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    BIOLOGICALLY DEGRADABLE POLYMERS, PROCESSES FOR MANUFACTURING THE SAME AND THE USE THEREOF FOR PRODUCING BIODEGRADABLE MOULDED ARTICLES
    1.
    发明申请
    BIOLOGICALLY DEGRADABLE POLYMERS, PROCESSES FOR MANUFACTURING THE SAME AND THE USE THEREOF FOR PRODUCING BIODEGRADABLE MOULDED ARTICLES 审中-公开
    生物降解聚合物，方法的生产和使用，其用于制造生物可降解成型

    公开(公告)号：WO9621689A2

    公开(公告)日：1996-07-18

    申请号：PCT/EP9502493

    申请日：1995-06-27

    Applicant: BASF AG ,  WARZELHAN VOLKER ,  SCHORNICK GUNNAR ,  BAUMANN EDWIN ,  SEELIGER URSULA ,  YAMAMOTO MOTONORI ,  RAMLOW GERHARD

    Inventor： WARZELHAN VOLKER ,  SCHORNICK GUNNAR ,  BAUMANN EDWIN ,  SEELIGER URSULA ,  YAMAMOTO MOTONORI ,  RAMLOW GERHARD

    IPC: C08G18/60 ,  C08G69/44 ,  C08G73/04 ,  C08J9/04 ,  C08L1/02 ,  C08L77/12 ,  C08L101/16 ,  C09D175/12 ,  C09J177/12 ,  D21H19/30

    CPC classification number: C08G69/44 ,  C08G18/606 ,  Y02W30/43

    Abstract: The invention concerns biologically degradable polyester amides P1 obtainable through reaction of a mixture consisting essentially of the following: (a1) a mixture consisting essentially of: 35-95 mol % adipic acid or ester-forming derivatives thereof or mixtures thereof, 5-65 mol % terephthalic acid or ester-forming derivatives thereof or mixtures thereof, and 0-5 mol % a compound containing sulphonate groups (the sum of the individual molar percentages is 100); (a2) a mixture consisting essentially of: (a21) 99.5-0.5 mol % a dihydroxy compound chosen from the group comprising C2-C6 alkane diols and C5-C10 cycloalkane diols, (a22) 0.5-99.5 mol % an amino C2-C12 alkanol or an amino-C5-C10 cycloalkanol, (a23) 0-50 mol % a diamino C1-C8 alkane; and (a24) 0-50 mol % a 2,2`-bisoxazoline of general formula (I), in which R is a single bond, a (CH2)q-alkylene group in which q = 2, 3 or 4, or a phenylene group (the sum of the individual molar percentages is 100 and the molar ratio of a1 to a2 is in the range 0.4:1 - 1.5:1). The polyester amides P1 will have a molecular weight (Mn) in the range 4000-40,000 g/mol, a viscosity number in the range 30-350 g/ml (measured in o-dichlorobenzene/phenol (weight ratio 50/50) at a concentration of 0.5 wt.% polyester amide P1 at a temperature of 25 DEG C) and a melting point in the range 50-220 DEG C; and a quantity of a compound D equivalent to 0-5 mol % of the molar quantity of components (a1) must also be used for the production of the polyester amides P1, said compound D having at least three groups capable of ester formation. The invention also concerns other biologically degradable polymers and thermoplastic moulding materials, processes for manufacturing the same, the use thereof for producing biologically degradable moulded articles and adhesives, and biologically degradable moulded articles, foams and blends with starch which can be obtained from the polymers or moulding materials according to the invention.

    Abstract translation: 可生物降解的聚酯酰胺通过基本上由混合物反应P1获得（a1）的基本上35由〜95摩尔％的己二酸或它们的酯形成性衍生物或者它们的混合物，5〜65摩尔％的对苯二甲酸或其酯形成性衍生物的混合物 或其混合物，和0〜5摩尔％磺酸酯化合物的，单独的摩尔百分比的总和为100摩尔％，和（a2）从99.5基本上由（A21）〜0.5摩尔的混合物 - （A22）0.5选自C2-C6烷二醇和C5-C10-环烷二醇的组中选择的二羟基化合物，的％至99.5摩尔％的氨基C2-C12链烷醇或氨基-C5的 C10-环烷醇，以及（A23）0〜50摩尔％的二氨基C1-C8烷烃，（A24）0〜50摩尔％通式（I）的2,2'-二恶唑啉，其中R <1 >一个单键，（CH 2）●亚烷基其中q = 2，3或4，或亚苯基，其中装置 各个摩尔百分比的总和为100摩尔％，并且其中的（a1）至（A2）的范围为0.4的摩尔比：1至1.5：1种选择，条件是该聚酯酰胺P1的分子量 （Mn）的范围为4000至40,000克/摩尔，在30至350范围内的粘度数克/毫升（在以0.5重量％的浓度的邻二氯苯/苯酚（50/50重量比）进行测定。 - ％聚酯酰胺P1在25℃的温度），并在50至220℃的范围内的熔点，并与一个从0〜5摩尔％基于组分的摩尔量进一步的条件（A1 ），与能够对聚酯酰胺的制备酯的形成至少三个基团的化合物D P1中使用的以及其它可生物降解的聚合物和热塑性模塑组合物，涉及它们的制备方法，它们用于制备可生物降解的模制品和粘合剂，生物可降解的成型品使用， 泡沫和从本发明的聚合物或模塑组合物获得的淀粉混合物。

    BIOLOGICALLY DEGRADABLE POLYMERS, PROCESSES FOR MANUFACTURING THE SAME AND THE USE THEREOF FOR PRODUCING BIODEGRADABLE MOULDED ARTICLES
    5.
    发明申请
    BIOLOGICALLY DEGRADABLE POLYMERS, PROCESSES FOR MANUFACTURING THE SAME AND THE USE THEREOF FOR PRODUCING BIODEGRADABLE MOULDED ARTICLES 审中-公开
    生物降解聚合物，方法的生产和使用，其用于制造生物可降解成型

    公开(公告)号：WO1996021691A1

    公开(公告)日：1996-07-18

    申请号：PCT/EP1996000064

    申请日：1996-01-09

    Applicant: BASF AKTIENGESELLSCHAFT ,  WARZELHAN, Volker ,  SCHORNICK, Gunnar ,  KRONER, Matthias ,  SEELIGER, Ursula ,  YAMAMOTO, Motonori ,  RAMLOW, Gerhard

    Inventor： BASF AKTIENGESELLSCHAFT

    IPC: C08G69/44

    CPC classification number: C08K5/09 ,  B65D65/466 ,  C08G69/44 ,  C08G69/48 ,  C08L3/02 ,  Y02W30/43 ,  Y02W90/11 ,  Y02W90/13 ,  C08L77/12 ,  C08L2666/02

    Abstract: The invention concerns biologically degradable polyether ester amides Q1 with a molecular weight (Mn) in the range 6000-8000 g/mol, a viscosity number in the range 30-450 g/ml (measured in o-dichlorobenzene/phenol (weight ratio 50/50) at a concentration of 0.5 wt.% polyether ester amide Q1 at a temperature of 25 DEG C) and a melting point in the range 50-200 DEG C, obtainable through reaction of a mixture consisting essentially of the following: (a1) 95-99.9 wt.% polyether ester amide P1 with a molecular weight (Mn) in the range 6000-80,000 g/mol, a viscosity number in the range 30-450 g/ml (measured in o-dichlorobenzene/phenol (weight ratio 50/50) at a concentration of 0.5 wt.% polyether ester amide P1 at a temperature of 25 DEG C) and a melting point in the range 50-200 DEG C, obtainable through reaction of a mixture consisting essentially of: (b1) a mixture consisting essentially of: 20-95 mol % adipic acid or ester-forming derivatives thereof or mixtures thereof; 5-80 mol % terephthalic acid or ester-forming derivatives thereof or mixtures thereof; and 0-5 mol % a compound containing sulphonate groups (the sum of the molar percentages is 100); (b2) a mixture of dihydroxy compounds consisting essentially of: (b21) 15-99.3 mol % a dihydroxy compound chosen from the group comprising C2-C6 alkane diols and C5-C10 cycloalkane diols; (b22) 0.2-85 mol % a dihydroxy compound containing ether functions, of formula I HO-[(CH2)n-O]m-H, wherein n is 2, 3 or 4 and m is an integer between 2 and 250, or mixtures thereof; (b23) 0.5-80 mol % an amino-C2-C12 alkanol or an amino C5-C10 cycloalkanol; and (b24) 0-50 mol % a diamino C1-C8 alkane; (b25) 0-50 mol % a 2,2`-bisoxazoline of general formula II, in which R is a single bond, a (CH2)q-alkylene group in which q = 2, 3 or 4, or a phenylene group (the sum of the individual molar percentages is 100 and the selected molar ratio of b1 to b2 is in the range 0.4:1 - 1.5:1; (a2) 0.1-5 wt.% a divinyl ether C1; and (a3) 0-5 mol % (in relation to components b1 from the production of P1) compound D. The invention also concerns other biologically degradable polymers and thermoplastic moulding materials, processes for manufacturing the same and the use thereof for producing biologically degradable moulded articles and adhesives, and biologically degradable moulded articles, foams and blends with starch obtainable from the polymers or moulding materials according to the invention.

    Abstract translation: 生物可降解的聚醚酯酰胺Q1与在范围内的分子量（Mn）为6000〜80000克/摩尔，在30至450范围内的粘度数克/毫升（邻二氯苯/苯酚测量（50/50重量比）在 在25℃的温度下0.5重量％聚醚酯酰胺Q1的浓度）和在50的范围内的熔点至200℃，由得到的基本上由（A1）95〜99.9的混合物反应 重量％聚醚酯酰胺P1与在范围内的分子量（Mn）为5000〜80000克/摩尔，在30至450范围内的粘度数克/毫升（邻二氯苯/苯酚测量（50/50重量比） 在在25℃的温度下0.5重量％聚醚酯酰胺P1的浓度）和在50的范围内的熔点至200℃，由得到的基本上由（B1）的混合物组成的混合物反应 基本上由己二酸或EST的20〜95摩尔％ 其埃尔比勒Dende衍生物或它们的混合物，对苯二甲酸或其酯形成性衍生物或者它们的混合物，以及0〜5摩尔％磺酸酯化合物的5〜80摩尔％时，各自的摩尔百分数的总和为100摩尔％，和（b2）一个 基本上由（B21）15〜99.3摩尔％的选自C2-C6烷二醇和C5-C10-环烷二醇的组中选择的二羟基化合物的，（B22）在0.2至85的二羟基化合物的混合物 摩尔％的二羟基化合物的含有醚官能团和式（I）HO的 - 是[（CH2）NO] mH的，其中n是2，3或4，且m为2至250的整数，或它们的混合物，（B23） 从0.5至80摩尔％的氨基C2-C12链烷醇或氨基C5-C10-环烷醇，以及二氨基-C1-C8烷烃的（B24）0至50摩尔％，（B25） 从0到50摩尔％的通式的2,2'-双恶唑啉的（II）式中，R <1>是一个单键，（CH 2）●亚烷基其中q = 2，3或4，或者表示亚苯基，其中，所述各自的摩尔百分数的总和为100摩尔％，其中，在范围从0.4的（B1）的摩尔比（B2）：1至1.5：1的 0.1选择，（A2）5重量的％从制备化合物D P1的，二乙烯基醚C1和（a3）为0〜5摩尔％，基于组分（b1）以及其它可生物降解的聚合物和 热塑性模塑组合物，其制备方法，它们用于制备可生物降解的模制品和粘合剂，可生物降解的模制品，泡沫以及与淀粉共混物从本发明的聚合物或模塑组合物获得的用途。

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