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    AMMOXIDATION OF CARBOXYLIC ACIDS TO A MIXTURE OF NITRILES
    1.
    发明申请
    AMMOXIDATION OF CARBOXYLIC ACIDS TO A MIXTURE OF NITRILES 审中-公开
    羧酸对氨基甲酸铵的氧化

    公开(公告)号：WO2003097583A1

    公开(公告)日：2003-11-27

    申请号：PCT/US2003/015983

    申请日：2003-05-16

    Applicant: THE STANDARD OIL COMPANY

    Inventor： GODBOLE, Sanjay, P. ,  PAPARIZOS, Christos ,  SEELY, Michael, J.

    IPC: C07C253/26

    CPC classification number: C07C253/26 ,  Y02P20/52 ,  C07C255/03 ,  C07C255/08

    Abstract: A process for increasing the yield of acetonitrile produced during the manufacture of acrylonitrile comprising introducing a hydrocarbon selected from the group consisting of propylene and propane, a carboxylic acid, ammonia and air into a reaction zone containing an ammoxidation catalyst, reacting the hydrocarbon, carboxylic acid, ammonia and oxygen over said catalyst at an elevated temperature to produce acrylonitrile, hydrogen cyanide and acetonitrile, and recovering the acrylonitrile, hydrogen cyanide and acetonitrile from the reactor.

    Abstract translation: 一种提高丙烯腈生产过程中产生的乙腈产率的方法，包括将选自丙烯和丙烷，羧酸，氨和空气的烃引入到含有氨氧化催化剂的反应区中，使烃，羧酸 ，氨和氧气在所述催化剂上升高，以产生丙烯腈，氰化氢和乙腈，并从反应器回收丙烯腈，氰化氢和乙腈。

    MIXED OXIDE CATALYST OF K, CS, CE, CR, CO, NI, FE, BI AND MO FOR THE MANUFACTURE OF ACRYLONITRILE
    2.
    发明申请
    MIXED OXIDE CATALYST OF K, CS, CE, CR, CO, NI, FE, BI AND MO FOR THE MANUFACTURE OF ACRYLONITRILE 审中-公开
    用于制造丙烯腈的K，CS，CE，CR，CO，NI，FE，BI和MO的混合氧化物催化剂

    公开(公告)号：WO2004050240A1

    公开(公告)日：2004-06-17

    申请号：PCT/US2003/036937

    申请日：2003-11-19

    Applicant: THE STANDARD OIL COMPANY

    Inventor： PAPARIZOS, Christos ,  JEVNE, Stephen, C. ,  SEELY, Michael, J.

    IPC: B01J37/00

    CPC classification number: C07C253/26 ,  B01J23/002 ,  B01J23/8876 ,  B01J23/8878 ,  B01J27/0576 ,  B01J27/1853 ,  B01J27/192 ,  B01J35/023 ,  B01J37/0045 ,  B01J37/0081 ,  B01J2523/00 ,  Y02P20/52 ,  B01J2523/13 ,  B01J2523/15 ,  B01J2523/3712 ,  B01J2523/54 ,  B01J2523/67 ,  B01J2523/68 ,  B01J2523/842 ,  B01J2523/845 ,  B01J2523/847 ,  B01J2523/11 ,  C07C255/08

    Abstract: A catalyst comprising a complex of catalytic oxides comprising potassium, cesium, cerium, chromium, cobalt, nickel, iron, bismuth, molybdenum, wherein the relative ratios of these elements is represented by the following general formula A a K b Cs c Ce d Cr e Co f Ni g X h Fe i Bi j Mo 12 O x wherein A is Rb, Na, Li, TI, or mixtures thereof, X is P, Sb, Te, B, Ge, W, Ca, Mg, a rare earth element, or mixtures thereof, a is about O to about 1, b is about 0.01 to about 1, c is about 0.01 to about 1, d is about 0.01 to about 3, e is about 0.01 to about 2, f is about 0.01 to about 10, g is about 0.1 to about 10, h is about 0 to about 4, i is about 0.1 to about 4, j is about 0.05 to about 4, x is a number determined by the valence requirements of the other elements present, and wherein the catalyst is substantially free of manganese and zinc. The catalyst is useful in processes for the ammoxidation of an olefin selected from the group consisting of propylene, isobutylene or mixtures thereof, to acrylonitrile, methacrylonitrile and mixtures thereof, respectively.

    Abstract translation: 一种催化剂，其包含包含钾，铯，铈，铬，钴，镍，铁，铋，钼的催化氧化物的络合物，其中这些元素的相对比例由以下通式表示：Aa Kb Csc Ced Cre Cof Nig Xh Fei 其中A为Rb，Na，Li，TI或其混合物，X为P，Sb，Te，B，Ge，W，Ca，Mg，稀土元素或其混合物，a为约O 至约1，b为约0.01至约1，c为约0.01至约1，d为约0.01至约3，e为约0.01至约2，f为约0.01至约10，g为约0.1至约 10，h为约0至约4，i为约0.1至约4，j为约0.05至约4，x为由存在的其它元素的化合价要求确定的数，并且其中催化剂基本上不含锰 和锌。 该催化剂可用于分别选自丙烯，异丁烯或其混合物的烯烃与丙烯腈，甲基丙烯腈及其混合物的氨氧化反应的方法。

    MIXED OXIDE CATALYST OF RB, CE, CR, NI, FE, BI AND MO FOR THE MANUFACTURE OF ACRYLONITRILE
    3.
    发明申请
    MIXED OXIDE CATALYST OF RB, CE, CR, NI, FE, BI AND MO FOR THE MANUFACTURE OF ACRYLONITRILE 审中-公开
    RB，CE，CR，NI，FE，BI和MO的混合氧化物催化剂用于制备丙烯腈

    公开(公告)号：WO2004050238A1

    公开(公告)日：2004-06-17

    申请号：PCT/US2003/036940

    申请日：2003-11-19

    Applicant: THE STANDARD OIL COMPANY

    Inventor： PAPARIZOS, Christos ,  JEVNE, Stephen, C. ,  SEELY, Michael, J.

    IPC: B01J23/887

    CPC classification number: C07C253/26 ,  B01J23/002 ,  B01J23/8876 ,  B01J23/8878 ,  B01J27/1853 ,  B01J27/192 ,  B01J35/023 ,  B01J37/0045 ,  B01J37/0081 ,  B01J2523/00 ,  Y02P20/52 ,  B01J2523/11 ,  B01J2523/14 ,  B01J2523/22 ,  B01J2523/3712 ,  B01J2523/54 ,  B01J2523/67 ,  B01J2523/68 ,  B01J2523/842 ,  B01J2523/845 ,  B01J2523/847 ,  B01J2523/12 ,  B01J2523/51 ,  C07C255/08

    Abstract: A catalyst comprising a complex of catalytic oxides comprising rubidium, cerium, chromium, iron, bismuth, molybdenum, and at least one of nickel or nickel and cobalt, optionally magnesium, and optionally one of phosphorus, antimony, tellurium, sodium, lithium, potassium, cesium, thallium, boron, germanium, tungsten calcium, wherein the relative ratios of these elements are represented by the following general formula: Rb a Ce b Cr c Mg d A e Fe f Bi g Y h Mo 12 O x wherein A is Ni or the combination of Ni and Co, Y is at least one of P, Sb, Te, Li, Na, K, Cs, TI, B, Ge, W, Ca, Zn, a rare earth element, or mixtures thereof, a is about 0.01 to about 1, b is about 0.01 to about 3, c is about 0.01 to about 2, d is 0 to about 7, e is about 0.01 to about 10, f is about 0.01 to about 4, g is about 0.05 to about 4, h is 0 to about 3, x is a number determined by the valence requirements of the other elements present, wherein "b" + "c" is greater than "g" and wherein the catalyst is substantially free of manganese, a noble metal and vanadium. The catalyst is useful in processes for the ammoxidation of an olefin selected from the group consisting of propylene, isobutylene or mixtures thereof, to acrylonitrile, methacrylonitrile and mixtures thereof, respectively.

    Abstract translation: 一种催化剂，其包含包含铷，铈，铬，铁，铋，钼以及镍或镍和钴，任选的镁中的至少一种的催化氧化物的复合物，以及任选的磷，锑，碲，钠，锂，钾 ，铯，铊，硼，锗，钨钙，其中这些元素的相对比例由以下通式表示：Rba Ceb Crc Mgd Ae Fef Big Yh Mo12 Ox其中A是Ni或Ni和Co的组合，Y 是P，Sb，Te，Li，Na，K，Cs，TI，B，Ge，W，Ca，Zn，稀土元素或其混合物中的至少一种，a为约0.01至约1，b为 约0.01至约3，c为约0.01至约2，d为0至约7，e为约0.01至约10，f为约0.01至约4，g为约0.05至约4，h为0至约 3，x是由存在的其它元素的化合价要求确定的数，其中“b”+“c”大于“g”，并且其中催化剂基本上不含 锰，贵金属和钒。 该催化剂可用于分别选自丙烯，异丁烯或其混合物的烯烃与丙烯腈，甲基丙烯腈及其混合物的氨氧化反应的方法。

    MIXED OXIDE CATALYST OF RB, CE, CR, NI, FE, BI AND MO FOR THE MANUFACTURE OF ACRYLONITRILE
    7.
    发明公开
    MIXED OXIDE CATALYST OF RB, CE, CR, NI, FE, BI AND MO FOR THE MANUFACTURE OF ACRYLONITRILE 有权
    MISCHOXIDKATALYSATOR AUS RB，CE，CR，NI，FE，BI UND MO ZUR HERSTELLUNG VON ACRYLNITRIL

    公开(公告)号：EP1590083A1

    公开(公告)日：2005-11-02

    申请号：EP03768979.1

    申请日：2003-11-19

    Applicant: THE STANDARD OIL COMPANY

    Inventor： PAPARIZOS, Christos ,  JEVNE, Stephen, C. ,  SEELY, Michael, J.

    IPC: B01J23/887 ,  B01J27/192 ,  B01J37/00 ,  C07C253/26 ,  C07C255/08

    CPC classification number: C07C253/26 ,  B01J23/002 ,  B01J23/8876 ,  B01J23/8878 ,  B01J27/1853 ,  B01J27/192 ,  B01J35/023 ,  B01J37/0045 ,  B01J37/0081 ,  B01J2523/00 ,  Y02P20/52 ,  B01J2523/11 ,  B01J2523/14 ,  B01J2523/22 ,  B01J2523/3712 ,  B01J2523/54 ,  B01J2523/67 ,  B01J2523/68 ,  B01J2523/842 ,  B01J2523/845 ,  B01J2523/847 ,  B01J2523/12 ,  B01J2523/51 ,  C07C255/08

    Abstract: A catalyst comprising a complex of catalytic oxides comprising rubidium, cerium, chromium, iron, bismuth, molybdenum, and at least one of nickel or nickel and cobalt, optionally magnesium, and optionally one of phosphorus, antimony, tellurium, sodium, lithium, potassium, cesium, thallium, boron, germanium, tungsten calcium, wherein the relative ratios of these elements are represented by the following general formula: Rb a Ce b Cr c Mg d A e Fe f Bi g Y h Mo 12 O x wherein A is Ni or the combination of Ni and Co, Y is at least one of P, Sb, Te, Li, Na, K, Cs, Tl, B, Ge, W, Ca, Zn, a rare earth element, or mixtures thereof, a is about 0.01 to about 1, b is about 0.01 to about 3, c is about 0.01 to about 2, d is 0 to about 7, e is about 0.01 to about 10, f is about 0.01 to about 4, g is about 0.05 to about 4, h is 0 to about 3, x is a number determined by the valence requirements of the other elements present, wherein "b"+"c" is greater than "g" and wherein the catalyst is substantially free of manganese, a noble metal and vanadium. The catalyst is useful in processes for the ammoxidation of an olefin selected from the group consisting of propylene, isobutylene or mixtures thereof, to acrylonitrile, methacrylonitrile and mixtures thereof, respectively.

    Abstract translation: 一种催化剂，其包含包含铷，铈，铬，铁，铋，钼以及镍或镍和钴，任选的镁中的至少一种的催化氧化物的复合物，以及任选的磷，锑，碲，钠，锂，钾 ，铯，铊，硼，锗，钨钙，其中这些元素的相对比例由以下通式表示：<？在线公式描述=“在线公式”end =“lead”→> Rb 一 CE b'/ SUB>的Cr C 镁ð A ë的Fe ˚F< ＆lt;＆lt;＆lt;＆lt;＆lt;＆lt;＆lt;＆lt;＆lt; 其中A为Ni或Ni和Co的组合，Y为P，Sb，Te，Li，Na，K，Cs，Tl，B，Ge，W中的至少一种 ，Ca，Zn，稀土元素或其混合物，a为约0.01至约1，b为约0.01至约3，c为约0.01至约2，d为0至约7，e为约0.01至 约10，f约为0.01 u 4为约0.05至约4，h为0至约3，x为由存在的其它元素的化合价要求确定的数，其中“b”+“c”大于“g”，其中 催化剂基本上不含锰，贵金属和钒。 催化剂可用于分别选自丙烯，异丁烯或其混合物的烯烃与丙烯腈，甲基丙烯腈及其混合物的氨氧化反应。

    MIXED OXIDE CATALYST OF K, CS, CE, CR, CO, NI, FE, BI AND MO FOR THE MANUFACTURE OF ACRYLONITRILE
    8.
    发明公开
    MIXED OXIDE CATALYST OF K, CS, CE, CR, CO, NI, FE, BI AND MO FOR THE MANUFACTURE OF ACRYLONITRILE 审中-公开
    MISCHOXIDKATALYSATOR AUS K，CS，CE，CR，CO，NI，FE，BI UND MO ZUR HERSTELLUNG VON ACRYLNITRIL

    公开(公告)号：EP1567263A1

    公开(公告)日：2005-08-31

    申请号：EP03786844.5

    申请日：2003-11-19

    Applicant: THE STANDARD OIL COMPANY

    Inventor： PAPARIZOS, Christos ,  JEVNE, Stephen, C. ,  SEELY, Michael, J.

    IPC: B01J37/00 ,  C07C255/08 ,  C07C253/26 ,  B01J23/887

    CPC classification number: C07C253/26 ,  B01J23/002 ,  B01J23/8876 ,  B01J23/8878 ,  B01J27/0576 ,  B01J27/1853 ,  B01J27/192 ,  B01J35/023 ,  B01J37/0045 ,  B01J37/0081 ,  B01J2523/00 ,  Y02P20/52 ,  B01J2523/13 ,  B01J2523/15 ,  B01J2523/3712 ,  B01J2523/54 ,  B01J2523/67 ,  B01J2523/68 ,  B01J2523/842 ,  B01J2523/845 ,  B01J2523/847 ,  B01J2523/11 ,  C07C255/08

    Abstract: A catalyst comprising a complex of catalytic oxides comprising potassium, cesium, cerium, chromium, cobalt, nickel, iron, bismuth, molybdenum, wherein the relative ratios of these elements is represented by the following general formula Aa Kb Csc Ced Cre Cof Nig Xh Fei Bi j Mo12 Ox wherein A is Rb, Na, Li, TI, or mixtures thereof, X is P, Sb, Te, B, Ge, W, Ca, Mg, a rare earth element, or mixtures thereof, a is about O to about 1, b is about 0.01 to about 1, c is about 0.01 to about 1, d is about 0.01 to about 3, e is about 0.01 to about 2, f is about 0.01 to about 10, g is about 0.1 to about 10, h is about 0 to about 4, i is about 0.1 to about 4, j is about 0.05 to about 4, x is a number determined by the valence requirements of the other elements present, and wherein the catalyst is substantially free of manganese and zinc. The catalyst is useful in processes for the ammoxidation of an olefin selected from the group consisting of propylene, isobutylene or mixtures thereof, to acrylonitrile, methacrylonitrile and mixtures thereof, respectively.

    Abstract translation: 一种催化剂，其包含包含钾，铯，铈，铬，钴，镍，铁，铋，钼的催化氧化物的络合物，其中这些元素的相对比例由以下通式表示： “In-line Formulas”end =“lead”？> A C C ë钴˚F的Ni 克 X ħ的Fe I 铋Ĵ< α-in-line-formula description =“In-line Formulas”end =“tail”？>其中A是Rb，Na， Li，Tl或其混合物，X为P，Sb，Te，B，Ge，W，Ca，Mg，稀土元素或其混合物，a为0至约1，b为约0.01至约1， c为约0.01至约1，d为约0.01至约3，e为约0.01至约2，f为约0.01至约10，g为约0.1至约10，h为0至约4，i为约 0.1至约4，j为约0.05至约4，x为由存在的其它元素的化合价要求确定的数， 并且其中所述催化剂基本上不含锰和锌。 催化剂可用于分别选自丙烯，异丁烯或其混合物的烯烃与丙烯腈，甲基丙烯腈及其混合物的氨氧化反应。

    IMPROVED CATALYST FOR THE MANUFACTURE OF ACRYLONITRILE
    9.
    发明公开
    IMPROVED CATALYST FOR THE MANUFACTURE OF ACRYLONITRILE 有权
    PROCESS丙烯酸生产

    公开(公告)号：EP1309402A2

    公开(公告)日：2003-05-14

    申请号：EP01956103.4

    申请日：2001-08-02

    Applicant: The Standard Oil Company

    Inventor： PAPARIZOS, Christos ,  SEELY, Michael, J. ,  FRIEDRICH, Maria, Strada ,  SURESH, Dev, D.

    IPC: B01J23/00

    CPC classification number: C07C253/26 ,  B01J23/8876 ,  Y02P20/52 ,  C07C255/08

    Abstract: A catalyst composition comprising a complex of catalytic oxides of iron, bismuth, molybdenum, cobalt, cerium, antimony, at least one of nickel or magnesium, and at least one of lithium, sodium, potassium, rubidium, or thallium, and characterized by the following empirical formula: AaBbCcFedBieCofCegSbhMomOx wherein A is at least one of Cr, P, Sn, Te, B, Ge, Zn, In, Mn, Ca, W, or mixtures thereof, B is at least one of Li, Na, K, Rb, Cs, Tl, or mixtures thereof, C is least one of Ni, Mg or mixtures thereof, a is 0 to 4.0, b is 0.01 to 1.5, c is 1.0 to 10.0, d is 0.1 to 5.0, e is 0.1 to 2.0, f is 0.1 to 10.0, g is 0.1 to 2.0, h is 0.1 to 2.0, m is 12.0 to 18.0 and x is a number determined by the valence requirements of the other elements present. The catalyst is useful in processes for the ammoxidation of an olefin selected from the group consisting of propylene, isobutylene or mixtures thereof, to acrylonitrile, methacrylonitrile and mixtures thereof, respectively.

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