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    Reactor comprising a packed bed of supported catalyst or supported catalyst precursor, and a use of the reactor
    11.
    发明申请
    Reactor comprising a packed bed of supported catalyst or supported catalyst precursor, and a use of the reactor 审中-公开
    反应器包括负载催化剂的填充床或负载型催化剂前体，以及反应器的用途

    公开(公告)号：US20030162848A1

    公开(公告)日：2003-08-28

    申请号：US10333888

    申请日：2003-02-28

    Inventor： Frederik Willem Hendrik Gimpel ,  Robert Martijn Van Hardeveld ,  Carolus Matthias Anna Maria Mesters ,  Gerardus Petrus Lambertus Niesen ,  Franciscus Johannes Maria Schrauwen

    IPC: B01J008/02 ,  B01J035/02 ,  C07C027/06

    CPC classification number: C10G2/341 ,  B01J8/008 ,  B01J8/02 ,  B01J12/007 ,  B01J23/8892 ,  B01J2208/00805

    Abstract: A reactor comprising a packed bed of supported catalyst or supported catalyst precursor wherein the supported cata-lyst or the supported catalyst precursor comprise an external surface comprising a catalytically active metal or a precursor compound thereof, and the packed bed has a void content of more than 50% v and a specific surface area of more than 10 cm2/cm3, which is calculated as the total external surface area of the particles relative to the bed volume; the use of the said reactor in a chemical conversion process; a process for preparing hydrocarbons from syngas, which process comprises contacting a mixture of carbon monoxide and hydrogen in the said reactor, on the understanding that the catalytically active metal is a Group VIII metal which is at least in part present in metallic form; a packed bed of catalyst particles or catalyst precursor particles; and a catalyst particle or catalyst precursor particle.

    Abstract translation: 一种包含负载催化剂或负载型催化剂前体的填充床的反应器，其中负载的催化剂或负载的催化剂前体包含包含催化活性金属或其前体化合物的外表面，并且填充床的空隙含量大于 50％v和大于10cm 2 / cm 3的比表面积，其计算为颗粒相对于床体积的总外表面积; 在化学转化过程中使用所述反应器; 从合成气制备烃的方法，该方法包括在所述反应器中使一氧化碳和氢气的混合物接触，理解催化活性金属是至少部分以金属形式存在的第Ⅷ族金属; 催化剂颗粒或催化剂前体颗粒的填充床; 和催化剂颗粒或催化剂前体颗粒。

    Chemical microreactor and method thereof
    14.
    发明申请
    Chemical microreactor and method thereof 失效
    化学微反应器及其方法

    公开(公告)号：US20030103878A1

    公开(公告)日：2003-06-05

    申请号：US10007412

    申请日：2001-12-05

    Applicant: The Regents of the University of California

    Inventor： Jeffrey D. Morse ,  Alan Jankowski

    IPC: B01J008/02 ,  B01L007/00

    CPC classification number: B01J19/0093 ,  B01J2219/00783 ,  B01J2219/00824 ,  B01J2219/00828 ,  B01J2219/00831 ,  B01J2219/00835 ,  B01J2219/00844 ,  B01J2219/00871 ,  B01J2219/00873

    Abstract: Disclosed is a chemical microreactor that provides a means to generate hydrogen fuel from liquid sources such as ammonia, methanol, and butane through steam reforming processes when mixed with an appropriate amount of water. The microreactor contains capillary microchannels with integrated resistive heaters to facilitate the occurrence of catalytic steam reforming reactions. Two distinct embodiment styles are discussed. One embodiment style employs a packed catalyst capillary microchannel and at least one porous membrane. Another embodiment style employs a porous membrane with a large surface area or a porous membrane support structure containing a plurality of porous membranes having a large surface area in the aggregate, i.e., greater than about 1 m2/cm3. Various methods to form packed catalyst capillary microchannels, porous membranes and porous membrane support structures are also disclosed.

    Abstract translation: 公开了一种化学微反应器，其提供了当与适量的水混合时通过蒸汽重整过程从液体源例如氨，甲醇和丁烷产生氢燃料的手段。 微反应器包含具有集成电阻加热器的毛细管微通道，以促进催化蒸汽重整反应的发生。 讨论了两种不同的实施方式。 一种实施方案采用填充催化剂毛细管微通道和至少一种多孔膜。 另一种实施方案采用具有大表面积的多孔膜或多孔膜支撑结构，其包含多个聚集体中具有大表面积的多孔膜，即大于约1m 2 / cm 3。 还公开了形成填充催化剂毛细管微通道，多孔膜和多孔膜支撑结构的各种方法。

    Contact, mixing, and quenching box for fluids, comprising at least one annular peripheral outlet and reaction cell with an elongated shape along an axis including said box
    17.
    发明申请
    Contact, mixing, and quenching box for fluids, comprising at least one annular peripheral outlet and reaction cell with an elongated shape along an axis including said box 有权
    用于流体的接触，混合和淬火箱包括至少一个环形外围出口和沿着包括所述箱体的轴线具有细长形状的反应池

    公开(公告)号：US20030031612A1

    公开(公告)日：2003-02-13

    申请号：US10187432

    申请日：2002-07-02

    Inventor： Ludovic Raynal ,  Isabelle Harter ,  Francis Aubry

    IPC: B01J008/02

    CPC classification number: C10G49/002 ,  B01F5/0068 ,  B01J8/008 ,  B01J8/0453 ,  B01J8/0492 ,  B01J8/0496 ,  B01J2208/00362 ,  B01J2208/00849

    Abstract: Contact, mixing, and often quenching box (8), with main dimension (D) and height (H7), comprising at least one duct section (B1) located on the upper part of said box (8) for entry of fluids in which said box (8) comprises, downstream from said duct section (B1), in the direction in which the fluids circulate, a means (B4) that provides, in said box (8), for making the fluids swirl in an approximately nonradial direction, and not parallel to the overall direction of circulation of said fluids, and comprising at least one annular, peripheral duct section (B6) for the exit of said mixture of fluids formed in said box (8) whose lower level is located above the upper level for fluid entry through at least one lateral inlet (B3) located in said box (8) above means (B4). Reaction cell (4), of an elongated shape along an approximately vertical axis comprising said contact, mixing, and quenching box (8) and use of this cell for performing exothermic reactions.

    Abstract translation: 具有主要尺寸（D）和高度（H7）的接触，混合和经常淬火箱（8）包括位于所述箱体（8）的上部的至少一个管道段（B1），用于进入流体 所述箱体（8）包括在所述管道部分（B1）的下游，沿着所述流体循环的方向，在所述箱体（8）中提供用于使所述流体在近似非辐射方向上旋转的装置（B4） 并且不平行于所述流体的总体循环方向，并且包括至少一个环形周边导管段（B6），用于排出所述箱体（8）中形成的所述流体混合物，所述混合物的下层位于上部 流体通过位于装置（B4）上方的所述盒（8）中的至少一个侧向入口（B3）的液体进入。 沿着包括所述接触，混合和淬火箱（8）的近似垂直轴的细长形状的反应池（4）和该电池用于进行放热反应的用途。

    Shift converter having an improved catalyst composition
    18.
    发明申请
    Shift converter having an improved catalyst composition 审中-公开
    具有改进的催化剂组成的换档转化器

    公开(公告)号：US20030007912A1

    公开(公告)日：2003-01-09

    申请号：US10217398

    申请日：2002-08-13

    Inventor： Ronald G. Silver

    IPC: B01J008/02

    CPC classification number: B01J23/63 ,  B01J8/025 ,  B01J21/066 ,  C01B3/16 ,  H01M8/0662 ,  Y02P20/52

    Abstract: A shift converter (16) in a fuel processing subsystem (14, 16, 18) for a fuel cell (12) uses an improved catalyst composition (50) to reduce the amount of carbon monoxide in a process gas for the fuel cell (12). The catalyst composition (50) is a noble metal catalyst having a promoted support of mixed metal oxide, including at least both ceria and zirconia. Cerium is present in the range of 30 to 50 mole %, and zirconium is present in the range of 70 to 50 mole %. Additional metal oxides may also be present. Use of the catalyst composition (50) obviates the requirement for prior reducing of catalysts, and minimizes the need to protect the catalyst from oxygen during operation and/or shutdown.

    Abstract translation: 用于燃料电池（12）的燃料处理子系统（14,16,18）中的换档转换器（16）使用改进的催化剂组合物（50）来减少燃料电池（12）的处理气体中的一氧化碳 ）。 催化剂组合物（50）是具有至少包括二氧化铈和氧化锆两者的混合金属氧化物的促进载体的贵金属催化剂。 铈的存在量为30〜50摩尔％，锆的含量为70〜50摩尔％。 另外的金属氧化物也可以存在。 催化剂组合物（50）的使用避免了先前还原催化剂的要求，并且最小化在操作和/或停止期间保护催化剂免受氧气的需要。

    Thin multi-stage catalytic reactor with internal heat exchanger, and use thereof
    19.
    发明申请
    Thin multi-stage catalytic reactor with internal heat exchanger, and use thereof 有权
    具有内部热交换器的薄型多级催化反应器及其应用

    公开(公告)号：US20020159933A1

    公开(公告)日：2002-10-31

    申请号：US10084493

    申请日：2002-02-28

    Applicant: Institut Francais du Petrole

    Inventor： Frederic Hoffmann ,  Eric Lenglet ,  Philippe Mege

    IPC: B01J008/12 ,  B01J008/02

    CPC classification number: B01J8/085 ,  B01J8/003 ,  B01J8/004 ,  B01J8/0426 ,  B01J8/0496 ,  B01J8/125 ,  B01J2208/00168 ,  B01J2219/185 ,  B01J2219/1943

    Abstract: An elongate reaction vessel includes at least two stages in the vertical direction in which an endothermic or exothermic catalytic reaction is carried out and comprises: A catalytic reaction zone (12a, 12b) per stage (6, 7); Introducing (2) a reaction fluid to a stage adapted for transverse motion of the fluid across the whole vertical extent of the reaction zone; introducing and extracting the catalyst; a heat exchanger (5a) for reaction fluids located inside the vessel between two successive reaction zones; means (6) for transporting reaction fluids from one stage to another preferably connected to the exchanger of the stage under consideration and to the inlet for reaction fluids of the subsequent stage; means for recovering reaction fluids downstream of the last stage. The temperature variation in each zone and the temperature level are respectively adjusted by the thickness of each zone and by heat exchange.

    Abstract translation: 细长反应容器包括在垂直方向上至少两个阶段，其中进行吸热或放热催化反应，并包括：每级催化反应区（12a，12b）（6,7）; 将反应流体引入（2）反应流体，以适应流体在整个反应区域的整个垂直范围内的横向运动; 引入和提取催化剂; 用于位于两个连续反应区之间的反应流体的热交换器（5a）; 用于将反应流体从一个阶段转移到另一个阶段的装置（6），优选地连接到所考虑的阶段的交换器和后续阶段的反应流体的入口; 用于在最后阶段下游回收反应液的装置。 每个区域的温度变化和温度水平分别通过每个区域的厚度和通过热交换来调整。

    Graded catalyst bed for split-feed hydrocracking/hydrotreating
    20.
    发明申请
    Graded catalyst bed for split-feed hydrocracking/hydrotreating 有权
    分级催化剂床用于分流加氢裂化/加氢处理

    公开(公告)号：US20020146358A1

    公开(公告)日：2002-10-10

    申请号：US09826476

    申请日：2001-04-04

    Inventor： Ben D. Smith ,  Richard O. Moore JR.

    IPC: B01J008/04 ,  B01J008/02

    CPC classification number: B01J8/0446 ,  B01J8/0085 ,  B01J2208/00805 ,  C10G65/12

    Abstract: A method for hydroprocessing hydrocarbon products, preferably Fischer-Tropsch products, and a reactor useful for performing the method, are disclosed. The reactor includes one or more first catalyst beds comprising a catalyst useful for conducting relatively severe hydroprocessing and one or more second catalyst beds comprising a catalyst useful for conducting relatively mild hydroprocessing. The second catalyst beds are located at a position in the reactor where they can receive the products from the first catalyst bed(s), at least one of each of the first and second catalyst bed(s) comprises a catalyst grading scheme sufficient to remove at least a portion of any particulates from their respective feeds, and the reactor is set up to receive hydrocarbon feeds at a position above or within the first catalyst bed(s) and above or within the second catalyst bed(s). A first hydrocarbon feed with a relatively high boiling point is introduced to the first catalyst bed(s) and is subjected to relatively severe hydroprocessing. A feed comprising 1) the products from the hydroprocessing of the first hydrocarbon feed and 2) a second hydrocarbon feed with a relatively low boiling point is introduced to the second catalyst beds and is subjected to relatively mild hydroprocessing. The catalyst grading scheme minimizes pressure drop build-up through the catalyst beds. The hydrocarbon feeds are preferably derived, in whole or in part, from Fischer-Tropsch synthesis, although they can include products from petroleum refining or other suitable sources. In one embodiment, the relatively high boiling fraction is a predominantly C20null fraction and the relatively low boiling fraction is a predominantly C5-20 fraction.

    Abstract translation: 公开了一种用于加氢处理烃产物，优选费 - 托产物的方法和用于实施该方法的反应器。 反应器包括一种或多种第一催化剂床，其包含可用于进行相对严格的加氢处理的催化剂和一种或多种第二催化剂床，其包含用于进行相对温和的加氢处理的催化剂。 第二催化剂床位于反应器中可以从第一催化剂床接收产物的位置，第一和第二催化剂床中的每一个中的至少一个包括足以除去的催化剂分级方案 至少一部分来自它们各自进料的任何颗粒，并且反应器设置为在第一催化剂床上方或第一催化剂床上方或第二催化剂床内的位置处接收烃进料。 将具有较高沸点的第一烃进料引入第一催化剂床并进行相对严格的加氢处理。 一种饲料，其包括1）来自第一烃进料的加氢处理的产物和2）具有相对低沸点的第二烃进料引入第二催化剂床并进行相对温和的加氢处理。 催化剂分级方案使通过催化剂床的压降累积最小化。 烃进料优选全部或部分来自费 - 托合成，尽管它们可以包括来自石油精炼或其它合适来源的产物。 在一个实施方案中，较高沸点馏分主要是C20 +馏分，相对低沸点馏分主要是C5-20馏分。

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