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公开(公告)号：US08466081B2
公开(公告)日：2013-06-18
申请号：US13580412
申请日：2011-02-24
Applicant: Linfeng Chen , Tak W. Leung , Tao Tao , Kuanqiang Gao , James X. Shu
Inventor： Linfeng Chen , Tak W. Leung , Tao Tao , Kuanqiang Gao , Xiaodong Huang
CPC classification number: C08F10/06 , C08F110/06 , C08F4/651 , C08F2500/12 , C08F2500/18 , C08F2500/04 , C08F4/654 , C08F4/6465 , C08F4/6494 , C08F4/6495 , C08F4/6497
Abstract: Disclosed are halogenated amide esters that are suitable as internal electron donors in procatalyst compositions. Ziegler-Natta catalyst compositions containing the present procatalyst compositions exhibit improved catalyst activity and/or improved catalyst selectivity and produce propylene-based olefins with broad molecular weight distribution.
Abstract translation: 公开了适合作为前催化剂组合物中的内电子供体的卤化酰胺酯。 包含本发明的前催化剂组合物的齐格勒 - 纳塔催化剂组合物表现出改进的催化剂活性和/或改进的催化剂选择性并产生具有宽分子量分布的丙烯基烯烃。
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公开(公告)号：US20120316299A1
公开(公告)日：2012-12-13
申请号：US13580414
申请日：2011-02-24
Applicant: Linfeng Chen , Tak W. Leung , Tao Tao , James X. Shu , Kuanqiang Gao , Clark C. Williams
Inventor： Linfeng Chen , Tak W. Leung , Tao Tao , James X. Shu , Kuanqiang Gao , Clark C. Williams
CPC classification number: C08F10/06 , C08F110/06 , C08F4/651 , C08F2500/12 , C08F2500/18 , C08F2500/04 , C08F4/654
Abstract: Disclosed is a process for producing a procatalyst composition having an amide ester internal electron donor. The process includes pre-halogenating a procatalyst precursor before reaction with the amide ester and forming the procatalyst composition. Ziegler-Natta catalyst compositions containing the present procatalyst composition exhibit improved catalyst activity and/or improved catalyst selectivity and produce propylene-based olefins with broad molecular weight distribution.
Abstract translation: 公开了一种制备具有酰胺酯内电子给体的前催化剂组合物的方法。 该方法包括在与酰胺酯反应并预先将催化剂前体预卤化并形成前催化剂组合物。 包含本发明的前催化剂组合物的齐格勒 - 纳塔催化剂组合物显示出改进的催化剂活性和/或改进的催化剂选择性并产生具有宽分子量分布的丙烯基烯烃。
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73.发明授权Procatalyst composition with substitute 1,2-phenylene aromatic diester internal donor and method 有权具有替代1,2-亚苯基芳族二酯内给体的助催化剂组合物及方法公开(公告)号：US08288585B2
公开(公告)日：2012-10-16
申请号：US12650834
申请日：2009-12-31
Applicant: Linfeng Chen , Tak W. Leung , Tao Tao
Inventor： Linfeng Chen , Tak W. Leung , Tao Tao
IPC: C07C309/00
CPC classification number: C08F4/6494 , C08F4/76 , C08F110/06 , C08F4/651 , C08F4/6465
Abstract: Disclosed are procatalyst compositions having an internal electron donor which include a substituted phenylene aromatic diester and optionally an electron donor component. Ziegler-Natta catalyst compositions containing the present procatalyst compositions exhibit high activity and produce propylene-based olefins with broad molecular weight distribution.
Abstract translation: 公开了具有内电子给体的前催化剂组合物，其包括取代的亚苯基芳族二酯和任选的电子给体组分。 包含本发明的前催化剂组合物的齐格勒 - 纳塔催化剂组合物表现出高活性并产生具有宽分子量分布的丙烯基烯烃。
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公开(公告)号：US08288304B2
公开(公告)日：2012-10-16
申请号：US12761854
申请日：2010-04-16
Applicant: Linfeng Chen , Tak W. Leung , Tao Tao , Kuanqiang Gao
Inventor： Linfeng Chen , Tak W. Leung , Tao Tao , Kuanqiang Gao
IPC: C08F4/44 , C08F110/06 , B01J31/00
CPC classification number: C08F10/06 , C08F110/06 , C08F4/651 , C08F4/654 , C08F2500/12 , C08F2500/18
Abstract: Disclosed are procatalyst compositions having an internal electron donor which includes an adamantane dicarboxylate and optionally an additional electron donor component. Ziegler-Natta catalyst compositions containing the present procatalyst compositions to produce propylene-based olefins with broad molecular weight distribution.
Abstract translation: 公开了具有内电子给体的前催化剂组合物，其包括金刚烷二羧酸酯和任选的另外的电子给体组分。 齐格勒 - 纳塔催化剂组合物，其含有本发明的主催化剂组合物以生产具有宽分子量分布的丙烯基烯烃。
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75.发明授权Procatalyst composition with multiple internal donor having silyl ester and method 有权具有多个内部供体的主催化剂组合物具有甲硅烷基酯和方法公开(公告)号：US08222357B2
公开(公告)日：2012-07-17
申请号：US12623514
申请日：2009-11-23
Applicant: Linfeng Chen
Inventor： Linfeng Chen
IPC: C08F4/50
CPC classification number: C08F10/06 , C08F110/06 , C08F4/654 , C08F4/651 , C08F2500/04 , C08F2500/18 , C08F2500/12
Abstract: Provided is a procatalyst composition containing a multiple internal electron donor with at least two components, one of which is a silyl ester. The other component of the mixed internal electron donor may be an electron donor component. The electron donor component may be an aromatic acid ester, a di-ether, and combinations thereof. Catalyst compositions containing the multiple internal electron donor exhibit improved hydrogen response during olefin polymerization and produce propylene-based polymers with broad molecular weight distribution, high flexural modulus, and high melt flow rate.
Abstract translation: 提供了含有至少两种组分的多重内电子给体的主催化剂组合物，其中一种是甲硅烷基酯。 混合内电子给体的另一组分可以是电子给体组分。 电子给体组分可以是芳族酸酯，二醚及其组合。 含有多重内电子给体的催化剂组合物在烯烃聚合期间表现出改善的氢响应，并产生具有宽分子量分布，高挠曲模量和高熔体流动速率的基于丙烯的聚合物。
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Patent Agency Ranking
76.发明申请Process for Producing Procatalyst Composition with Alkoxyalkyl Ester Internal Electron Donor and Product 审中-公开用烷氧基烷基酯内部电子给体和产物生产主催化剂组合物的方法公开(公告)号：US20120157295A1
公开(公告)日：2012-06-21
申请号：US12974548
申请日：2010-12-21
Applicant: Linfeng Chen , Tak W. Leung , Kelly Gonzalez , Tao Tao
Inventor： Linfeng Chen , Tak W. Leung , Kelly Gonzalez , Tao Tao
CPC classification number: C08F4/6498 , C08F10/00 , C08F110/06 , C08F4/651 , C08F2500/12 , C08F2500/18 , C08F2500/24
Abstract: Disclosed herein are processes for preparing procatalyst compositions with an internal electron donor containing greater than 4.5 wt % of a compounded alkoxyalkyl ester. Also disclosed are catalyst compositions containing the procatalyst composition and polymers, i.e., propylene-based polymers, produced therefrom. The present procatalyst compositions improve catalyst selectivity, catalyst activity, procatalyst morphology and polymer particle morphology, and improve hydrogen response during olefin polymerization.
Abstract translation: 本文公开了用含有大于4.5重量％的配合的烷氧基烷基酯的内电子给体制备原催化剂组合物的方法。 还公开了含有前催化剂组合物和聚合物的催化剂组合物，即由其制备的基于丙烯的聚合物。 本发明的主催化剂组合物改善催化剂选择性，催化剂活性，原催化剂形态和聚合物颗粒形态，并改善烯烃聚合期间的氢响应。
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公开(公告)号：US08178633B2
公开(公告)日：2012-05-15
申请号：US12970617
申请日：2010-12-16
Applicant: Ping Cai , Linfeng Chen , Jan W. Van Egmond , Michael W. Tilston
Inventor： Ping Cai , Linfeng Chen , Jan W. Van Egmond , Michael W. Tilston
CPC classification number: C08F10/06 , C08F4/649 , C08F4/00 , C08F2500/24 , C08F2500/18
Abstract: The present invention relates to an improvement for gas phase olefin polymerization process under two or more different flow regimes. The process involves adding a mixed electron donor system to a reactor having two or more different flow regimes, wherein the mixed electron donor system comprises at least one selectivity control agent and at least one activity limiting agent. The invention is particularly well suited for reactor systems which include a regime characterized by having a low-velocity or high-solid holdup, which have been reported to have operational problems such as particle agglomeration and formation of polymer “chunks”.
Abstract translation: 本发明涉及在两种或多种不同流动状态下气相烯烃聚合方法的改进。 该方法包括向具有两个或多个不同流动状态的反应器中加入混合电子给体系，其中混合电子给体系包含至少一种选择性控制剂和至少一种活性限制剂。 本发明特别适用于包括具有低速或高固体滞留的状态的反应器系统，其被报告具有诸如颗粒聚集和形成聚合物“块”的操作问题。
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公开(公告)号：US08067510B2
公开(公告)日：2011-11-29
申请号：US12390897
申请日：2009-02-23
Applicant: William G. Sheard , Jeffrey D. Goad , Linfeng Chen
Inventor： William G. Sheard , Jeffrey D. Goad , Linfeng Chen
IPC: C08F2/00 , C08F210/00 , C08L23/00
CPC classification number: C08F10/02 , B01J8/1809 , B01J8/1872 , C08F10/06 , C08F110/06 , C08F210/06 , C08F297/083 , C08F2400/02 , C08L23/10 , C08L23/12 , C08L23/142 , C08L23/16 , C08L2207/02 , C08L2314/02 , C08F2/40 , C08F2/001 , C08F4/6465 , C08F2/34 , C08F4/6494 , C08F2/00 , C08L2666/06 , C08F2500/12 , C08F2500/24 , C08F2500/18 , C08F210/16
Abstract: The present disclosure provides a polymerization process for the production of a high melt flow propylene impact copolymer. The process includes contacting an active propylene-based polymer having a melt flow rate greater than about 100 g/10 min with one or more olefins in a polymerization reactor to form the propylene impact copolymer with a melt flow rate greater than about 60 g/10 min. The production of the high melt flow propylene impact copolymer may occur in one or more polymerization reactors, utilizing standard hydrogen concentration, and no visbreaking.
Abstract translation: 本公开内容提供了用于生产高熔体流动丙烯抗冲共聚物的聚合方法。 该方法包括在聚合反应器中将熔体流动速率大于约100g / 10min的活性丙烯基聚合物与一种或多种烯烃接触以形成丙烯冲击共聚物，其熔体流动速率大于约60g / 10 分钟 高熔体流动丙烯抗冲共聚物的生产可以在一个或多个聚合反应器中发生，利用标准氢浓度，不进行减粘裂化。
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公开(公告)号：US07989383B2
公开(公告)日：2011-08-02
申请号：US12850170
申请日：2010-08-04
Applicant: Linfeng Chen , Richard E. Campbell, Jr.
Inventor： Linfeng Chen , Richard E. Campbell, Jr.
CPC classification number: C08F10/00 , B01J31/0201 , B01J31/0272 , B01J31/04 , B01J31/143 , C08F10/06 , C08F110/06 , C08F4/6496 , C08F4/6495 , C08F4/6494 , C08F4/6465 , C08F2500/12 , C08F2500/18
Abstract: A catalyst composition for the polymerization of propylene comprising one or more Ziegler-Natta procatalyst compositions comprising one or more transition metal compounds and one or more esters of aromatic dicarboxylic acid internal electron donors; one or more aluminum containing cocatalysts; a selectivity control agent (SCA) comprising at least one silicon containing compound containing at least one C1-10 alkoxy group bonded to a silicon atom, and one or more activity limiting agent (ALA) compounds comprising one or more aliphatic or cycloaliphatic carboxylic acids; alkyl-, cycloalkyl- or alkyl(poly)(oxyalkyl)-(poly)ester derivatives thereof; or inertly substituted derivatives of the foregoing.
Abstract translation: 一种用于丙烯聚合的催化剂组合物，其包含一种或多种齐格勒 - 纳塔前催化剂组合物，其包含一种或多种过渡金属化合物和一种或多种芳族二羧酸内电子给体的酯; 一种或多种含铝助催化剂; 包含至少一种含有至少一个与硅原子键合的C 1-10烷氧基的含硅化合物的选择性控制剂（SCA）和一种或多种包含一种或多种脂族或脂环族羧酸的活性限制剂（ALA）化合物; 烷基 - ，环烷基 - 或烷基（聚）（烷氧基） - （聚）酯衍生物; 或惰性取代的衍生物。
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公开(公告)号：US07935766B2
公开(公告)日：2011-05-03
申请号：US12650625
申请日：2009-12-31
Applicant: William G. Sheard , Linfeng Chen
Inventor： William G. Sheard , Linfeng Chen
IPC: C08F297/08 , C08F4/649
CPC classification number: C08F10/06 , C07C37/02 , C07C37/14 , C07C37/16 , C07C37/50 , C07C37/56 , C07C37/60 , C07C67/14 , C08F110/06 , C08F210/06 , C07C69/78 , C08F4/651 , C08F210/16 , C08F2500/12 , C07C39/08 , C08F4/6494 , C08F4/6465 , C08F2500/18 , C08F4/6545
Abstract: Disclosed are propylene impact copolymer compositions, articles thereof, and processes for producing same. Polymerization with an improved catalyst composition provides a propylene impact copolymer with high melt flow and low volatiles content.
Abstract translation: 公开了丙烯抗冲共聚物组合物，其制品及其制备方法。 具有改进的催化剂组合物的聚合提供了具有高熔体流动性和低挥发物含量的丙烯抗冲共聚物。
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