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    SOLID OXIDE FUEL BATTERY CELL
    71.
    发明申请
    SOLID OXIDE FUEL BATTERY CELL 审中-公开
    固体氧化物燃料电池

    公开(公告)号：US20130183594A1

    公开(公告)日：2013-07-18

    申请号：US13728021

    申请日：2012-12-27

    Applicant: Toto Ltd.

    Inventor： Hiroshi NIIMI ,  Akira KAWAKAMI ,  Shigeru ANDO ,  Masayoshi YUZURIHARA ,  Ryoichi NISHIMIZU

    IPC: H01M4/86 ,  H01M12/06

    CPC classification number: H01M4/8657 ,  H01M4/8889 ,  H01M4/9033 ,  H01M4/9058 ,  H01M4/9066 ,  H01M8/0232 ,  H01M8/0236 ,  H01M8/0243 ,  H01M12/06 ,  H01M2008/1293

    Abstract: Disclosed is a solid oxide fuel battery cell having a high initial power generation performance and a good power generation durability while ensuring adhesion between an air electrode and a current collector. The solid oxide fuel battery cell includes a solid electrolyte, a fuel electrode, an air electrode, and a current collector provided on the surface of the air electrode, wherein the air electrode is formed of lanthanum ferrite perovskite oxides, lanthanum cobalt perovskite oxides, or samarium cobalt perovskite oxides, and the current collector is porous including silver, palladium, and an oxide and has an average porosity of 20% to 70% in a portion other than a portion near a boundary between the current collector and the air electrode and, in the near-boundary portion, an average porosity of not less than 50% of the average porosity of the portion other than the near-boundary portion.

    Abstract translation: 公开了一种固体氧化物燃料电池，其具有高的初始发电性能和良好的发电耐久性，同时确保空气电极和集电器之间的粘附。 固体氧化物燃料电池单元包括设置在空气电极表面上的固体电解质，燃料电极，空气电极和集电器，其中空气电极由铁酸镧钙钛矿氧化物，镧钴钙钛矿氧化物或 钐钴钙钛矿氧化物，并且集电体是多孔的，包括银，钯和氧化物，并且在除了集电器和空气电极之间的边界附近的部分之外的平均孔隙率为20％至70％，并且， 在近边界部分中，平均孔隙率不小于近边界部分以外的部分的平均孔隙率的50％。

    PROCESS FOR MANUFACTURING ELEMENTARY ELECTROCHEMICAL CELLS FOR ENERGY- OR HYDROGEN-PRODUCING ELECTROCHEMICAL SYSTEMS, IN PARTICULAR OF SOFC AND HTE TYPE
    72.
    发明申请
    PROCESS FOR MANUFACTURING ELEMENTARY ELECTROCHEMICAL CELLS FOR ENERGY- OR HYDROGEN-PRODUCING ELECTROCHEMICAL SYSTEMS, IN PARTICULAR OF SOFC AND HTE TYPE 有权
    用于生产电化学系统的电化学电池的制备方法，特别是SOFC和HTE型

    公开(公告)号：US20130082421A1

    公开(公告)日：2013-04-04

    申请号：US13703516

    申请日：2011-06-10

    Applicant: Alexandre Allemand ,  Sophie Beaudet Savignat ,  Eric Bruneton

    Inventor： Alexandre Allemand ,  Sophie Beaudet Savignat ,  Eric Bruneton

    IPC: H01M8/10 ,  C25B1/02

    CPC classification number: H01M8/1016 ,  C25B1/02 ,  C25B9/00 ,  H01M4/8621 ,  H01M4/8663 ,  H01M4/8889 ,  H01M8/0206 ,  H01M8/0213 ,  H01M8/0215 ,  H01M8/1213 ,  Y02E60/521 ,  Y02E60/525

    Abstract: The invention relates to a process for manufacturing at least one elementary electrochemical cell comprising a first and a second electrode between which an electrolyte is intercalated, said first and second electrodes and said electrolyte being in the form of layers, which process is characterized in that it comprises: a) producing at least one structure comprising a layer of a powder of a first electrode material and a layer of a powder of a second electrode material between which a layer of a powder of an electrolyte material is intercalated; and b) simultaneously sintering all the powder layers by an electric field sintering. Applications: manufacture of energy- or hydrogen-producing electrochemical systems, in particular solid oxide fuel cells (SOFCs) or high temperature electrolysers cells (HTEs).

    Abstract translation: 本发明涉及一种用于制造至少一个基本电化学电池的方法，该电化学电池包括第一和第二电极，其间插入有电解质，所述第一和第二电极和所述电解质为层的形式，其特征在于， 包括：a）产生至少一种结构，其包括第一电极材料的粉末层和第二电极材料的粉末层，其间插入电解质材料的粉末层; 和b）通过电场烧结同时烧结所有的粉末层。 应用：制造生产能量或氢的电化学系统，特别是固体氧化物燃料电池（SOFC）或高温电解槽电池（HTE）。

    SOLID OXIDE FUEL CELL
    73.
    发明申请
    SOLID OXIDE FUEL CELL 有权
    固体氧化物燃料电池

    公开(公告)号：US20120237849A1

    公开(公告)日：2012-09-20

    申请号：US13421969

    申请日：2012-03-16

    Applicant: Ayano KOBAYASHI ,  Makoto Ohmori

    Inventor： Ayano KOBAYASHI ,  Makoto Ohmori

    IPC: H01M8/10 ,  H01M4/86

    CPC classification number: H01M4/86 ,  H01M4/8621 ,  H01M4/8642 ,  H01M4/8889 ,  H01M4/9066 ,  H01M8/10 ,  H01M8/1213 ,  H01M8/1231 ,  H01M8/1253 ,  H01M2008/1293 ,  Y02E60/521 ,  Y02E60/525 ,  Y02P70/56

    Abstract: The present invention provides a solid oxide fuel cell (SOFC) including a “porous fuel electrode which allows reaction of a fuel gas to proceed and which is formed of Ni and YSZ”; a “porous air electrode which allows reaction of an oxygen-containing gas to proceed”; and a “dense solid electrolyte membrane which is provided between the fuel electrode and the air electrode and which has an interface with the fuel electrode.” In the fuel electrode, Ni grains present in a region located within 3 μm from the interface (i.e., a “near-interface region”) have a mean size of 0.28 to 0.80 μm; YSZ grains present in the “near-interface region” have a mean size of 0.28 to 0.80 μm; and pores present in the “near-interface region” have a mean size of 0.10 to 0.87 μm. Thus, the fuel electrode of the SOFC exhibits low reaction resistance.

    Abstract translation: 本发明提供一种固体氧化物型燃料电池（SOFC），其包括能够进行燃料气体的反应而由Ni和YSZ形成的多孔质燃料电极; “允许含氧气体进行反应的”多孔空气电极“; 以及在燃料电极和空气极之间设置并具有与燃料极的界面的“密实的固体电解质膜”。在燃料电极中，存在于距界面3μm以内的区域的Ni晶粒（即， “近界面区域”）的平均粒径为0.28〜0.80μm; 存在于“近界面区域”的YSZ晶粒的平均粒径为0.28〜0.80μm; 并且存在于“近界面区域”中的孔的平均尺寸为0.10〜0.87μm。 因此，SOFC的燃料电极具有低反应性。

    FUEL CELL WITH A BRAZED INTERCONNECT AND METHOD OF ASSEMBLING THE SAME
    75.
    发明申请
    FUEL CELL WITH A BRAZED INTERCONNECT AND METHOD OF ASSEMBLING THE SAME 审中-公开
    燃料电池与BRAZED互连及其组装方法

    公开(公告)号：US20110269054A1

    公开(公告)日：2011-11-03

    申请号：US13183161

    申请日：2011-07-14

    Applicant: Wayne Charles Hasz

    Inventor： Wayne Charles Hasz

    IPC: H01M8/10 ,  B23K31/02 ,  H01M8/00

    CPC classification number: H01M4/8889 ,  H01M4/8885 ,  H01M8/0232 ,  H01M8/0273 ,  H01M8/0282 ,  H01M8/0286 ,  H01M8/0297 ,  H01M8/1213 ,  H01M8/1246 ,  Y02E60/525 ,  Y02P70/56

    Abstract: A fuel cell including an anode, a cathode and an electrolyte interposed between the anode and the cathode is disclosed. The fuel cell also includes an anode interconnect disposed adjacent to the anode, and a brazing material disposed between the anode interconnect and the anode to bond the anode interconnect to the anode. A method of assembling a fuel cell including forming a package of an anode and an electrolyte is also disclosed. It includes heating the package with a brazing material disposed adjacent to the anode, to bond the anode to an interconnect.

    Abstract translation: 公开了一种包括阳极，阴极和介于阳极和阴极之间的电解质的燃料电池。 燃料电池还包括邻近阳极设置的阳极互连和设置在阳极互连和阳极之间的钎焊材料，以将阳极互连件接合到阳极。 还公开了一种组装包括形成阳极和电解质的封装的燃料电池的方法。 它包括用邻近阳极设置的钎焊材料加热封装，以将阳极粘合到互连件上。

    Low-temperature bonding of refractory ceramic layers
    78.
    发明申请
    Low-temperature bonding of refractory ceramic layers 有权
    难熔陶瓷层的低温结合

    公开(公告)号：US20100075194A1

    公开(公告)日：2010-03-25

    申请号：US12284499

    申请日：2008-09-23

    Applicant: Kailash C. Jain ,  Rick D. Kerr ,  Bryan Gillispie ,  Mohammad Parsian ,  Joseph M. Keller ,  David A. Thompson

    Inventor： Kailash C. Jain ,  Rick D. Kerr ,  Bryan Gillispie ,  Mohammad Parsian ,  Joseph M. Keller ,  David A. Thompson

    IPC: H01M8/10 ,  B32B38/00

    CPC classification number: H01M4/8657 ,  H01M4/8889 ,  H01M4/9016 ,  H01M4/9033 ,  H01M8/1253 ,  H01M2004/8689 ,  H01M2008/1293 ,  Y02E60/521 ,  Y02E60/525 ,  Y02P70/56

    Abstract: A cathode of a solid-oxide fuel cell includes a first ionic conducting layer, a second layer deposited over the first layer and formed from a mixed ionic and electronic conductor layer including an oxygen ion conducting phase, and a third layer deposited over the second layer and formed from a mixed ionic and electronic conductor layer. A sintering aid and pore formers are added to the second layer and the third layer to establish ionic, electronic, and gas diffusion paths that are contiguous. By adjusting the microstructure of the second and the third layer, a high performance low resistance cathode is formed that bonds well to the electrolyte, is highly electro-catalytic, and has a relatively low overall resistance. By using inexpensive and readily available substances as sintering aid and as pore formers, a low-cost cathode is provided.

    Abstract translation: 固体氧化物燃料电池的阴极包括第一离子导电层，沉积在第一层上并由包括氧离子传导相的混合离子和电子导体层形成的第二层，以及沉积在第二层上的第三层 并由混合的离子和电子导体层形成。 向第二层和第三层加入烧结助剂和成孔剂以建立邻接的离子，电子和气体扩散路径。 通过调整第二层和第三层的微结构，形成了与电解质结合良好的高性能低电阻阴极，高电催化，总体电阻较低。 通过使用便宜且容易获得的物质作为烧结助剂和成孔剂，提供了低成本的阴极。

    Current collector to conduct an electrical current to or from an electrode layer
    79.
    发明授权
    Current collector to conduct an electrical current to or from an electrode layer 有权
    电流集电器，用于向电极层或从电极层传导电流

    公开(公告)号：US07449262B2

    公开(公告)日：2008-11-11

    申请号：US11007220

    申请日：2004-12-09

    Applicant: Gervase Maxwell Christie ,  Jonathan Andrew Lane

    Inventor： Gervase Maxwell Christie ,  Jonathan Andrew Lane

    IPC: H01M4/64 ,  H01M4/66 ,  H01M4/86

    CPC classification number: H01M8/0236 ,  B22F3/11 ,  B22F7/002 ,  B22F2998/00 ,  C22C32/001 ,  H01M4/8621 ,  H01M4/8889 ,  H01M8/0232 ,  H01M8/0245 ,  H01M8/1231 ,  H01M2008/1293 ,  Y02P70/56 ,  B22F1/02

    Abstract: A current collector and method of forming the same in which a slurry is prepared that contains electrically conductive particles having surface deposits of a metallic oxide on a metal or metal alloy conductor that has a lower weight percentage of the electrically conductive particles than the metal or metal alloy. The slurry is applied to a structure that contains an electrolyte and electrode layers. The resultant coated form is then fired to partly sinter the electrically conductive particles and thereby to obtain porous current collector layers affixed to the electrode layers. The current collector of the present invention is between about 5 microns and about 100 microns thick and preferably has a porosity of between about 10 percent and about 70 percent with pores having a pore size of between about 0.1 microns and about 20 microns.

    Abstract translation: 一种集流体及其制备方法，其中制备了一种浆料，其含有在金属或金属合金导体上具有金属氧化物表面沉积物的导电颗粒，该导电颗粒具有比金属或金属更低的导电颗粒重量百分比 合金。 将浆料施加到包含电解质和电极层的结构。 然后将所得涂层形式烧制以部分地烧结导电颗粒，从而获得固定到电极层的多孔集电器层。 本发明的集电器的厚度在约5微米至约100微米之间，优选具有约10％至约70％之间的孔隙率，孔径为约0.1微米至约20微米。

    Method of forming membrane electrode assemblies for electrochemical devices
    80.
    发明申请
    Method of forming membrane electrode assemblies for electrochemical devices 有权
    形成电化学装置的膜电极组件的方法

    公开(公告)号：US20080182150A1

    公开(公告)日：2008-07-31

    申请号：US11700407

    申请日：2007-01-30

    Applicant: David S. De Haan ,  Ben Tham ,  Liviu Catoiu

    Inventor： David S. De Haan ,  Ben Tham ,  Liviu Catoiu

    IPC: H01M2/00 ,  B32B37/00

    CPC classification number: B32B37/26 ,  B32B2457/18 ,  H01M4/8605 ,  H01M4/8657 ,  H01M4/881 ,  H01M4/8889 ,  H01M4/8896 ,  H01M8/028 ,  H01M8/0297 ,  H01M8/1004 ,  H01M8/241 ,  H01M8/2457 ,  Y10T156/10

    Abstract: A method of forming a membrane electrode assembly (MEA) includes first bonding a first electrode layer to a first side of an ion-exchange membrane. The method may further include protecting a second side of the membrane with a release sheet. The method may further include removing the release sheet and bonding the second side of the membrane to a first side of a second electrode layer. The method may further include positioning venting members on a second side of the second electrode layer to remove at least one of a liquid and a vapor that may be generated during the bonding process. In another embodiment an electrocatalyst can first bond to at least one side of the membrane, and subsequently, to a gas diffusion layer. An opposing side of the membrane can bond to an electrode layer in aqueous state.

    Abstract translation: 形成膜电极组件（MEA）的方法包括：首先将第一电极层接合到离子交换膜的第一侧。 该方法还可以包括用剥离片保护膜的第二侧。 该方法还可以包括去除剥离片并将膜的第二面粘合到第二电极层的第一侧。 该方法还可以包括将排气构件定位在第二电极层的第二侧上以去除在接合过程中可能产生的液体和蒸汽中的至少一种。 在另一个实施方案中，电催化剂可以首先结合至膜的至少一侧，随后结合到气体扩散层。 膜的相对侧可以以水性状态结合到电极层。

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