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    HYBRID ANODES FOR REDOX FLOW BATTERIES
    2.
    发明申请
    HYBRID ANODES FOR REDOX FLOW BATTERIES 审中-公开
    用于REDOX流量电池的混合阳极

    公开(公告)号：WO2014197012A1

    公开(公告)日：2014-12-11

    申请号：PCT/US2014/015696

    申请日：2014-02-11

    Applicant: BATTELLE MEMORIAL INSTITUTE

    Inventor： WANG, Wei ,  XIAO, Jie ,  WEI, Xiaoliang ,  LIU, Jun ,  SPRENKLE, Vincent L.

    IPC: H01M8/18 ,  H01M12/08

    CPC classification number: H01M12/08 ,  H01M4/382 ,  H01M4/90 ,  H01M4/96 ,  H01M8/188 ,  Y02E60/128

    Abstract: RFBs having solid hybrid electrodes can address at least the problems of active material consumption, electrode passivation, and metal electrode dendrite growth that can be characteristic of traditional batteries, especially those operating at high current densities. The RFBs each have a first half cell containing a first redox couple dissolved in a solution or contained in a suspension. The solution or suspension can flow from a reservoir to the first half cell. A second half cell contains the solid hybrid electrode, which has a first electrode connected to a second electrode, thereby resulting in an equipotential between the first and second electrodes. The first and second half cells are separated by a separator or membrane.

    Abstract translation: 具有固体混合电极的RFB至少可以解决活性材料消耗，电极钝化和金属电极枝晶生长的问题，其可以是传统电池的特征，特别是以高电流密度工作的电池。 RFB各自具有包含溶解在溶液中或包含在悬浮液中的第一氧化还原对的第一半电池。 溶液或悬浮液可以从储存器流到前半单元。 第二半单元包含固体混合电极，其具有连接到第二电极的第一电极，从而在第一和第二电极之间产生等电位。 第一和第二个细胞被分离器或膜隔开。

    ELECTRODES FOR MAGNESIUM ENERGY STORAGE DEVICES
    3.
    发明申请
    ELECTRODES FOR MAGNESIUM ENERGY STORAGE DEVICES 审中-公开
    用于镁能量储存装置的电极

    公开(公告)号：WO2014168691A1

    公开(公告)日：2014-10-16

    申请号：PCT/US2014/018190

    申请日：2014-02-25

    Applicant: BATTELLE MEMORIAL INSTITUTE

    Inventor： SHAO, Yuyan ,  LIU, Jun

    IPC: H01M10/054 ,  H01M4/46 ,  H01M2/16

    CPC classification number: H01M4/466 ,  H01M2/1613 ,  H01M4/134 ,  H01M10/054 ,  H01M10/0568

    Abstract: Nanostructured bismuth materials can be utilized as an insertion material in electrodes for magnesium energy storage devices to take advantage of short diffusion lengths for Mg 2+ . The result can be a significantly increased charge/discharge rates and/or improved cycling stabilities. In one example, an energy storage device has magnesium as an electroactive species, an electrolyte salt containing magnesium, and an anode having bismuth nanostructures. The bismuth nanostructures have at least one dimension that is less than or equal to 25 nm. At least a portion of the magnesium is reversibly inserted into, and extracted from, the anode during discharging and charging states, respectively.

    Abstract translation: 纳米结构的铋材料可以用作镁能量储存装置的电极中的插入材料，以利用Mg2 +的短扩散长度。 结果可以是显着增加的充电/放电速率和/或改善的循环稳定性。 在一个实例中，能量存储装置具有镁作为电活性物质，含镁的电解质盐和具有铋纳米结构的阳极。 铋纳米结构具有至少一个小于或等于25nm的尺寸。 分别在放电和充电状态期间，镁的至少一部分可逆地插入阳极中并从其中提取出来。

    MAGNESIUM-BASED ENERGY STORAGE SYSTEMS AND METHODS HAVING IMPROVED ELECTROLYTES
    4.
    发明申请
    MAGNESIUM-BASED ENERGY STORAGE SYSTEMS AND METHODS HAVING IMPROVED ELECTROLYTES 审中-公开
    基于镁的能源储存系统和具有改进电解质的方法

    公开(公告)号：WO2014168671A1

    公开(公告)日：2014-10-16

    申请号：PCT/US2014/013371

    申请日：2014-01-28

    Applicant: BATTELLE MEMORIAL INSTITUTE

    Inventor： LIU, Tianbiao ,  LI, Guosheng ,  LIU, Jun ,  SHAO, Yuyan

    IPC: H01M10/056 ,  H01M10/054

    CPC classification number: H01M10/0568 ,  H01M10/054

    Abstract: Electrolytes for Mg-based energy storage devices can be formed from non-nucleophilic Mg 2+ sources to provide outstanding electrochemical performance and improved electrophilic susceptibility compared to electrolytes employing nucleophilic sources. The instant electrolytes are characterized by high oxidation stability (up to 3.4 V vs Mg), improved electrophile compatibility and electrochemical reversibility (up to 100% coulombic efficiency). Synthesis of the Mg 2+ electrolytes utilizes inexpensive and safe magnesium dihalides as non-nucleophilic Mg 2+ sources in combination with Lewis acids, MR a X 3-a (for 3≥ a≥ 1). Furthermore, addition of free-halide-anion donors can improve the coulombic efficiency of Mg electrolytes from nucleophilic or non-nucleophilic Mg 2+ sources.

    Abstract translation: 用于Mg基能量储存装置的电解质可以由非亲核Mg 2+源形成，以提供与使用亲核源的电解质相比优异的电化学性能和改善的亲电子敏感性。 瞬时电解质的特征在于高氧化稳定性（高达3.4V vs镁），改善的亲电子相容性和电化学可逆性（高达100％的库仑效率）。 Mg2 +电解质的合成使用廉价和安全的二卤化镁作为非亲核Mg2 +源与路易斯酸MRaX3-a（3≥a≥1）的组合。 此外，添加游离卤化物 - 阴离子供体可以提高Mg电解质从亲核或非亲核Mg2 +来源的库仑效率。

    SODIUM-BASED ENERGY STORAGE DEVICES BASED ON SURFACE-DRIVEN REACTIONS
    5.
    发明申请
    SODIUM-BASED ENERGY STORAGE DEVICES BASED ON SURFACE-DRIVEN REACTIONS 审中-公开
    基于表面驱动反应的基于钠的能量储存装置

    公开(公告)号：WO2014109791A1

    公开(公告)日：2014-07-17

    申请号：PCT/US2013/050689

    申请日：2013-07-16

    Applicant: BATTELLE MEMORIAL INSTITUTE

    Inventor： SHAO, Yuyan ,  LIU, Jun ,  XIAO, Jie ,  WANG, Wei

    IPC: H01M10/054 ,  H01M10/39

    CPC classification number: H01M4/381 ,  H01G11/06 ,  H01G11/30 ,  H01G11/32 ,  H01G11/62 ,  H01M4/13 ,  H01M4/663 ,  H01M10/054 ,  H01M10/44 ,  Y02E60/13 ,  Y02T10/7022

    Abstract: The performance of sodium-based energy storage devices can be improved according to methods and devices based on surface-driven reactions between sodium ions and functional groups attached to surfaces of the cathode. The cathode substrate, which includes a conductive material, can provide high electron conductivity while the surface functional groups can provide reaction sites to store sodium ions. During discharge cycles, sodium ions will bind to the surface functional groups. During charge cycles, the sodium ions will be released from the surface functional groups. The surface-driven reactions are preferred compared to intercalation reactions.

    Abstract translation: 可以根据钠离子和附着于阴极表面的官能团之间的表面驱动反应的方法和装置，改​​善钠基储能装置的性能。 包括导电材料的阴极基底可以提供高电子导电性，而表面官能团可以提供反应位点来储存钠离子。 在放电循环期间，钠离子将与表面官能团结合。 在充电循环期间，钠离子将从表面官能团释放出来。 与嵌入反应相比，表面驱动的反应是优选的。

    ELECTROSYNTHESIS OF NANOFIBERS AND NANO-COMPOSITE FILMS
    10.
    发明申请
    ELECTROSYNTHESIS OF NANOFIBERS AND NANO-COMPOSITE FILMS 审中-公开
    纳米纤维和纳米复合薄膜的电合成

    公开(公告)号：WO2004048644A2

    公开(公告)日：2004-06-10

    申请号：PCT/US2003/016273

    申请日：2003-05-21

    Applicant: BATTELLE MEMORIAL INSTITUTE

    Inventor： LIN, Yuehe ,  LIANG, Liang ,  LIU, Jun

    IPC: C25D

    CPC classification number: B82Y30/00 ,  C09D5/4476 ,  C25D9/00

    Abstract: A method of producing an array of oriented nanofibers that involves forming a solution that includes at least one electroactive species. An electrode substrate is brought into contact with the solution. A current density is applied to the electrode substrate that includes at least a first step of applying a first substantially constant current density for a first time period and a second step of applying a second substantially constant current density for a second time period. The first and second time periods are of sufficient duration to electrically deposit on the electrode substrate an array of oriented nanofibers produced from the electroactive species. Also disclosed are films that include arrays or networks of oriented nanofibers and a method for amperometrically detecting or measuring at least one analyte in a sample.

    Abstract translation: 生产取向纳米纤维阵列的方法，其涉及形成包含至少一种电活性物质的溶液。 使电极基板与溶液接触。 向电极基板施加电流密度，该电流密度至少包括在第一时间段施加第一基本上恒定的电流密度的第一步骤和在第二时间段施加第二基本上恒定的电流密度的第二步骤。 第一和第二时间段具有足够的持续时间以在电极基板上电沉积由电活性物质产生的取向纳米纤维的阵列。 还公开了包含取向纳米纤维的阵列或网络的膜以及用于安培检测或测量样品中的至少一种分析物的方法。

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