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    Production of Aromatics from Methanol and Co-Feeds
    13.
    发明申请
    Production of Aromatics from Methanol and Co-Feeds 有权
    从甲醇和共同饲料生产芳烃

    公开(公告)号：US20160090332A1

    公开(公告)日：2016-03-31

    申请号：US14829399

    申请日：2015-08-18

    Applicant: ExxonMobil Chemical Patents Inc.

    Inventor： John S. Buchanan ,  Stephen H. Brown ,  Lorenzo C. DeCaul ,  Brett T. Loveless ,  Rohit Vijay ,  Stephen J. McCarthy ,  Michel Daage ,  Mayank Shekhar

    IPC: C07C1/20 ,  C07C1/207

    CPC classification number: C07C1/20 ,  C07C1/2076 ,  C07C2529/44 ,  C10G3/49 ,  C10G2400/30 ,  C07C15/00

    Abstract: Methods are provided for improving the yield of aromatics during conversion of oxygenate feeds. An oxygenate feed can contain a mixture of oxygenate compounds, including one or more compounds with a hydrogen index of less than 2, so that an effective hydrogen index of the mixture of oxygenates is between about 1.4 and 1.9. Methods are also provided for converting a mixture of oxygenates with an effective hydrogen index greater than about 1 with a pyrolysis oil co-feed. The difficulties in co-processing a pyrolysis oil can be reduced or minimized by staging the introduction of pyrolysis oil into a reaction system. This can allow varying mixtures of pyrolysis oil and methanol, or another oxygenate feed, to be introduced into a reaction system at various feed entry points.

    Abstract translation: 提供了用于提高含氧化合物进料转化期间芳烃产率的方法。 含氧化合物进料可以含有含氧化合物的混合物，包括氢指数小于2的一种或多种化合物，使得含氧化合物混合物的有效氢指数在约1.4和1.9之间。 还提供了用热解油共同进料将含氧化合物的混合物与有效氢指数大于约1转化的方法。 通过将热解油引入反应体系中，可以减少或最小化共解热解油中的困难。 这可以允许不同的热解油和甲醇或另一种含氧化合物进料的混合物在各种进料入口处被引入反应体系中。

    Process for Converting Oxygenates to Aromatic Hydrocarbons
    14.
    发明申请
    Process for Converting Oxygenates to Aromatic Hydrocarbons 有权
    将氧化剂转化为芳香族烃的方法

    公开(公告)号：US20150175501A1

    公开(公告)日：2015-06-25

    申请号：US14560953

    申请日：2014-12-04

    Applicant: ExxonMobil Chemical Patents Inc.

    Inventor： Nikolaos Soultanidis ,  Mayank Shekhar ,  John S. Coleman ,  Jeevan S. Abichandani ,  Stephen J. McCarthy

    IPC: C07C1/24 ,  C07C2/64 ,  C07C6/00

    CPC classification number: C07C1/22 ,  C07C1/24 ,  C07C2/64 ,  C07C5/2729 ,  C07C6/00 ,  C07C6/06 ,  C07C2529/40 ,  C10G3/49 ,  C10G29/205 ,  C10G2400/30 ,  Y02P30/20 ,  Y02P30/42

    Abstract: Processes for catalytically converting oxygenates to hydrocarbon products having an increased C6-C8 aromatics content therein. A first mixture comprising ≧10.0 wt. % of at least one oxygenate, based on the weight of the first mixture, contacts a catalyst in a fluidized bed reactor to produce a product stream including water, one or more hydrocarbons comprising ≧30.0 wt. % of aromatics, based on the weight of the hydrocarbons in the product stream, hydrogen, and one or more oxygenates. The catalyst comprises at least one molecular sieve, a binder, and at least one element selected from Groups 2-14 of the Periodic Table. At least one water-rich stream, at least one aromatic-rich hydrocarbon stream, and at least one aromatic-depleted hydrocarbon stream are separated from the product stream, and at least a portion of one of the aromatic-rich hydrocarbon stream or the aromatic-depleted hydrocarbon stream is recycled back to the reactor.

    Abstract translation: 将含氧化合物催化转化成其中具有增加的C6-C8芳烃含量的烃产物的方法。 第一混合物包含≥10.0wt。 基于第一混合物的重量，至少一种含氧化合物的％与流化床反应器中的催化剂接触以产生包含水，一种或多种包含≥30.0wt。 ％的芳族化合物，基于产物流中的烃的重量，氢和一种或多种含氧化合物。 催化剂包含至少一种分子筛，粘合剂和选自元素周期表第2-14族的至少一种元素。 将至少一种富水流，至少一种富含芳烃的烃流和至少一种贫芳烃流与产物流分离，并且至少一部分富含芳烃的烃流或芳族烃 将去除的烃流循环回反应器。

    Process for Converting Syngas to Aromatics and Catalyst System Suitable Therefor
    18.
    发明申请
    Process for Converting Syngas to Aromatics and Catalyst System Suitable Therefor 审中-公开
    将合成气转化为芳烃和催化剂体系的方法适用于此

    公开(公告)号：US20160207846A1

    公开(公告)日：2016-07-21

    申请号：US14965099

    申请日：2015-12-10

    Applicant: ExxonMobil Chemical Patents Inc.

    Inventor： Nikolaos Soultanidis ,  Mayank Shekhar ,  John S. Coleman

    IPC: C07C1/20 ,  C07C29/158 ,  C07C29/154 ,  C07C29/36 ,  B01J29/40 ,  B01J23/656

    CPC classification number: C07C1/20 ,  B01J23/6562 ,  B01J29/405 ,  B01J35/0006 ,  C07C29/1518 ,  C07C2529/40 ,  C07C2529/65 ,  C07C2529/70 ,  Y02P20/52 ,  C07C15/04 ,  C07C15/06 ,  C07C15/08 ,  C07C31/04 ,  C07C31/08 ,  C07C31/10

    Abstract: The present invention relates to a multistage process and catalyst system therefor to convert syngas to aromatics. In a first stage, syngas is converted to a C1-C4 alcohol mixture by contacting syngas with a first catalyst comprising rhodium or copper at moderate temperature. In a second stage, the C1-C4 alcohol mixture is converted into an aromatic product by contact with a second catalyst comprising a molecular sieve and at least one Group 8-14 element, the molecular sieve having a Constraint Index about 1 to 12 and a silica to alumina ratio of about 10 to 100 at effective conversion conditions. The final aromatic product is rich in benzene, toluene, and xylenes (e.g. greater than 50% aromatics on a hydrocarbon basis).

    Abstract translation: 本发明涉及一种用于将合成气转化为芳族化合物的多级方法和催化剂体系。 在第一阶段，通过使合成气与中等温度的包含铑或铜的第一催化剂接触将合成气转化为C1-C4醇混合物。 在第二阶段中，C1-C4醇混合物通过与包含分子筛和至少一种第8-14族元素的第二催化剂接触而转化成芳香族产物，分子筛具有约1-12的约束指数和 在有效转化条件下，二氧化硅与氧化铝的比例约为10-100。 最终的芳香族产物富含苯，甲苯和二甲苯（例如在烃基上大于50％的芳族化合物）。

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