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    Aromatic Polymer and Producing Method Thereof
    22.
    发明申请
    Aromatic Polymer and Producing Method Thereof 失效
    芳香族聚合物及其制备方法

    公开(公告)号：US20090105445A1

    公开(公告)日：2009-04-23

    申请号：US11920168

    申请日：2006-05-08

    Applicant: Shigeki Habaue ,  Soichiro Murakami ,  Hideyuki Higashimura

    Inventor： Shigeki Habaue ,  Soichiro Murakami ,  Hideyuki Higashimura

    IPC: C08G65/44 ,  C08G65/40 ,  C08G65/48

    CPC classification number: C08G61/10

    Abstract: An aromatic polymer, containing a repeating unit represented by Formula (I), and having properties (A1) and (B1):(A1) the number average degree of polymerization of an acetylated product obtained by acetylation of the hydroxyl groups of the polymer is 3 or more, and (B1) at a wavelength where an absolute value of molar ellipticity (degree·cm−2·dmol−1) per mole of the repeating unit of the acetylated product in a circular dichroism spectrum of the acetylated product reaches maximum in a wavelength range of from 200 to 350 nm, the absolute value is 50,000 or more: wherein R represents a hydrocarbon, hydrocarbon-oxy, hydrocarbon-mercapto or hydrocarbon-amino group that may be substituted; the two R′s may bind to each other to form a ring; and the repeating unit represented by Formula (I) has two binding sites and has no symmetrical plane perpendicular to the benzene ring.

    Abstract translation: 含有由式（I）表示的重复单元，具有（A1）和（B1）性质的芳族聚合物：（A1）通过聚合物的羟基乙酰化得到的乙酰化产物的数均聚合度为 3个以上，和（B1）在乙酰化产物的圆二色谱中每摩尔乙酰化产物的重复单元的绝对摩尔数椭圆率（度.cm-2.dmol-1）的波长达到最大 在200〜350nm的波长范围内，绝对值为50,000以上：其中R表示可被取代的烃，烃 - 氧，烃 - 巯基或烃 - 氨基; 两个R可以彼此结合形成环; 并且由式（I）表示的重复单元具有两个结合位点，并且没有与苯环垂直的对称平面。

    Novel Aryl Compound
    23.
    发明申请
    Novel Aryl Compound 审中-公开
    新型芳基化合物

    公开(公告)号：US20090099391A1

    公开(公告)日：2009-04-16

    申请号：US11921796

    申请日：2006-06-09

    Applicant: Kazuei Ohuchi ,  Hideyuki Higashimura ,  Daisuke Fukushima

    Inventor： Kazuei Ohuchi ,  Hideyuki Higashimura ,  Daisuke Fukushima

    IPC: C07C209/18

    CPC classification number: C07F5/025 ,  C07C211/56

    Abstract: A novel aryl compound represented by the formula (1) in which the characteristic groups represented by X1 and X2 are different from each other: wherein X1 and X2 are characteristic groups which are different from each other and each of which is selected from the group consisting of a chlorine, bromine or iodine atom, —OSO2Q1, —B(OQ2)2, —Si(OQ3)3, —Sn(Q4)3, Z1 (Z2)m, a metal acetylide group and a terminal acetylene group (where Q represents a hydrocarbon group; Q2 represents a hydrogen atom or a hydrocarbon group; two Q2's may be the same as or different from each other or may together form a ring; Q3 represents a hydrocarbon group and three Q3's may be the same as or different from one another; Q4 represents a hydrocarbon group and three Q4's may be the same as different from one another; Z1 represents a metal atom or a metal ion; Z2 represents a counter anion; and m is an integer of 0 or higher); Ar1 and Ar2 independently represent an arylene group and Ar3 represetns an aryl group, provided that any two of Ar1, Ar2 and Ar3 may be bound to each other via a substituent or directly; Y represents a trivalent atomic group having a nitrogen, carbon, boron or silicon atom to which a hydrogen atom or a hydrocarbon group may be added if required; J represents an arylene group; and n is an integer of 0 or higher; provided that, when each of J, Y and Ar3 is present in the molecule in plural number, they may be the same as or different from each other or one another.

    Abstract translation: 由式（1）表示的由X1和X2表示的特征基团彼此不同的式（1）表示的新型芳基化合物：其中X1和X2是彼此不同的特征基团，其各自选自 的氯，溴或碘原子，-OSO 2 Q 1，-B（OQ 2）2，-Si（OQ 3）3，-Sn（Q 4）3，Z 1（Z 2）m，金属乙炔基和末端乙炔基 Q表示烃基; Q2表示氢原子或烃基;两个Q2可以相同或不同，也可以一起形成环; Q3表示烃基，三个Q3可以相同或不同 Q4表示烃基，3个Q4可以相同，Z1表示金属原子或金属离子，Z2表示抗衡阴离子，m表示0以上的整数）表示的化合物。 Ar1和Ar2独立地表示亚芳基，Ar3表示芳基，只要Ar1，Ar2和Ar3中的任意两个可以通过取代基彼此结合或直接键合; Y表示如果需要，可以加入氢原子或烃基的具有氮原子，碳原子，硼原子或硅原子的三价原子团; J表示亚芳基; n为0以上的整数， 条件是，当分子中存在多个数量的J，Y和Ar 3中的每一个时，它们可以彼此相同或不同。

    MULTINUCLEAR COMPLEX AND CONDENSATION PRODUCT THEREOF
    24.
    发明申请
    MULTINUCLEAR COMPLEX AND CONDENSATION PRODUCT THEREOF 审中-公开
    多功能复合物和凝结产品

    公开(公告)号：US20090036687A1

    公开(公告)日：2009-02-05

    申请号：US12278415

    申请日：2007-02-08

    Applicant: Yoshiyuki Sugahara ,  Takeshi Ishiyama ,  Hideyuki Higashimura

    Inventor： Yoshiyuki Sugahara ,  Takeshi Ishiyama ,  Hideyuki Higashimura

    IPC: C07D403/14 ,  C07F7/10

    CPC classification number: C07F15/025 ,  B01J31/183 ,  B01J31/2243 ,  B01J2231/62 ,  B01J2531/0216 ,  B01J2531/0258 ,  B01J2531/16 ,  B01J2531/72 ,  B01J2531/842 ,  B01J2531/845 ,  B01J2531/847 ,  C07F7/1804

    Abstract: A multinuclear complex comprising a plurality of metal atoms and a ligand L coordinating to the metal atoms, and satisfying the following conditions (i), (ii), (iii) and (iv):(i) The ligand L has a monovalent group represented by the following general formula (1) and/or a divalent group represented by the following general formula (2), (ii) The ligand L has at least 5 coordination atoms bonding to the metal atom, (iii) At least one of the coordination atoms bonds to two of the metal atoms, or the minimum number of covalent bonds between any two selected coordination atoms is 1-5, and (iv) The ligand L is soluble in the solvent.

    Abstract translation: 包含多个金属原子的多核络合物和与金属原子配位的配位体L，并满足下列条件（i），（ii），（iii）和（iv）：（i）配体L具有一价基团 由下述通式（1）表示的化合物和/或由以下通式（2）表示的二价基团，（ii）配体L具有至少5个与金属原子键合的配位原子，（iii）至少一个 配位原子与两个金属原子键合，或任意两个选定的配位原子之间的最小共价键数为1-5，和（ⅳ）配体L可溶于溶剂中。

    Crystallizable poly (2,5-di-substituted-1,4-phenylene oxide) and a method of preparing the same
    25.
    发明授权
    Crystallizable poly (2,5-di-substituted-1,4-phenylene oxide) and a method of preparing the same 有权
    可结晶的聚（2,5-二取代-1,4-亚苯基氧化物）及其制备方法

    公开(公告)号：US06841650B2

    公开(公告)日：2005-01-11

    申请号：US10157862

    申请日：2002-05-31

    Applicant: Hideyuki Higashimura ,  Kiyoshi Fujisawa ,  Yoshihiko Moro-Oka ,  Shiro Kobayashi

    Inventor： Hideyuki Higashimura ,  Kiyoshi Fujisawa ,  Yoshihiko Moro-Oka ,  Shiro Kobayashi

    IPC: C08G65/44 ,  C08G59/50

    CPC classification number: C08G65/44

    Abstract: There is disclosed a crystallizable poly(2,5-di-substituted-1,4-phenylene oxide), which exhibits an exothermic peak for crystallization of not less than 5 J/g at 150° C. or over when cooled after melting, and/or an endothermic peak, at the time of melting of crystals thereof, of not less than 5 J/g at 150° C. or over when re-heated after cooling of the melt, and which comprises a recurring unit of the following formula (I), and a method of preparing the same by polymerization of a 2,5-di-substituted-phenol of the following formula (II) by use of a copper complex catalyst made of a tridentate ligand of which nitrogen atoms coordinate to a copper atom in coexistence with oxygen: wherein R1's independently represent a hydrocarbon group or a substituted hydrocarbon group, and they may be the same or different. The crystallizable poly(2,5-di-substituted-1,4-phenylene oxide) is able to provide a melt molding which has a reduced degree of coloration and good heat resistance.

    Abstract translation: 公开了一种可结晶的聚（2,5-二取代-1,4-亚苯基氧化物），其在熔化后冷却时在150℃或更高温度下表现出不低于5J / g的结晶放热峰， 和/或其结晶时的吸热峰在熔融物冷却后再加热时在150℃以上不低于5J / g，并且其包含以下的重复单元 式（I）的方法和通过使用由氮原子配位的三齿配体构成的铜络合物催化剂聚合下述式（II）的2,5-二取代苯酚而制备的方法 与氧共存的铜原子：其中R 1独立地表示烃基或取代的烃基，它们可以相同或不同。 可结晶的聚（2,5-二取代-1,4-亚苯基氧化物）能够提供具有降低的着色程度和良好的耐热性的熔融模塑。

    Oxidation polymer of a substituted phenol
    26.
    发明授权
    Oxidation polymer of a substituted phenol 失效
    取代苯酚的氧化聚合物

    公开(公告)号：US06576800B2

    公开(公告)日：2003-06-10

    申请号：US09905978

    申请日：2001-07-17

    Applicant: Hideyuki Higashimura ,  Shiro Kobayashi

    Inventor： Hideyuki Higashimura ,  Shiro Kobayashi

    IPC: C07C4100

    CPC classification number: C08G65/44

    Abstract: An oxidation polymer of a substituted phenol, obtained by oxidative polymerization of at least one compound selected from the group consisting of a compound of formula (Ia) and a compound of formula (Ib), in which the oxidation polymer has a number-average polymerization degree of 3 or more: wherein R1 to R4 each represent a hydrogen atom and the like; provided that at least one of R1 to R4 represents a substituted or unsubstituted, saturated hydrocarbon group having 10 or more carbon atoms, and R1 and/or R4 represent a hydrogen atom; wherein R11 represents a substituted or unsubstituted, saturated hydrocarbon group having 15 or more carbon atoms, and R12 is the same as R11, or when R12 is different from R11, R12 represents a substituted or unsubstituted hydrocarbon group and the like.

    Abstract translation: 通过氧化聚合至少一种选自式（Ia）化合物和式（Ib）化合物的化合物的化合物获得的取代苯酚的氧化聚合物，其中氧化聚合物具有数均聚合 3以上：其中，R1〜R4各自表示氢原子等; 条件是R 1至R 4中的至少一个表示具有10个或更多个碳原子的取代或未取代的饱和烃基，R 1和/或R 4表示氢原子;其中R 11表示取代或未取代的饱和烃基，其具有15或 更多的碳原子，R 12与R 11相同，或者当R 12与R 11不同时，R 12表示取代或未取代的烃基等。

    Polyphenylene ether resin composition
    27.
    发明授权
    Polyphenylene ether resin composition 失效
    聚苯醚树脂组合物

    公开(公告)号：US5484831A

    公开(公告)日：1996-01-16

    申请号：US383179

    申请日：1995-02-03

    Applicant: Hideyuki Higashimura ,  Yoshitaka Ohbe ,  Akihiko Okada ,  Kazutoshi Ohashi ,  Ryuhei Matsui ,  Shigeki Kriyama

    Inventor： Hideyuki Higashimura ,  Yoshitaka Ohbe ,  Akihiko Okada ,  Kazutoshi Ohashi ,  Ryuhei Matsui ,  Shigeki Kriyama

    IPC: C08G65/48 ,  C08K5/17

    CPC classification number: C08G65/485 ,  C08K5/17

    Abstract: A resin composition comprising a polyphenylene ether having, on the average, 0.01 to 10 terminal structures of the formula (1): ##STR1## wherein R.sub.1 to R.sub.5 are each hydrogen, halogen, a substituted or unsubstituted alkyl, alkenyl or alkynyl group, or a substituted or unsubstituted aryl group, R.sub.6 is a substituted or unsubstituted alkylene group, and R.sub.7 to R.sub.11 are each hydrogen, halogen, an alkyl group, an alkoxy group, a phenyl group, a phenoxy group, a nitro group or a cyano group per 100 phenylene ether units, and a primary aliphatic monoamine having an aromatic substituent, which composition has good thermal stability.

    Abstract translation: 一种树脂组合物，其包含平均具有式（1）的0.01至10个末端结构的聚苯醚：其中R 1至R 5各自为氢，卤素，取代或未取代的烷基，烯基或炔基 基团或取代或未取代的芳基，R6是取代或未取代的亚烷基，R7〜R11分别为氢，卤素，烷基，烷氧基，苯基，苯氧基，硝基或 氰基，每100个亚苯基醚单元和具有芳香族取代基的伯脂肪族单胺，该组合物具有良好的热稳定性。

    Composition comprising phosphorescent compound and light emitting device using the composition
    30.
    发明授权
    Composition comprising phosphorescent compound and light emitting device using the composition 有权
    包含磷光化合物和使用该组合物的发光器件的组合物

    公开(公告)号：US08697256B2

    公开(公告)日：2014-04-15

    申请号：US13056259

    申请日：2009-07-28

    Applicant: Nobuhiko Akino ,  Kenta Tanaka ,  Hideyuki Higashimura

    Inventor： Nobuhiko Akino ,  Kenta Tanaka ,  Hideyuki Higashimura

    IPC: C09K11/06 ,  C07D239/24 ,  H01L51/54

    CPC classification number: C07D239/26 ,  C08G2261/3221 ,  C08G2261/5242 ,  C08K5/3462 ,  C08L65/00 ,  C09K11/06 ,  C09K2211/1044 ,  H01L51/0067 ,  H01L51/0085 ,  H01L51/5016 ,  H05B33/14

    Abstract: A composition comprising a phosphorescent compound, and a compound having a structure containing three or more repeating units having a dipole moment dimension of 1.0 Debye or more connected in series, wherein, based on the total number of dimer structures composed of any two repeating units connected in series contained in the above-described structure, the proportion of the number of dimer structures in which the dimension D2 of the dipole moment of the dimer structure, the dimension D1a of the dipole moment of the first repeating unit constituting the dimer structure and the dimension D1b of the dipole moment of the second repeating unit constituting the dimer structure satisfy a relation represented by the following formula (A): D1a

    Abstract translation: 包含磷光化合物的组合物和具有包含三个或更多个偶极矩尺寸为1.0德拜或更多的重复单元的结构的化合物，其中基于由连接的任何两个重复单元组成的二聚体结构的总数 串联包含在上述结构中，二聚体结构的偶极矩的尺寸D2，构成二聚体结构的第一重复单元的偶极矩的尺寸D1a和二聚体结构的二聚体结构的数量的比例 构成二聚体结构的第二重复单元的偶极矩的尺寸D1b满足由下式（A）表示的关系：D1a

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