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    PROCESS FOR CONVERSION OF METHANE TO HIGHER HYDROCARBONS, INCLUDING LIQUID FUELS
    81.
    发明申请
    PROCESS FOR CONVERSION OF METHANE TO HIGHER HYDROCARBONS, INCLUDING LIQUID FUELS 有权

    公开(公告)号：US20170101352A1

    公开(公告)日：2017-04-13

    申请号：US15288329

    申请日：2016-10-07

    Applicant: GAS TECHNOLOGY INSTITUTE

    Inventor： Terry MARKER ,  Martin LINCK ,  Jim WANGEROW ,  Pedro ORTIZ-TORAL ,  Naomi KLINGHOFFER

    IPC: C07C1/00 ,  C07C2/86 ,  C01B3/34

    CPC classification number: C07C1/00 ,  C01B3/34 ,  C07C1/322 ,  C07C2/86 ,  C10G50/00 ,  C10G57/02 ,  C10G69/126

    Abstract: Aspects of the invention are associated with the discovery of processes for converting methane (CH4), present in a methane-containing feedstock that may be obtained from a variety of sources such as natural gas, to higher hydrocarbons (e.g., C4+ hydrocarbons) such as gasoline, diesel fuel, or jet fuel boiling-range hydrocarbons, which may optionally be separated (e.g., by fractionation) for use as transportation fuels, or otherwise as blending components for such fuels. Particular aspects of the invention are associated with advantages arising from maintaining reaction conditions that improve the yield of C4+ hydrocarbons. Further aspects relate to the advantages gained by integration of the appropriate reactions to carry out the methane conversion, with downstream separation to recover and recycle desirable components of the reaction effluent, thereby improving process economics to the extent needed for commercial viability.

    Method for producing liquid organic fuels and hydrogen
    82.
    发明授权
    Method for producing liquid organic fuels and hydrogen 有权
    生产液体有机燃料和氢气的方法

    公开(公告)号：US09528190B2

    公开(公告)日：2016-12-27

    申请号：US13719267

    申请日：2012-12-19

    Applicant: GAS TECHNOLOGY INSTITUTE

    Inventor： Qinbai Fan

    IPC: C25B3/00 ,  C25B3/02 ,  C25B9/06 ,  C25B9/08 ,  C25B13/04 ,  C25B1/04 ,  C10L1/02 ,  H01M8/06

    CPC classification number: C25B1/04 ,  C10L1/023 ,  C25B3/02 ,  H01M8/06 ,  Y02E60/366 ,  Y02E60/50

    Abstract: A method for producing organic liquid fuels and other valuable products in which an organic compound is provided to an anode electrode having a metal oxide catalyst disposed on an anode side of an electrolyte membrane, thereby producing an organic liquid fuel and/or other valuable organic product and electrons on the anode side. The electrons are conducted to a cathode electrode disposed on a cathode side of the electrolyte membrane, thereby transforming water provided to the cathode side to H2 gas and hydroxide ions. The method is carried out at a temperature less than or equal to about 160° C., preferably at room temperature.

    Abstract translation: 一种生产有机液体燃料和其它有价值产品的方法，其中向具有设置在电解质膜的阳极侧的金属氧化物催化剂的阳极电极提供有机化合物，由此生产有机液体燃料和/或其它有价值的有机产物 和阳极侧的电子。 电子被传导到设置在电解质膜的阴极侧的阴极电极，从而将提供给阴极侧的水转化为H 2气体和氢氧根离子。 该方法在小于或等于约160℃的温度下进行，优选在室温下进行。

    Non-Faradaic electrochemical promotion of catalytic methane reforming for methanol production
    83.
    发明授权
    Non-Faradaic electrochemical promotion of catalytic methane reforming for methanol production 有权
    用于甲醇生产的非法拉第电化学促进催化甲烷重整

    公开(公告)号：US09499917B2

    公开(公告)日：2016-11-22

    申请号：US14076445

    申请日：2013-11-11

    Applicant: GAS TECHNOLOGY INSTITUTE

    Inventor： Qinbai Fan

    IPC: C25B3/00 ,  C25B3/02 ,  C25B1/04

    CPC classification number: C25B3/02 ,  C25B1/04 ,  C25B13/02 ,  Y02E60/366 ,  Y02P20/132

    Abstract: A method of converting methane to methanol at low temperatures utilizes a reactor including an anode, a cathode, a membrane separator between the anode and cathode, a metal oxide catalyst at the anode and a hydrogen recovery catalyst at the cathode. The method can convert methane to methanol at as rate exceeding the theoretical Faradaic rate due to the contribution of an electrochemical reaction occurring in tandem with a Faradaic reaction.

    Abstract translation: 在低温下将甲烷转化为甲醇的方法利用了包括阳极，阴极，阳极和阴极之间的膜分离器，阳极处的金属氧化物催化剂和阴极处的氢回收催化剂的反应器。 由于与法拉第反应一起发生的电化学反应的贡献，该方法可以以超过理论法拉第率的速率将甲烷转化为甲醇。

    CO-PROCESSING FOR CONTROL OF HYDROPYROLYSIS PROCESSES AND PRODUCTS THEREOF
    85.
    发明申请
    CO-PROCESSING FOR CONTROL OF HYDROPYROLYSIS PROCESSES AND PRODUCTS THEREOF 审中-公开
    用于控制水解过程及其制品的CO加工

    公开(公告)号：US20160312125A1

    公开(公告)日：2016-10-27

    申请号：US14696632

    申请日：2015-04-27

    Applicant: GAS TECHNOLOGY INSTITUTE

    Inventor： Martin B. LINCK ,  Terry L. MARKER ,  Michael J. ROBERTS ,  Larry G. FELIX

    IPC: C10G1/06 ,  C10G3/00

    CPC classification number: C10G1/06 ,  C10G1/002 ,  C10G1/08 ,  C10G3/42 ,  C10G3/50 ,  C10G2300/1011 ,  C10G2300/1014 ,  C10G2300/1018 ,  C10G2300/1022 ,  C10G2300/301 ,  C10G2300/305 ,  C10G2300/307 ,  C10G2400/02 ,  C10G2400/04 ,  C10G2400/08 ,  Y02P30/20

    Abstract: Hydropyrolysis processes are described, in which differing types of feedstocks, including at least one biorenewable feedstock, namely a biomass-containing feedstock, may be co-processed to allow enhancements in operating conditions and/or product properties, depending on changing customer requirements and/or overall market demands. According to specific embodiments, an aliphatic hydrocarbon precursor or an aromatic hydrocarbon precursor is co-processed with the biomass-containing feedstock to enhance an operating condition (e.g., a reactor temperature profile) of the hydropyrolysis process and/or a property (e.g., cetane number) of a liquid product (e.g., a diesel boiling range fraction) obtained from a substantially fully deoxygenated hydrocarbon liquid.

    Abstract translation: 描述了氢解法，其中不同类型的原料，包括至少一种生物可再生原料，即含生物质的原料，可以被共同处理，以允许在操作条件和/或产品性质方面的增强，这取决于不断变化的客户要求和/ 或整体市场需求。 根据具体实施方案，脂族烃前体或芳族烃前体与含生物质的原料共处理以增强加氢热解过程的操作条件（例如，反应器温度分布）和/或性质（例如，十六烷 数量）从基本上完全脱氧的烃液体获得的液体产物（例如柴油沸程级分）。

    BUBBLING BED CATALYTIC HYDROPYROLYSIS PROCESS UTILIZINIG LARGER CATALYST PARTICLES AND SMALL BIOMASS PARTICLES FEATURING AN ANTI-SLUGGING REACTOR
    87.
    发明申请
    BUBBLING BED CATALYTIC HYDROPYROLYSIS PROCESS UTILIZINIG LARGER CATALYST PARTICLES AND SMALL BIOMASS PARTICLES FEATURING AN ANTI-SLUGGING REACTOR 有权
    沸腾床催化水解法过程利用大型催化剂颗粒和小生物颗粒特征抗反应剂

    公开(公告)号：US20150141716A1

    公开(公告)日：2015-05-21

    申请号：US14492840

    申请日：2014-09-22

    Applicant: GAS TECHNOLOGY INSTITUTE

    Inventor： Terry L. MARKER ,  Larry G. FELIX ,  Martin B. LINCK ,  Michael J. ROBERTS

    IPC: C10G1/06 ,  C10L1/04 ,  C10G1/00

    CPC classification number: C10G1/06 ,  B01J8/1809 ,  B01J8/34 ,  B01J23/755 ,  B01J23/882 ,  B01J2208/00061 ,  B01J2208/00115 ,  B01J2208/00548 ,  B01J2208/0084 ,  B01J2219/00252 ,  C10G1/002 ,  C10G1/086 ,  C10G1/10 ,  C10G3/45 ,  C10G3/46 ,  C10G3/50 ,  C10G3/57 ,  C10G2300/1003 ,  C10G2300/1014 ,  C10G2300/1018 ,  C10G2300/202 ,  C10G2400/02 ,  C10G2400/04 ,  C10G2400/08 ,  C10L1/04 ,  C10L2200/0469 ,  C10L2290/02 ,  Y02E50/14 ,  Y02E50/32 ,  Y02P30/20

    Abstract: This invention relates to a process for thermochemically transforming biomass or other oxygenated feedstocks into high quality liquid hydrocarbon fuels. In particular, a catalytic hydropyrolysis reactor, containing a deep bed of fluidized catalyst particles is utilized to accept particles of biomass or other oxygenated feedstocks that are significantly smaller than the particles of catalyst in the fluidized bed. The reactor features an insert or other structure disposed within the reactor vessel that inhibits slugging of the bed and thereby minimizes attrition of the catalyst. Within the bed, the biomass feedstock is converted into a vapor-phase product, containing hydrocarbon molecules and other process vapors, and an entrained solid char product, which is separated from the vapor stream after the vapor stream has been exhausted from the top of the reactor. When the product vapor stream is cooled to ambient temperatures, a significant proportion of the hydrocarbons in the product vapor stream can be recovered as a liquid stream of hydrophobic hydrocarbons, with properties consistent with those of gasoline, kerosene, and diesel fuel. Separate streams of gasoline, kerosene, and diesel fuel may also be obtained, either via selective condensation of each type of fuel, or via later distillation of the combined hydrocarbon liquid.

    Abstract translation: 本发明涉及将生物质或其它含氧原料热化学变换成高质量液体烃燃料的方法。 特别地，使用含有流化催化剂颗粒的深层的催化加氢热解反应器来接受显着小于流化床中的催化剂颗粒的生物质或其它含氧原料的颗粒。 反应器具有设置在反应器容器内的插入物或其它结构，其抑制床的压块，从而使催化剂的磨损最小化。 在床内，生物质原料转化为含有烃分子和其他工艺蒸气的气相产物，以及夹带的固体焦炭产物，其在蒸气流已经从蒸汽流的顶部排出之后与蒸气流分离 反应堆。 当产物蒸气流被冷却到环境温度时，产物蒸气流中的相当大比例的烃可作为疏水性烃的液体流回收，其特性与汽油，煤油和柴油燃料的性质一致。 也可以通过每种类型的燃料的选择性冷凝，或通过后来的组合烃液体的蒸馏来获得单独的汽油，煤油和柴油燃料。

    Hydrodeoxygenation of oxygenated polymers to liquid hydrocarbons
    90.
    发明授权
    Hydrodeoxygenation of oxygenated polymers to liquid hydrocarbons 有权

    公开(公告)号：US12065618B2

    公开(公告)日：2024-08-20

    申请号：US17182783

    申请日：2021-02-23

    Applicant: Gas Technology Institute

    Inventor： Martin B. Linck ,  Terry Marker ,  Pedro Ortiz-Toral ,  Jim Wangerow

    IPC: C10G3/00 ,  B01J23/85 ,  C08J11/16

    CPC classification number: C10G3/49 ,  B01J23/85 ,  C08J11/16 ,  C10G3/50 ,  C10G3/56 ,  C08J2367/02 ,  C10G2300/1003 ,  C10G2300/4012 ,  C10G2400/30

    Abstract: Process are disclosed for converting plastics, and especially thermoplastic oxygenated polymers, by hydrodeoxygenation (HDO) to hydrocarbons, such as aromatic hydrocarbons including benzene, toluene, ethylbenzene, and xylene isomers. These hydrocarbons may be recovered as chemicals and/or fuels, depending on the particular chemical structures of the starting materials, including the presence of oxygen in the polymer backbones. Advantageously, using a sufficiently active catalyst, only moderate conditions, such as in terms of hydrogen partial pressure, are required, in comparison to known hydrotreating processes. This leads to the formation, with fewer non-selective side reactions, of desired liquid hydrocarbons from substantially all carbon in the oxygenated polymer, as well as water from substantially all oxygen in the oxygenated polymer. In some cases, the liquid hydrocarbons obtained are platform chemicals that can be used for a number of specialized purposes. For example, they may be converted to monomers for regenerating the oxygenated polymer or otherwise for producing a different polymer.

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