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    CATALYST AND METHOD FOR THE CONVERSION OF OXYGENATES TO OLEFINS
    1.
    发明申请
    CATALYST AND METHOD FOR THE CONVERSION OF OXYGENATES TO OLEFINS 审中-公开
    催化剂和工艺含氧化合物转化成烯烃

    公开(公告)号：WO2014001410A3

    公开(公告)日：2014-03-06

    申请号：PCT/EP2013063434

    申请日：2013-06-26

    Applicant: BASF SE ,  BASF SCHWEIZ AG

    Inventor： SPANNHOFF KIRSTEN ,  PATCAS FLORINA CORINA ,  BAY KEREM ,  GAAB MANUELA ,  SCHWAB EKKEHARD ,  HESSE MICHAEL

    IPC: B01J29/40 ,  B01J29/70 ,  B01J37/00 ,  B01J37/02 ,  B01J37/28

    CPC classification number: B01J29/40 ,  B01J29/70 ,  B01J29/7038 ,  B01J37/0009 ,  B01J37/0201 ,  B01J37/28 ,  B01J2229/18 ,  B01J2229/183 ,  B01J2229/186 ,  B01J2229/20 ,  B01J2229/42 ,  Y02P30/20

    Abstract: The present invention relates to a catalyst for the conversion of oxygenates to olefins, the catalyst containing one or more zeolites of an MFI-, MEL- and/or MWW-type structure and particles of one or more metal oxides, wherein the one or more zeolites of the MFI-, MEL- and/or MWW-type structure contain one or more alkaline earth metals, and the particles of the one or more metal oxides contain phosphorus, the phosphorus being at least partially present as an oxide, and the one or more alkaline earth metals being selected from the group consisting of Mg, Ca, Sr, Ba and combinations of two or more of these elements. The invention also relates to the production and use of said catalyst and to a method for the conversion of oxygenates to olefins using the catalyst.

    Abstract translation: 本发明涉及一种用于含氧化合物至烯烃的转化的催化剂，其中所述催化剂包括MFI，MEL和/或由MWW型结构的一种或多种沸石，以及一种或多种金属氧化物的粒子，其中该MFI的一种或多种沸石， 含有MEL和/或由MWW型结构，一种或多种碱土金属和磷的一种或多种金属氧化物的颗粒，其中，所述磷以氧化物形式至少部分地，并且其中，所述选择的一个或更多种碱土选自下组的金属 镁，钙，锶，钡，以及两种或更多种的组合，其制备和用途，以及用于含氧物转化为使用该催化剂的烯烃的方法的组合。

    SILICON-BRIDGED PILLARED SILICATE COMPOUNDS AND PROCESS FOR THEIR PRODUCTION
    2.
    发明申请
    SILICON-BRIDGED PILLARED SILICATE COMPOUNDS AND PROCESS FOR THEIR PRODUCTION 审中-公开
    有机硅填料的硅酸盐化合物及其生产工艺

    公开(公告)号：WO2015032851A3

    公开(公告)日：2015-06-04

    申请号：PCT/EP2014068822

    申请日：2014-09-04

    Applicant: BASF SE ,  TOKYO INST TECH

    Inventor： FEYEN MATHIAS ,  RUETZ ROGER ,  MÜLLER ULRICH ,  GAAB MANUELA ,  BAO XINHE ,  ZHANG WEIPING ,  DE VOS DIRK ,  WEISS RALF ,  GIES HERMANN ,  TATSUMI TAKASHI ,  XIAO FENG-SHOU ,  TOSHIYUKI YOKOI ,  YILMAZ BILGE ,  DE BAERDEMAEKER TREES

    IPC: C01B37/02 ,  B01J29/035 ,  B01J29/04 ,  C01B33/38 ,  C01B39/02 ,  C01B39/46 ,  C01B39/48 ,  C04B35/16 ,  C07C1/20 ,  C07C11/02 ,  C10G3/00

    CPC classification number: B01J29/035 ,  B01J29/049 ,  B01J29/06 ,  B01J35/002 ,  B01J35/1019 ,  B01J2229/32 ,  B01J2229/37 ,  B01J2229/40 ,  B01J2229/42 ,  C01B33/38 ,  C04B35/16 ,  C04B2235/5409 ,  C07C1/20 ,  C07C2521/08 ,  C07C2529/00 ,  C07C11/02

    Abstract: The present invention relates to a process for the preparation of a pillared silicate compound comprising a layered silicate structure and bridging silicon atoms located between adjacent silicate layers of the silicate structure, wherein said bridging silicon atoms form at least one covalent bond to each of the adjacent silicate layers, said process comprising (1) providing one or more layered silicates; (2) adding said one or more layered silicates to a solvent system, wherein the resulting mixture has a pH of 5 or less; and (3) subjecting the mixture obtained in step (2) to solvothermal conditions; wherein no silicon-containing compound according to formula (I) R4-mSi[-(SiR2)n-R]m (I) is used at any point of the process up to and including step (3), wherein m is 1, 2, 3, or 4, and n is an integer greater than or equal to 0, wherein when n is equal to 0, one or more residues R are leaving groups, and wherein none of the residues R contains Si, as well as to a pillared silicate compound per se, preferably as obtained and/or obtainable according to the inventive process as well as to the use of the inventive compounds. A further process is disclosed wherein a sulfur oxoacid is present in step (2), and wherein a silicon-containing compound may or may not be used.

    Abstract translation: 本发明涉及一种制备柱状硅酸盐化合物的方法，其包括层状硅酸盐结构和位于硅酸盐结构的相邻硅酸盐层之间的桥连硅原子，其中所述桥连硅原子与相邻的每个相邻的硅酸盐层形成至少一个共价键 所述方法包括（1）提供一层或多层层状硅酸盐; （2）将所述一种或多种层状硅酸盐加入到溶剂体系中，其中所得混合物的pH为5以下; 和（3）将步骤（2）中获得的混合物经受溶剂热条件; 其中在直到并包括步骤（3）的任何一个步骤中，不使用根据式（I）的含硅化合物R 4-m Si [ - （SiR 2）n R] m（I），其中m为1,2， 3或4，并且n是大于或等于0的整数，其中当n等于0时，一个或多个残基R是离去基团，并且其中残基R中没有一个含有Si，以及被支化的 硅酸盐化合物本身，优选根据本发明方法获得和/或可获得，以及本发明化合物的用途。 公开了另一种方法，其中在步骤（2）中存在硫含氧酸，并且其中可以使用或不使用含硅化合物。

    POST-TREATMENT OF DEBORONATED ZEOLITE BETA
    5.
    发明专利
    POST-TREATMENT OF DEBORONATED ZEOLITE BETA 未知

    公开(公告)号：MY185228A

    公开(公告)日：2021-04-30

    申请号：MYPI2015001014

    申请日：2013-10-09

    Applicant: BASF SE

    Inventor： GERLACH OLGA ,  YANG JEFF ,  SEIDEL KARSTEN ,  PARVULESCU ANDREI-NICOLAE ,  GAAB MANUELA ,  MAURER STEFAN ,  MULLER ULRICH

    Abstract: A process for the post-treatment of a zeolitic material having a BEA framework structure, the process comprising (i) providing a zeolitic material having a BEA framework structure, wherein the framework structure of the zeolitic material comprises X203 and Y02, wherein Y is a tetravalent element and X is a trivalent element and wherein the molar ratio X203 : Y02 is greater than 0.02 : 1; (ii) treating the zeolitic material provided in (i) with a liquid solvent system thereby obtaining a zeolitic material having a molar ratio X203 : Y02 of at most 0.02 : 1, and at least partially separating the zeolitic material from the liquid solvent system; (iii) treating the zeolitic material obtained from (ii) with a liquid aqueous system having a pH in the range of 5.5 to 8 and a temperature of at least 75 ?C.

    CATALYST AND PROCESS FOR THE CONVERSION OF OXYGENATES TO OLEFINS
    6.
    发明专利
    CATALYST AND PROCESS FOR THE CONVERSION OF OXYGENATES TO OLEFINS 未知

    公开(公告)号：CA2877560C

    公开(公告)日：2020-07-21

    申请号：CA2877560

    申请日：2013-06-26

    Applicant: BASF SE

    Inventor： SPANNHOFF KIRSTEN ,  PATCAS FLORINA CORINA ,  BAY KEREM ,  GAAB MANUELA ,  SCHWAB EKKEHARD ,  HESSE MICHAEL

    IPC: B01J37/28 ,  B01J29/70 ,  B01J37/00 ,  B01J37/02 ,  C07C1/00

    Abstract: The present invention relates to a catalyst for the conversion of oxygenates to olefins, the catalyst containing one or more zeolites of an MFI-, MEL- and/or MWW-type structure and particles of one or more metal oxides, wherein the one or more zeolites of the MFI-, MEL- and/or MWW-type structure contain one or more alkaline earth metals, and the particles of the one or more metal oxides contain phosphorus, the phosphorus being at least partially present as an oxide, and the one or more alkaline earth metals being selected from the group consisting of Mg, Ca, Sr, Ba and combinations of two or more of these elements. The invention also relates to the production and use of said catalyst and to a method for the conversion of oxygenates to olefins using the catalyst.

    PROCESS FOR ION EXCHANGE ON ZEOLITES
    10.
    发明专利
    PROCESS FOR ION EXCHANGE ON ZEOLITES 未知

    公开(公告)号：IN3736CHN2014A

    公开(公告)日：2015-09-04

    申请号：IN3736CHN2014

    申请日：2014-05-16

    Applicant: BASF SE

    Inventor： LUYKEN HERMANN ,  GAAB MANUELA ,  FISCHER ROLF HARTMUTH

    IPC: C01B39/02

    Abstract: The present invention relates to an improved process for exchanging alkali metal or alkaline earth metal ions in zeolites for ammonium ions. For this exchange aqueous solutions of ammo nium salts for example ammonium sulfate ammonium nitrate or ammonium chloride are cur rently being used. The resulting 'ammonium zeolites' are calcined to convert them with release of ammonia to the H form of the zeolites suitable as a catalyst. It is proposed in accordance with the invention to use ammonium carbonate instead of the am monium compounds mentioned. Since excess ammonium carbonate in contrast to the nitrates sulfates or chlorides can be recycled in the form of carbon dioxide and ammonia the amount of salt which has to be discharged is lowered significantly.

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