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    OLEFIN METATHESIS CATALYSTS AND RELATED METHODS
    65.
    发明申请
    OLEFIN METATHESIS CATALYSTS AND RELATED METHODS 有权
    OLEFIN METATHESIS催化剂及相关方法

    公开(公告)号：US20110237815A1

    公开(公告)日：2011-09-29

    申请号：US13033472

    申请日：2011-02-23

    Applicant: Adam S. Hock ,  Richard R. Schrock

    Inventor： Adam S. Hock ,  Richard R. Schrock

    IPC: C07F11/00

    CPC classification number: B01J31/2295 ,  B01J31/122 ,  B01J31/1805 ,  B01J31/181 ,  B01J31/2234 ,  B01J31/2265 ,  B01J31/2291 ,  B01J2231/482 ,  B01J2231/54 ,  B01J2231/543 ,  B01J2531/64 ,  B01J2531/66 ,  C07C6/04 ,  C07C2531/22

    Abstract: The present invention provides methods for the synthesis of catalysts and precursors thereof. Methods of the invention may comprise combining a catalyst precursor and at least one ligand to generate a catalytically active species, often under mild conditions and in high yields. In some cases, a wide variety of catalysts may be synthesized from a single catalyst precursor. Methods of the invention may also include the preparation of catalysts which, under reaction conditions known in the art, may have been difficult or impossible to prepare and/or isolate due to, for example, steric crowding at the metal center. The present invention also provides catalyst compositions, and precursors thereof, which may be useful in various chemical reactions including olefin metathesis. In some cases, methods of the invention may reduce the number of synthetic and purification steps required to produce catalysts and/or other reaction products, as well as reducing time, cost, and waste production.

    Abstract translation: 本发明提供合成催化剂及其前体的方法。 本发明的方法可以包括将催化剂前体和至少一种配体结合以产生催化活性物质，通常在温和条件下和高产率下。 在一些情况下，可以从单一催化剂前体合成多种催化剂。 本发明的方法还可以包括催化剂的制备，其在本领域已知的反应条件下可能由于例如在金属中心的空间拥挤而难以或不可能制备和/或分离。 本发明还提供催化剂组合物及其前体，其可用于包括烯烃复分解的各种化学反应。 在一些情况下，本发明的方法可以减少制备催化剂和/或其它反应产物所需的合成和纯化步骤的数量，以及减少时间，成本和废物的产生。

    Copper-catalysed ligation of azides and acetylenes
    67.
    发明申请
    Copper-catalysed ligation of azides and acetylenes 有权
    铜催化的叠氮化物和乙炔的连接

    公开(公告)号：US20110105764A1

    公开(公告)日：2011-05-05

    申请号：US12804644

    申请日：2010-07-26

    Applicant: K. Barry Sharpless ,  Valery Fokin ,  Vsevold A. Rostovtsev ,  Luke Green ,  Fahmi Himo

    Inventor： K. Barry Sharpless ,  Valery Fokin ,  Vsevold A. Rostovtsev ,  Luke Green ,  Fahmi Himo

    IPC: C07D249/04

    CPC classification number: C07D249/04 ,  B01J31/1805 ,  B01J2231/327 ,  B01J2531/16 ,  B01J2531/96 ,  C07D249/06 ,  C07D403/06

    Abstract: A copper catalyzed click chemistry ligation process is employed to bind azides and terminal acetylenes to provide 1,4-disubstituted 1,2,3-triazole triazoles. The process comprises contacting an organic azide and a terminal alkyne with a source of reactive Cu(I) ion for a time sufficient to form by cycloaddition a 1,4-disubstituted 1,2,3-triazole. The source of reactive Cu(I) ion can be, for example, a Cu(I) salt or copper metal. The process is preferably carried out in a solvent, such as an aqueous alcohol. Optionally, the process can be performed in a solvent that comprises a ligand for Cu(I) and an amine.

    Abstract translation: 使用铜催化的点击化学连接方法结合叠氮化物和末端炔烃以提供1,4-二取代的1,2,3-三唑三唑。 该方法包括使有机叠氮化物和末端炔与活性Cu（I）离子源接触一段时间，足以通过环加成1,4-二取代的1,2,3-三唑形成。 反应性Cu（I）离子的来源可以是例如Cu（I）盐或铜金属。 该方法优选在溶剂如乙醇中进行。 任选地，该方法可以在包含Cu（I）和胺的配体的溶剂中进行。

    Process for homo- or copolymerization of conjugated olefins
    68.
    发明授权
    Process for homo- or copolymerization of conjugated olefins 有权
    共轭烯烃的均相或共聚方法

    公开(公告)号：US07915194B2

    公开(公告)日：2011-03-29

    申请号：US12557121

    申请日：2009-09-10

    Applicant: Sven K. H. Thiele

    Inventor： Sven K. H. Thiele

    IPC: B01J31/22 ,  B01J31/14 ,  C08F4/52

    CPC classification number: B01J31/143 ,  B01J31/146 ,  B01J31/1805 ,  B01J2531/0216 ,  B01J2531/37 ,  B01J2531/38 ,  C07F5/00 ,  C07F15/00 ,  C08F10/00 ,  C08F36/06 ,  C08F297/04 ,  C08F297/046 ,  C08F297/06 ,  C08L53/02 ,  C08F4/545

    Abstract: Metal complexes, catalyst compositions containing the metal complexes, and processes for making the metal complexes and the catalyst compositions are described for the manufacture of polymers from ethylenically unsaturated addition polymerizable monomers. The metal complexes have chemical structures corresponding to one of the following formulae: wherein MI and MII are metals; T is nitrogen or phosphorus; P is a carbon, nitrogen or phosphorus atom; groups R1, R2 and R3 may be linked to each other; Y is a divalent bridging group; X, X1, and X2 are anionic ligand groups with certain exceptions; D is a neutral Lewis base ligand; and s, o, k, i, ii, p, m, a, b, c, d, e, t, and y are numbers as further described in the claims.

    Abstract translation: 描述了金属络合物，含有金属络合物的催化剂组合物，以及用于制备金属络合物和催化剂组合物的方法，用于由烯键式不饱和加成聚合单体制备聚合物。 金属络合物具有对应于下式之一的化学结构：其中MI和MII是金属; T是氮或磷; P是碳，氮或磷原子; 基团R 1，R 2和R 3可以彼此连接; Y是二价桥基; X，X1和X2是阴离子配体基团，有一些例外; D是中性路易斯碱配体; 并且s，o，k，i，ii，p，m，a，b，c，d，e，t和y是权利要求中进一步描述的数字。

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