성한단위전지를사용하여연료극과전해질의접촉을극대화함으로써에너지밀도를향상시킬수 있다.
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公开(公告)号：KR101341974B1
公开(公告)日：2013-12-16
申请号：KR1020120119863
申请日：2012-10-26
Applicant: 한국에너지기술연구원
Abstract: An embodiment of the present invention, a solid oxide fuel cell stack comprises: multiple unit cells connected through conductors; fixing zigs positioned on both ends of the unit cells, respectively for supporting and fixing the both ends of the unit cells; and a manifold for supplying fuel to the unit cells and accommodating the unit cells and fixing zigs. The conductors connect the multiple unit cells electrically serially. The fixing zigs are made of a ceramic material. The fixing zigs can have multiple through holes in which a part of the unit cells is penetrated and fixed. Another embodiment of the present invention, a solid oxide fuel cell comprises: cylindrical unit cells; fixing zigs positioned in the both sides of the unit cells for fixing and supporting them; and a manifold for supplying fuel cell and accommodating the unit cells and fixing zigs. The unit cells comprise: a first electrode; an electrolyte layer positioned on the first electrode; a second electrode positioned on the electrolyte layer; and a spiral shaped conductor positioned on the second electrode to surround the outer periphery of the second electrode while being connected to the first electrode electrically. The fixing zigs comprise: multiple through holes for accommodating the both sides of the unit cells; and a sealing material for sealing and combining gas between the unit cells and fixing zigs.
Abstract translation: 本发明的一个实施例，一种固体氧化物燃料电池堆包括：通过导体连接的多个单元电池; 固定位于单元电池两端的夹具，用于支撑和固定单元电池的两端; 以及用于向单元电池供应燃料并容纳单位电池并固定电弧头的歧管。 导体串联连接多个单元电池。 固定夹具由陶瓷材料制成。 固定夹具可以具有多个通孔，其中一部分单元电池被穿透和固定。 本发明的另一个实施方案，固体氧化物燃料电池包括：圆柱形单元电池; 定位在单元电池两侧的固定夹具用于固定和支撑它们; 以及用于供应燃料电池并容纳所述单元电池并固定所述夹具的歧管。 单元电池包括：第一电极; 位于所述第一电极上的电解质层; 位于所述电解质层上的第二电极; 以及定位在所述第二电极上以围绕所述第二电极的外周边同时与所述第一电极电连接的螺旋状导体。 固定夹具包括：用于容纳单元电池两侧的多个通孔; 以及用于密封和组合单元电池和固定夹具之间的气体的密封材料。
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Patent Agency Ranking26.发明公开
公开(公告)号：KR1020130128572A
公开(公告)日：2013-11-27
申请号：KR1020120052380
申请日：2012-05-17
Applicant: 한국에너지기술연구원
Abstract: The present invention relates to a composite cathode for a solid oxide fuel cell, the solid oxide fuel cell including the same, and a manufacturing method thereof, wherein the composite cathode enhances oxygen reduction activity at low and middle temperatures by coating and dispersing Ag and CeO2 on a sintered oxide cathode layer having aperovskite structure and improves durability.
Abstract translation: 本发明涉及一种固体氧化物燃料电池用复合阴极，其固体氧化物型燃料电池及其制造方法，其中复合阴极通过涂布分散Ag和CeO 2来提高低温和中温下的氧还原活性 在具有钙钛矿结构的烧结氧化物阴极层上，提高耐久性。
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27.发明公开스크린 프린팅 방법에 의한 직접탄소 연료전지의 전해질층 형성방법 및 이를 이용한 직접탄소 연료전지의 제조방법 无效使用丝网印刷涂布方法制造直接碳素燃料电池的方法和方法，用于制造直接碳燃料电池
公开(公告)号：KR1020130124047A
公开(公告)日：2013-11-13
申请号：KR1020120047659
申请日：2012-05-04
Applicant: 한국에너지기술연구원
Abstract: The present invention relates to a method for fabricating an electrolyte layer of a direct carbon fuel cell using a screen printing coating method and a method for fabricating a direct carbon fuel cell therewith. The method for fabricating an electrolyte layer of a direct carbon fuel cell according to the present invention comprises the steps of: churning the mixture of electrolyte powder, a dispersant and a solvent (S1); producing paste by churning the mixture after adding the mixture of a binder and a solvent to the mixture (S2); milling the paste with a roll so as to disperse the electrolyte powder in the paste (S3); and conducting thermal treatment after coating the paste on an anode support by using a screen printing method (S4). According to the method for fabricating an electrolyte layer of a direct carbon fuel cell and the method for fabricating a direct carbon fuel cell, the performance and long-term stability of a direct carbon fuel cell can be improved by forming the electrolyte layer on the anode support to be a thin and compact coating layer. [Reference numerals] (S1) Step of churning the mixture of electrolyte powder, a dispersant and a solvent;(S2) Step of producing paste by churning the mixture after adding the mixture of a binder and a solvent to the mixture;(S3) Step of roll-milling the paste with a roll so as to disperse the electrolyte powder in the paste;(S4) Step of conducting thermal treatment after coating the paste on an anode support by using a screen printing method
Abstract translation: 本发明涉及使用丝网印刷涂布法制造直接碳燃料电池的电解质层的方法及其制造直接碳燃料电池的方法。 根据本发明的用于制造直接碳燃料电池的电解质层的方法包括以下步骤：搅拌电解质粉末，分散剂和溶剂的混合物（S1）; 通过在混合物（S2）中加入粘合剂和溶剂的混合物之后搅拌混合物来生产糊料; 用辊研磨糊剂以将电解质粉末分散在糊料中（S3）; 并且通过使用丝网印刷法（S4）将糊料涂覆在阳极支撑体上之后进行热处理。 根据直接碳燃料电池的电解质层的制造方法和直接碳燃料电池的制造方法，可以通过在阳极上形成电解质层来提高直接碳燃料电池的性能和长期稳定性 支持成为一个薄而紧凑的涂层。 （S1）将电解质粉末，分散剂和溶剂的混合物搅拌的步骤;（S2）向混合物中加入粘合剂和溶剂的混合物后，通过搅拌混合物来制造糊料的步骤;（S3） 用辊滚磨糊剂以使电解质粉末分散在糊料中的步骤;（S4）通过使用丝网印刷法将糊剂涂布在阳极支撑体上之后进行热处理的步骤
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公开(公告)号：KR1020130040311A
公开(公告)日：2013-04-24
申请号：KR1020110104971
申请日：2011-10-14
Applicant: 한국에너지기술연구원
CPC classification number: Y02P70/56 , H01M8/1213 , H01M8/0236 , H01M8/0245 , H01M2008/1293 , H01M2300/0074 , Y02E60/525
Abstract: PURPOSE: A bi-layer interconnector for a solid oxide fuel cell is provided to have high electric conductivity in a fuel electrode reduction atmosphere and in an air electrode oxidation atmosphere, and to be thinly and densely manufactured. CONSTITUTION: A bi-layer interconnector(100) for a solid oxide fuel cell consists of an n-type semiconductor layer(101) and a p-type semiconductor layer(102), The n-type semiconductor layer is formed of a perovskite SrTiO3 oxide The perovskite SrTiO3 oxide includes parts of Sr substituted by one or more elements selected from La, Y, Ce, Pr, Nd, Sm, Gd, and Pm, or parts of Ti substituted by one or more selected from Co, Mn, Fe, Cr, Cu, V, Ni, Zn, Ag, Au, Pt, Pd, Mo, W, and Si. The p-type semiconductor layer is formed of a perovskite LaMnO3 oxide. The perovskite LaMnO3 oxide includes parts of La substituted by one or more selected from Sr, Ca, Ba, and Mg, or parts of Mn are substituted by one or more selected from Co, Mn, Fe, Cr, Cu, V, Ni, Zn, Ag, Au, Pt, Pd, Mo, W, and Si. [Reference numerals] (AA) Air electrode; (BB) Fuel electrode;
Abstract translation: 目的：提供一种用于固体氧化物燃料电池的双层互连器，用于在燃料电极还原气氛和空气极氧化气氛中具有高导电性，并且被薄且致密地制造。 构成：用于固体氧化物燃料电池的双层互连器（100）由n型半导体层（101）和p型半导体层（102）组成.n型半导体层由钙钛矿型SrTiO 3 氧化物钙钛矿SrTiO3氧化物包括被选自La，Y，Ce，Pr，Nd，Sm，Gd和Pm中的一种或多种元素取代的Sr的部分，或被选自Co，Mn，Fe中的一种或多种 ，Cr，Cu，V，Ni，Zn，Ag，Au，Pt，Pd，Mo，W和Si。 p型半导体层由钙钛矿型LaMnO 3氧化物形成。 钙钛矿LaMnO3氧化物包括被选自Sr，Ca，Ba和Mg中的一种或多种的La取代的部分，或部分Mn被选自Co，Mn，Fe，Cr，Cu，V，Ni， Zn，Ag，Au，Pt，Pd，Mo，W和Si。 （标号）（AA）空气电极; （BB）燃料电极;
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公开(公告)号：KR1020130035460A
公开(公告)日：2013-04-09
申请号：KR1020110099765
申请日：2011-09-30
Applicant: 한국에너지기술연구원
Abstract: PURPOSE: A bundle module for a fuel cell is provided to improve electricity efficiency by uniformly supplying fuel gas to a plurality of unit batteries and gas channels. CONSTITUTION: A bundle module for a fuel cell comprises a support on which two or more unit batteries which includes an interconnector and an air electrode formed on both sides of the support with a gas channel; an inlet manifold(200a) which is connected to a supply pipe(21) to one end, has an outlet at the opposite end, homogenizes a flux of the fuel gas to two or more gas channels of each unit battery; and an outlet manifold(220a) transferring exhaust gas from the bundle to the outlet.
Abstract translation: 目的：提供一种用于燃料电池的束模块，用于通过向多个单元电池和气体通道均匀地供应燃料气体来提高电力效率。 构成：用于燃料电池的束模块包括支撑件，两个或更多个单元电池包括互连器和形成在支撑件的两侧的空气电极，其中气体通道具有气体通道; 连接到一端的供给管（21）的入口歧管（200a）具有在相对端的出口，将燃料气体的通量均匀化为每个单位电池的两个或更多个气体通道; 以及将废气从束传送到出口的出口歧管（220a）。
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公开(公告)号：KR101226962B1
公开(公告)日：2013-01-28
申请号：KR1020110023276
申请日：2011-03-16
Applicant: 한국에너지기술연구원
IPC: C04B35/624 , C04B35/622 , C04B35/50 , H01M8/02
CPC classification number: Y02P70/56
Abstract: 본 발명은 고체산화물 연료전지(Solid Oxide Fuel Cell, SOFC)의 접속자 제조용 세라믹 분말에 관한 것으로, 페로브스카이트 구조를 가지며 란탄 (La), 칼슘 (Ca) 및 크롬(Cr)을 함유하는 나노 크기의 세라믹 접속자 분말을 제조하는 방법 및 그 세라믹 분말로 제조된 접속자에 관한 것이다.
본 발명의 방법은, 각기 란탄, 칼슘 및 크롬을 함유하는 질산염을 출발물질로 하여 이를 증류수에 용해시키는 단계; 상기 금속질산염 용액에 연료물질로서의 글리신을 첨가하여 졸(sol)을 얻는 단계;상기 졸 용액을 가열하여 물을 증발시킴으로써 겔(gel)을 제조하는 단계;상기 겔을 계속 가열하여 열분해시키는 단계; 상기 열분해된 겔을 건조 공기와 접촉시키면서 고온에서 열처리하는 단계로 이루어진다.
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