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    Process for disproportionating rosin, poly-unsaturated fatty acids and mixtures thereof
    71.
    发明授权
    Process for disproportionating rosin, poly-unsaturated fatty acids and mixtures thereof 失效
    歧化松香，多不饱和脂肪酸及其混合物的方法

    公开(公告)号：US4271066A

    公开(公告)日：1981-06-02

    申请号：US91490

    申请日：1979-11-05

    Applicant: Kohtaro Matsuo ,  Satoshi Kawamura ,  Tatsumi Toshine

    Inventor： Kohtaro Matsuo ,  Satoshi Kawamura ,  Tatsumi Toshine

    IPC: B01F17/00 ,  C08F2/26 ,  C09F1/04 ,  C09F7/08 ,  B01J27/02 ,  B01J27/08

    CPC classification number: C09F7/08 ,  B01F17/0028 ,  C08F2/26 ,  C09F1/04

    Abstract: This invention provides a process for disproportionating rosin, poly-unsaturated fatty acid or mixture thereof, characterized in that the disproportionation reaction is conducted in the presence of a catalyst comprising (A) at least one iodide selected from the group consisting of sodium iodide and potassium iodide and (B) at least one iron compound selected from the group consisting of iron, iron oxides, iron hydroxides and iron sulfides. The disproportionated product of this invention affords an emulsifier suitable for emulsion polymerization when neutralized with an alkali.

    Abstract translation: 本发明提供了一种歧化松香，多不饱和脂肪酸或其混合物的方法，其特征在于歧化反应在催化剂存在下进行，所述催化剂包含（A）至少一种选自碘化钠和钾的碘化物 碘化物和（B）选自铁，氧化铁，氢氧化铁和硫化铁中的至少一种铁化合物。 当用碱中和时，本发明的歧化产物提供适用于乳液聚合的乳化剂。

    Hydrocarbon conversion with an attenuated superactive multimetallic catalytic composite
    72.
    发明授权
    Hydrocarbon conversion with an attenuated superactive multimetallic catalytic composite 失效
    用减弱的超多活性多金属催化复合材料进行烃转化

    公开(公告)号：US4256608A

    公开(公告)日：1981-03-17

    申请号：US80639

    申请日：1979-10-01

    Applicant: George J. Antos

    Inventor： George J. Antos

    IPC: B01J23/656 ,  C10G35/09 ,  B01J27/08 ,  B01J23/89 ,  B01J27/10

    CPC classification number: B01J23/6567 ,  C10G35/09

    Abstract: Hydrocarbons are converted by contacting them at hydrocarbon conversion conditions with a novel attenuated superactive multimetallic catalytic composite comprising a combination of a catalytically effective amount of a pyrolyzed rhenium carbonyl component with a porous carrier material containing a uniform dispersion of a catalytically effective amount of a platinum group component, which is maintained in the elemental metallic state during the incorporation and pyrolysis of the rhenium carbonyl component, and of an iron component. In a highly preferred embodiment, this novel catalytic composite also contains a catalytically effective amount of a halogen component. The platinum group component, pyrolyzed rhenium carbonyl component, iron component and optional halogen component are preferably present in the multimetallic catalytic composite in amounts, calculated on an elemental basis, corresponding to about 0.01 to about 2 wt. % platinum group metal, about 0.01 to about 5 wt. % rhenium, about 0.005 to about 5 wt. % iron and about 0.1 to about 3.5 wt. % halogen. A key feature associated with the preparation of the subject catalytic composite is reaction of a rhenium carbonyl complex with a porous carrier material containing a uniform dispersion of an iron component and of a platinum group component maintained in the elemental state, whereby the interaction of the rhenium moiety with the platinum group moiety is maximized due to the platinophilic (i.e. platinum-seeking) propensities of the carbon monoxide ligands associated with the rhenium reagent. A specific example of the type of hydrocarbon conversion process disclosed herein is a process for the catalytic reforming of a low octane gasoline fraction wherein the gasoline fraction and a hydrogen stream are contacted with the attenuated superactive multimetallic catalytic composite at reforming conditions.

    Abstract translation: 通过在碳氢化合物转化条件下使它们与新型减弱的超活性多金属催化复合材料接触来转化碳氢化合物，该催化复合材料包含催化有效量的热解的铼羰基组分与含有催化有效量的铂的均匀分散体的多孔载体材料的组合 组分，其在羰基铼组分和铁组分的引入和热解期间保持在元素金属状态。 在一个非常优选的实施方案中，该新型催化复合材料还含有催化有效量的卤素组分。 铂族组分，热解的铼羰基组分，铁组分和任选的卤素组分优选以基于元素计算的量存在于多金属催化复合物中，相当于约0.01至约2重量％ ％铂族金属，约0.01至约5wt。 ％铼，约0.005至约5wt。 ％铁和约0.1至约3.5wt。 ％卤素。 与制备本发明的催化复合材料相关的一个关键特征是羰基钌络合物与保持在元素状态的铁组分和铂族组分的均匀分散体的多孔载体材料的反应，由此铼的相互作用 与铂族部分的部分由于与铼试剂相关的一氧化碳配体的铂嗜性（即铂寻求）倾向而最大化。 本文公开的烃转化方法的具体实例是低辛烷值汽油馏分的催化重整方法，其中汽油馏分和氢气流在重整条件下与减弱的超活性多金属催化复合材料接触。

    Attenuated superactive multimetallic catalytic composite
    76.
    发明授权
    Attenuated superactive multimetallic catalytic composite 失效
    衰减超活性多金属催化复合材料

    公开(公告)号：US4229319A

    公开(公告)日：1980-10-21

    申请号：US48957

    申请日：1979-06-15

    Applicant: George J. Antos

    Inventor： George J. Antos

    IPC: B01J23/68 ,  B01J27/08 ,  B01J23/66 ,  B01J27/10

    CPC classification number: B01J23/688

    Abstract: An attenuated superactive multimetallic catalytic composite especially useful for converting hydrocarbons comprises a combination of a catalytically effective amount of a pyrolyzed rhenium carbonyl component with a porous carrier material containing a uniform dispersion of a catalytically effective amount of a platinum group component, which is maintained in the elemental metallic state, and of a silver component. In a highly preferred embodiment, this novel catalytic composite also contains a catalytically effective amount of a halogen component. The platinum group component, pyrolyzed rhenium carbonyl component, silver component and optional halogen component are preferably present in the multimetallic catalytic composite in amounts, calculated on an elemental basis, corresponding to about 0.01 to about 2 wt. % platinum group metal, about 0.01 to about 5 wt. % rhenium, about 0.01 to about 5 wt. % silver and about 0.1 to about 3.5 wt. % halogen. A key feature associated with the preparation of the subject catalytic composite is reaction of a rhenium carbonyl complex with a porous carrier material containing a uniform dispersion of a silver component and of a platinum group component maintained in the elemental state, whereby the interaction of the rhenium moiety with the platinum group moiety is maximized due to the platinophilic (i.e. platinum-seeking) propensities of the carbon monoxide ligands associated with the rhenium reagent.

    Abstract translation: 特别可用于转化烃的减毒超活性多金属催化复合物包括催化有效量的热解的铼羰基组分与含有催化有效量的铂族组分的均匀分散体的多孔载体材料的组合，其保持在 元素金属状态和银组分。 在一个非常优选的实施方案中，该新型催化复合材料还含有催化有效量的卤素组分。 铂族组分，热解的铼羰基组分，银组分和任选的卤素组分优选以基于元素计算的量存在于多金属催化复合物中，相当于约0.01至约2重量％ ％铂族金属，约0.01至约5wt。 ％铼，约0.01至约5wt。 ％银和约0.1至约3.5重量％ ％卤素。 与本发明催化复合材料的制备相关的主要特征是羰基铑合金与含有均匀分散的银组分和维持在元素状态的铂族组分的多孔载体材料的反应，由此铼的相互作用 与铂族部分的部分由于与铼试剂相关的一氧化碳配体的铂嗜性（即铂寻求）倾向而最大化。

    Attenuated superactive multimetallic catalytic composite
    79.
    发明授权
    Attenuated superactive multimetallic catalytic composite 失效
    衰减超活性多金属催化复合材料

    公开(公告)号：US4220558A

    公开(公告)日：1980-09-02

    申请号：US29507

    申请日：1979-04-12

    Applicant: George J. Antos

    Inventor： George J. Antos

    IPC: B01J23/62 ,  B01J23/656 ,  B01J27/08 ,  B01J23/64 ,  B01J27/10

    CPC classification number: B01J23/62 ,  B01J23/6567

    Abstract: A novel attenuated superactive multimetallic catalytic composite, especially useful for the conversion of hydrocarbons, comprises a combination of a catalytically effective amount of a pyrolyzed rhenium carbonyl component with a porous carrier material containing a uniform dispersion of catalytically effective amounts of a platinum group component, which is maintained in the elemental metallic state, and of an indium component. In a highly preferred embodiment, this novel catalytic composite also contains a catalytically effective amount of a halogen component. The platinum group component, pyrolyzed rhenium carbonyl component, indium component and optional halogen component are preferably present in the multimetallic catalytic composite in amounts, calculated on an elemental basis, corresponding to about 0.01 to about 2 wt. % platinum group metal, about 0.01 to about 5 wt. % rhenium, about 0.01 to about 5% indium and about 0.1 to about 3.5 wt. % halogen. A key feature associated with the preparation of the subject catalytic composite is reaction of a rhenium carbonyl complex with a porous carrier material containing a uniform dispersion of an indium component and of a platinum group metal maintained in the elemental state, whereby the interaction of the rhenium moiety with the platinum group moiety is maximized due to the platinophilic (i.e. platinum-seeking) propensities of the carbon monoxide ligand used in the rhenium reagent.

    Abstract translation: 特别可用于烃转化的新颖的减毒超活性多金属催化复合材料包括催化有效量的热解铼羰基组分与含有催化有效量的铂族组分的均匀分散体的多孔载体材料的组合，其中 保持在元素金属状态和铟组分。 在一个非常优选的实施方案中，该新型催化复合材料还含有催化有效量的卤素组分。 铂族组分，热解的铼羰基组分，铟组分和任选的卤素组分优选以基于元素计算的量存在于多金属催化复合物中，相当于约0.01至约2重量％ ％铂族金属，约0.01至约5wt。 ％铼，约0.01至约5％的铟和约0.1至约3.5wt。 ％卤素。 与本发明的催化复合材料的制备相关的关键特征是羰基钌络合物与保持在元素状态的铟组分和铂族金属的均匀分散体的多孔载体材料的反应，由此铼的相互作用 由于在铼试剂中使用的一氧化碳配体的铂嗜性（即铂寻求）倾向，铂基团部分被最大化。

    Attenuated superactive multimetallic catalytic composite
    80.
    发明授权
    Attenuated superactive multimetallic catalytic composite 失效
    衰减超活性多金属催化复合材料

    公开(公告)号：US4212769A

    公开(公告)日：1980-07-15

    申请号：US13490

    申请日：1979-02-21

    Applicant: George J. Antos

    Inventor： George J. Antos

    IPC: B01J23/648 ,  B01J23/656 ,  C10G35/09 ,  B01J27/08 ,  B01J27/10

    CPC classification number: B01J23/6567 ,  C10G35/09 ,  B01J23/6486 ,  B01J35/0093

    Abstract: A novel attenuated superactive multimetallic catalytic composite especially useful for converting hydrocarbons comprises a combination of a catalytically effective amount of a pyrolyzed rhenium carbonyl component with a porous carrier material containing a uniform dispersion of catalytically effective amounts of a platinum group component, which is maintained in the elemental metallic state, and of a tantalum component. In a highly preferred embodiment, this novel catalytic composite also contains a catalytically effective amount of a halogen component. The platinum group component, pyrolyzed rhenium carbonyl component, tantalum component and optional halogen component are preferably present in the multimetallic catalytic composite in amounts, calculated on an elemental basis, corresponding to about 0.01 to about 2 wt. % platinum group metal, about 0.01 to about 5 wt. % rhenium, about 0.01 to about 5 wt. % tantalum and about 0.1 to about 3.5 wt. % halogen. A key feature associated with the preparation of the subject catalytic composite is reaction of a rhenium carbonyl complex with a porous carrier material containing a uniform dispersion of a tantalum component and of a platinum group metal maintained in the elemental state, whereby the interaction of the rhenium moiety with the platinum group moiety is maximized due to the platinophilic (i.e. platinum-seeking) propensities of the carbon monoxide ligand used in the rhenium reagent.

    Abstract translation: 特别适用于转化烃类的新型减毒超活性多金属催化复合物包括催化有效量的热解铼羰基组分与含有催化有效量的铂族组分的均匀分散体的多孔载体材料的组合，其保持在 元素金属状态和钽组分。 在一个非常优选的实施方案中，该新型催化复合材料还含有催化有效量的卤素组分。 铂族组分，热解的铼羰基组分，钽组分和任选的卤素组分优选以基于元素计算的量存在于多金属催化复合物中，相当于约0.01至约2重量％ ％铂族金属，约0.01至约5wt。 ％铼，约0.01至约5wt。 ％钽和约0.1至约3.5重量％ ％卤素。 与本发明催化复合材料的制备相关的关键特征是羰基铑合金与含有均匀分散的钽组分和维持在元素状态的铂族金属的多孔载体材料的反应，由此铼的相互作用 由于在铼试剂中使用的一氧化碳配体的铂嗜性（即铂寻求）倾向，铂基团部分被最大化。

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