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    Process for dehydrating methanol to dimethyl ether
    41.
    发明授权
    Process for dehydrating methanol to dimethyl ether 有权

    公开(公告)号：US12084410B2

    公开(公告)日：2024-09-10

    申请号：US17433135

    申请日：2019-02-22

    Applicant: BP P.L.C. ,  BP (CHINA) HOLDINGS LTD

    Inventor： Benjamin James Dennis-Smither ,  John Glenn Sunley ,  Zhiqiang Yang

    IPC: C07C41/09 ,  B01J29/06 ,  B01J29/08 ,  B01J29/18 ,  B01J29/40 ,  B01J29/70

    CPC classification number: C07C41/09 ,  B01J29/06 ,  B01J29/084 ,  B01J29/18 ,  B01J29/40 ,  B01J29/7007 ,  B01J29/7042 ,  B01J29/7046 ,  B01J2229/42

    Abstract: A process for dehydrating methanol to dimethyl ether product in the presence of a catalyst and a promoter, wherein the catalyst is at least one aluminosilicate zeolite, wherein: —the aluminosilicate zeolite is selected from: (i) a zeolite having a 2-dimensional framework structure comprising at least one channel having a 10-membered ring, and having a maximum free sphere diameter of at least 4.8 Angstroms; (ii) a zeolite having a 3-dimensional framework structure comprising at least one channel having a 10-membered ring; or (iii) a zeolite comprising at least one channel having a 12-membered ring; —the promoter is selected from one or more compounds of Formula I: (I) wherein Y is selected from a C1-C4 hydrocarbyl substituent, and wherein each of X and any or all of the Z's may independently be selected from hydrogen, halide, a substituted or unsubstituted hydrocarbyl substituent, or a compound of the formula —CHO, —CO2R, —COR, or —OR, where R is hydrogen or a substituted or unsubstituted hydrocarbyl substituent, and wherein the molar ratio of promoter to methanol is maintained at less than 1.

    Fischer-Tropsch Process, Supported Fischer-Tropsch Synthesis Catalyst and Uses Thereof
    43.
    发明申请
    Fischer-Tropsch Process, Supported Fischer-Tropsch Synthesis Catalyst and Uses Thereof 有权

    公开(公告)号：US20220186123A1

    公开(公告)日：2022-06-16

    申请号：US17554218

    申请日：2021-12-17

    Applicant: BP P.L.C.

    Inventor： Alexander James PATERSON

    IPC: C10G2/00 ,  B01J23/889 ,  B01J35/00 ,  B01J37/02

    Abstract: A process for converting a mixture of hydrogen and carbon monoxide gases to a composition comprising alcohols and liquid hydrocarbons by means of a Fischer-Tropsch synthesis reaction, said process comprising contacting a mixture of hydrogen and carbon monoxide gases, preferably in the form of synthesis gas mixture, with a supported Co—Mn Fischer-Tropsch synthesis catalyst, wherein: the support material of the supported Co—Mn Fischer-Tropsch synthesis catalyst comprises a material selected from titania, zinc oxide, zirconia, and ceria; the supported synthesis catalyst comprises at least 2.5 wt % of manganese, on an elemental basis, based on the total weight of the supported synthesis catalyst; the weight ratio of manganese to cobalt, on an elemental basis, is 0.2 or greater; the molar ratio of hydrogen to carbon monoxide is at least 1; and, the Fischer-Tropsch synthesis reaction is conducted at a pressure in the range of from 1.0 to 10.0 MPa absolute.

    PROCESS
    44.
    发明申请
    PROCESS 有权

    公开(公告)号：US20220098136A1

    公开(公告)日：2022-03-31

    申请号：US17433118

    申请日：2019-02-22

    Applicant: BP P.L.C. ,  BP (CHINA) HOLDINGS LTD

    Inventor： Benjamin James DENNIS-SMITHERS ,  John Glenn SUNLEY ,  Zhiqiang YANG

    IPC: C07C41/09 ,  B01J29/08 ,  B01J29/85 ,  B01J29/18 ,  B01J29/65 ,  B01J29/40 ,  B01J29/70

    Abstract: A process for dehydrating methanol to dimethyl ether product in the presence of a catalyst and a promoter, wherein the catalyst is at least one aluminosilicate zeolite, and the promoter is selected from one or more compounds of Formula I: (I) wherein each of X and any or all of the Y's may independently be selected from hydrogen, halide, a substituted or unsubstituted hydrocarbyl substituent, or a compound of the formula —CHO, —CO2R, —COR, or —OR, where R is hydrogen or a substituted or unsubstituted hydrocarbyl substituent, and wherein the molar ratio of promoter to methanol is maintained at less than 1.

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