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61.发明授权Process for upgrading heavy oil using a reactor with a novel reactor separation system 有权使用具有新型反应器分离系统的反应器升级重油的方法公开(公告)号：US07901569B2
公开(公告)日：2011-03-08
申请号：US12212231
申请日：2008-09-17
Applicant: Darush Farshid , James Murphy , Bruce Reynolds
Inventor： Darush Farshid , James Murphy , Bruce Reynolds
IPC: C10G1/08
CPC classification number: C10G65/02 , C10G49/12 , C10G2300/1022 , C10G2300/1033 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/1088 , C10G2300/4081 , C10G2300/703
Abstract: Applicants have developed a new residuum full hydroconversion slurry reactor system that allows the catalyst, unconverted oil, hydrogen, and converted oil to circulate in a continuous mixture throughout an entire reactor with no confinement of the mixture. The mixture is separated internally, within one of more of the reactors, to separate only the converted oil and hydrogen into a vapor product while permitting the unconverted oil and the slurry catalyst to continue on into the next sequential reactor as a liquid product. A portion of the unconverted oil is then converted to lower boiling point hydrocarbons in the next reactor, once again creating a mixture of unconverted oil, hydrogen, converted oil, and slurry catalyst. Further hydroprocessing may occur in additional reactors, fully converting the oil. The oil may alternately be partially converted, leaving a concentrated catalyst in unconverted oil which can be recycled directly to the first reactor.
Abstract translation: 申请人开发了一种新的残渣全加氢转化淤浆反应器系统，其允许催化剂，未转化的油，氢和转化的油在连续混合物中在整个反应器中循环，而不限制混合物。 将混合物在更多的反应器之一内部分离，仅将转化的油和氢分离成蒸气产物，同时允许未转化的油和浆料催化剂作为液体产物继续进入下一个连续的反应器。 然后将未转化的油的一部分转化为下一个反应器中的低沸点烃，再次产生未转化的油，氢，转化的油和浆料催化剂的混合物。 进一步的加氢处理可能发生在额外的反应器中，完全转化油。 油可以替代地部分转化，留下浓缩的催化剂在未转化的油中，其可以直接再循环到第一反应器。
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62.发明申请Direct coal liquefaction with integrated product hydrotreating and catalyst cascading 有权直接煤液化与综合产品加氢处理和催化剂级联公开(公告)号：US20110042272A1
公开(公告)日：2011-02-24
申请号：US12583276
申请日：2009-08-19
Applicant: James B. MacArthur , John E. Duddy
Inventor： James B. MacArthur , John E. Duddy
CPC classification number: C10G1/02 , C10G1/002 , C10G1/06 , C10G1/08 , C10G1/086 , C10G45/04 , C10G45/16
Abstract: A multi-stage catalytic process for the direct liquefaction of coal is utilized with a hydrotreater to first liquefy and subsequently treat the product in one integrated process. A fresh hydrogenation catalyst is used to reduce heteroatoms (S, N) from coal liquids in the downstream hydrotreater. This catalyst is then cascaded and re-used in the direct coal liquefaction process, first in the low temperature Stage 1, and then re-used in the high temperature Stage 2. Coal liquid products have very low contaminants and can be readily used to produce gasoline and diesel fuel. Catalyst requirements are substantially lowered utilizing this novel process.
Abstract translation: 用于直接液化煤的多阶段催化方法与加氢处理器一起利用，以首先在一个整合过程中液化并随后处理该产物。 使用新鲜的氢化催化剂从下游加氢处理机中的煤液中还原杂原子（S，N）。 然后将该催化剂级联并在直接煤液化过程中重新使用，首先在低温阶段1中，然后在高温阶段2中重新使用。煤液体产物具有非常低的污染物并且可以容易地用于生产 汽油和柴油燃料。 利用这种新颖的方法，催化剂需求大大降低。
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公开(公告)号：US20100200463A1
公开(公告)日：2010-08-12
申请号：US12601343
申请日：2008-05-19
Applicant: Luigi Patron , Alberto Malandrino , Mario Molinari
Inventor： Luigi Patron , Alberto Malandrino , Mario Molinari
CPC classification number: C10G65/00 , C10G47/02 , C10G47/26 , C10G49/04 , C10G2300/1003 , C10G2300/1014 , C10G2300/1033 , C10G2300/107 , C10G2300/1077 , C10G2300/207 , Y02P30/20
Abstract: A process for the conversion of heavy oils comprising sending the heavy oil to hydrotreatment, of the high severity type, in the presence of high concentrations of a suitable hydrogenation catalyst dispersed in slurry phase, effected in a suitable solid accumulation reactor capable of operating stably in the presence of solids deriving from and generated by the feedstock charged, wherein the hydrogen or mixtures thereof is fed at suitable flow-rates and suitably distributed, obtaining the conversion products in vapour phase directly in the reactor.
Abstract translation: 一种重油转化方法，包括在高浓度的分散在淤浆相中的合适的氢化催化剂存在下将重油送入高浓度类型的加氢处理剂，该合适的固体积聚反应器能够稳定地运行 由所加入的原料产生的固体的存在，其中氢气或其混合物以合适的流速进料并适当分布，直接在反应器中获得汽相转化产物。
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公开(公告)号：US20050252833A1
公开(公告)日：2005-11-17
申请号：US11139503
申请日：2005-05-31
Applicant: James Doyle , Fred Hildebrandt
Inventor： James Doyle , Fred Hildebrandt
Abstract: Three new embodiments to the Chattanooga Process that convert or upgrade oil bitumen, a combination of oil sands and bitumen, a combination of sand and bitumen, and oil shale to high grade low sulfur (about 0.1 to 0.5 wt. % sulfur, or less) crude oil. The invention relates to a continuous process for producing synthetic crude oil (SCO) from oil sand bitumen which has been extracted from under ground via in situ processes, or strip mined and extracted via hot water extraction processes before upgrading. It can also apply to kerogen extracted in situ from shale underground. The process involves treating the hot bitumen with sand from an extraction process or the hot oil from kerogen with ground shale containing kerogen in a fluid bed reactor where the reactant and fluidizing medium is only hydrogen. The invention also relates to a continuous process for producing synthetic crude oil (SCO) from oil shale kerogen. The invention relates to a continuous process for producing synthetic crude oil from oil bearing material, e.g., oil shale or oil sand (tar sand), through continuous process for producing synthetic crude oil from bituminous oil sand (tar sand) or shale. The process includes treating the oil sand (tar sand) or shale to produce a fluidizable feed, feeding the fluidizable feed to a fluidized bed reactor, and fluidizing and reacting the fluidizable feed in the fluidized bed reactor with a feed of hydrogen provided by a feed stream having a stream containing hydrogen in a concentration greater than 90 vol % (90 vol %-100 vol % H2). In one embodiment, the invention relates to a continuous process which can recover methane and ethane from a recycle hydrogen stream. In one embodiment, the process can recover PSA tail gas as feed to a hydrogen plant. In one embodiment, the process can be operated to reduce or eliminate the requirement for externally provided methane feed to the hydrogen plant.
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65.发明申请Grid plate bubble cap for reaction vessel used in hydroconversion of fossil fuels 有权用于化石燃料加氢转化的反应容器的网板气泡盖公开(公告)号：US20050244311A1
公开(公告)日：2005-11-03
申请号：US11044947
申请日：2005-01-27
Applicant: Thomas Kao , Robert Chang
Inventor： Thomas Kao , Robert Chang
CPC classification number: B01J8/22 , B01J8/224 , B01J8/226 , C10G1/065 , C10G1/083 , C10G47/24 , C10G49/002
Abstract: A catalytic hydrocracking reactor vessel includes enhanced components for the conversion of a hydrogen gas and fossil fuel feedstream to light liquid hydrocarbons. The reactor vessel comprises one or more of a reactor cup riser with a helical cyclonic separator conduit for separating a liquid and vapor product stream to provide an essentially vapor-free liquid recycle stream; a grid plate bubble cap with wall housing having serrated edges for producing small hydrogen bubbles of increased total surface area of bubbles at lower pressure drop; a feedstream inlet pipe sparger containing rows of downward directed slots for even distribution of the feedstream across the cross-sectional area of the reactor and providing free drain of solid particles from the sparger; and optionally a liquid recycle inlet distributor containing vertically curved plates for creating a whirling motion in the liquid recycle stream for better mixing with the feedstream with minimal solids settling.
Abstract translation: 催化加氢裂化反应器容器包括用于将氢气和化石燃料原料流转化为轻质液体烃的增强组分。 反应器容器包括一个或多个具有用于分离液体和蒸汽产物流的螺旋旋风分离器导管的反应器杯提升管，以提供基本上不含蒸气的液体循环流; 具有壁壳的栅板气泡盖，其具有锯齿状边缘，用于产生在较低压降下气泡总表面积增加的小氢气泡; 进料流入口管喷雾器，其包含一排向下定向的槽，用于均匀地分配进料流跨过反应器的横截面积并提供来自喷雾器的固体颗粒的自由排出物; 以及任选的包含垂直弯曲板的液体再循环入口分配器，用于在液体再循环流中产生旋转运动，以更好地与最小固体沉降的进料流混合。
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Patent Agency Ranking
66.发明申请Feedstream inlet sparger for reaction vessel used in hydroconversion of fossil fuels 有权用于化石燃料加氢转化的反应容器的进料流入口喷雾器公开(公告)号：US20050169822A1
公开(公告)日：2005-08-04
申请号：US11044683
申请日：2005-01-27
Applicant: Thomas Kao , Robert Chang
Inventor： Thomas Kao , Robert Chang
CPC classification number: B01J8/22 , B01J8/224 , B01J8/226 , C10G1/065 , C10G1/083 , C10G47/24 , C10G49/002
Abstract: A catalytic hydrocracking reactor vessel includes enhanced components for the conversion of a hydrogen gas and fossil fuel feedstream to light liquid hydrocarbons. The reactor vessel comprises one or more of a reactor cup riser with a helical cyclonic separator conduit for separating a liquid and vapor product stream to provide an essentially vapor-free liquid recycle stream; a grid plate bubble cap with wall housing having serrated edges for producing small hydrogen bubbles of increased total surface area of bubbles at lower pressure drop; a feedstream inlet pipe sparger containing rows of downward directed slots for even distribution of the feedstream across the cross-sectional area of the reactor and providing free drain of solid particles from the sparger; and optionally a liquid recycle inlet distributor containing vertically curved plates for creating a whirling motion in the liquid recycle stream for better mixing with the feedstream with minimal solids settling.
Abstract translation: 催化加氢裂化反应器容器包括用于将氢气和化石燃料原料流转化为轻质液体烃的增强组分。 反应器容器包括一个或多个具有用于分离液体和蒸汽产物流的螺旋旋风分离器导管的反应器杯提升管，以提供基本上不含蒸气的液体循环流; 具有壁壳的栅板气泡盖，其具有锯齿状边缘，用于产生在较低压降下气泡总表面积增加的小氢气泡; 进料流入口管喷雾器，其包含一排向下定向的槽，用于均匀地分配进料流跨过反应器的横截面积并提供来自喷雾器的固体颗粒的自由排出物; 以及任选的包含垂直弯曲板的液体再循环入口分配器，用于在液体再循环流中产生旋转运动，以更好地与最小固体沉降的进料流混合。
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67.发明申请Liquid recycle inlet distributor for reaction vessel used in hydroconversion of fossil fuels 有权用于化石燃料加氢转化的反应容器的液体再循环入口分配器公开(公告)号：US20050129595A1
公开(公告)日：2005-06-16
申请号：US11044690
申请日：2005-01-27
Applicant: Thomas Kao , Robert Chang
Inventor： Thomas Kao , Robert Chang
CPC classification number: B01J8/22 , B01J8/224 , B01J8/226 , C10G1/065 , C10G1/083 , C10G47/24 , C10G49/002
Abstract: A catalytic hydrocracking reactor vessel includes enhanced components for the conversion of a hydrogen gas and fossil fuel feedstream to light liquid hydrocarbons. The reactor vessel comprises one or more of a reactor cup riser with a helical cyclonic separator conduit for separating a liquid and vapor product stream to provide an essentially vapor-free liquid recycle stream; a grid plate bubble cap with wall housing having serrated edges for producing small hydrogen bubbles of increased total surface area of bubbles at lower pressure drop; a feedstream inlet pipe sparger containing rows of downward directed slots for even distribution of the feedstream across the cross-sectional area of the reactor and providing free drain of solid particles from the sparger; and optionally a liquid recycle inlet distributor containing vertically curved plates for creating a whirling motion in the liquid recycle stream for better mixing with the feedstream with minimal solids settling.
Abstract translation: 催化加氢裂化反应器容器包括用于将氢气和化石燃料原料流转化为轻质液体烃的增强组分。 反应器容器包括一个或多个具有用于分离液体和蒸汽产物流的螺旋旋风分离器导管的反应器杯提升管，以提供基本上不含蒸气的液体循环流; 具有壁壳的栅板气泡盖，其具有锯齿状边缘，用于产生在较低压降下气泡总表面积增加的小氢气泡; 进料流入口管喷雾器，其包含一排向下定向的槽，用于均匀地分配进料流跨过反应器的横截面积并提供来自喷雾器的固体颗粒的自由排出物; 以及任选的包含垂直弯曲板的液体再循环入口分配器，用于在液体再循环流中产生旋转运动，以更好地与最小固体沉降的进料流混合。
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公开(公告)号：US20050129586A1
公开(公告)日：2005-06-16
申请号：US10225937
申请日：2002-08-22
Applicant: Thomas Kao , Robert Chang
Inventor： Thomas Kao , Robert Chang
CPC classification number: B01J8/22 , B01J8/224 , B01J8/226 , C10G1/065 , C10G1/083 , C10G47/24 , C10G49/002
Abstract: A catalytic hydrocracking reactor vessel for the conversion of a hydrogen gas and fossil fuel feedstream to light liquid hydrocarbons. The reactor vessel comprises reactor cup riser means with a helical cyclonic separator conduit for separating a liquid and vapor product stream to provide an essentially vapor-free liquid recycle stream, grid plate bubble cap means with tapered bell cap wall housing having serrated edges for producing small hydrogen bubbles of increased total surface area of bubbles at lower pressure drop, optionally feedstream inlet pipe sparger means containing rows of downward directed slots for even distribution of the feedstream across the cross-sectional area of the reactor and providing free drain of solid particles from the sparger, and optionally liquid recycle inlet distributor means containing vertically curved plates for creating a whirling motion in the liquid recycle stream for better mixing with the feedstream with minimal solids settling.
Abstract translation: 用于将氢气和化石燃料原料流转化为轻质液体烃的催化加氢裂化反应器。 反应器容器包括具有用于分离液体和蒸汽产物流的螺旋旋风分离器导管的反应器杯提升装置，以提供基本上不含蒸气的液体循环流，栅格板气泡帽装置，具有锥形壁罩壳体，其具有锯齿状边缘，用于产生小的 氢气泡在较低的压降下气泡的总表面积增加，任选的进料流入口管喷雾器装置包含一排向下指向的槽，用于均匀地分配进料流跨过反应器的横截面积并提供固体颗粒的自由排出 以及任选的液体再循环入口分配器装置，其包含垂直弯曲的板，用于在液体再循环流中产生旋转运动，以便以最少的固体沉降与进料流更好地混合。
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69.发明申请Diesel oil from residues by catalytic depolymerization with energy input from a pump-agitator system 失效通过催化解聚与来自泵 - 搅拌器系统的能量输入的残余物的柴油公开(公告)号：US20050115871A1
公开(公告)日：2005-06-02
申请号：US10891971
申请日：2004-07-15
Applicant: Christian Koch
Inventor： Christian Koch
IPC: B01J29/08 , C10G1/00 , C10G1/02 , C10G1/08 , C10G1/10 , C10G11/00 , C10G11/16 , F24J3/00 , C10G11/05
CPC classification number: C10G1/10 , C10G1/08 , C10G2300/1003 , C10G2300/1011 , C10G2400/04 , F24V40/00 , Y02P30/20
Abstract: Production of diesel oil from hydrocarbon-containing residues in an oil circuit with solids separation and product distillation for the diesel product with energy input by means of pumps and counterrotating agitators and by the use of fully crystallized catalysts of potassium, sodium, calcium, and magnesium-aluminum silicates, where all surfaces are cleaned continuously by the agitator mechanisms.
Abstract translation: 在具有固体分离的油路中的含烃残留物中生产柴油，并通过泵和反旋转搅拌器输入能量的柴油产品进行产物蒸馏，并使用钾，钠，钙和镁的完全结晶的催化剂 铝硅酸盐，其中所有表面通过搅拌机构连续清洁。
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70.发明授权Pyrolysis and hydrolysis of mixed polymer waste comprising polyethyleneterephthalate and polyethylene to sequentially recover 失效包含聚对苯二甲酸乙二醇酯和聚乙烯的混合聚合物废物的热解和水解顺序地回收
公开(公告)号：US5821553A
公开(公告)日：1998-10-13
申请号：US350392
申请日：1994-12-06
Applicant: Robert J. Evans , Helena L. Chum
Inventor： Robert J. Evans , Helena L. Chum
Abstract: A process of using fast pyrolysis in a carrier gas to convert a plastic waste feedstream having a mixed polymeric composition in a manner such that pyrolysis of a given polymer to its high value monomeric constituent occurs prior to pyrolysis of other plastic components therein comprising: selecting a first temperature program range to cause pyrolysis of said given polymer to its high value monomeric constituent prior to a temperature range that causes pyrolysis of other plastic components; selecting a catalyst and support for treating said feed streams with said catalyst to effect acid or base catalyzed reaction pathways to maximize yield or enhance separation of said high value monomeric constituent in said temperature program range; differentially heating said feed stream at a heat rate within the first temperature program range to provide differential pyrolysis for selective recovery of optimum quantities of the high value monomeric constituent prior to pyrolysis of other plastic components; separating the high value monomeric constituents; selecting a second higher temperature range to cause pyrolysis of a different high value monomeric constituent of said plastic waste and differentially heating the feedstream at the higher temperature program range to cause pyrolysis of the different high value monomeric constituent; and separating the different high value monomeric constituent.
Abstract translation: 在载气中使用快速热解以转化具有混合聚合物组合物的塑料废物进料流的方法，使得给定聚合物在其高价值单体组分的热解之前发生在其中其它塑料组分的热解之前，其中包括：选择 第一温度程序范围，以使所述给定的聚合物在导致其它塑料组分的热解的温度范围之前被热分解成其高价值的单体组分; 选择催化剂和用所述催化剂处理所述进料流的载体以实现酸或碱催化的反应途径，以使得所述高价值单体组分在所述温度程序范围内产率最大化或增强分离; 在第一温度程序范围内的热速率差异加热所述进料流，以提供差别热解，以在其它塑料组分的热解之前选择性回收最佳量的高价值单体组分; 分离高价值的单体成分; 选择第二较高温度范围以引起所述塑料废料的不同高价值单体组分的热解，并在较高温度程序范围内差异加热进料流，以引起不同高价值单体组分的热解; 并分离不同的高价值单体成分。
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