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    3.
    发明专利
    未知

    公开(公告)号：DE60139117D1

    公开(公告)日：2009-08-13

    申请号：DE60139117

    申请日：2001-08-31

    Applicant: MITSUI CHEMICALS INC

    Inventor： KOJOH SHINICHI ,  MATSUGI TOMOAKI ,  KASHIWA NORIO

    IPC: C08G81/02 ,  C08F255/00 ,  C08F255/02 ,  C08L23/00 ,  C08L101/00

    Abstract: The present invention is intended to provide a branched polyolefin having various excellent properties, a process for preparing the branched polyolefin and a thermoplastic resin composition containing the branched polyolefin. This branched polyolefin comprises an olefin chain (A) and olefin chain(s) (B) which have recurring units obtained from at least one olefin as main constituent units. In the branched polyolefin, the olefin chain (B) is linked to a position other than both ends of the olefin chain (A), and at least one olefin chain (B) per one olefin chain (A) is present. The process for preparing a branched polyolefin comprises allowing a functional group-containing polyolefin (C) having one or more carboxyl groups and/or acid anhydride groups at positions other than both ends to react with a terminal modified polyolefin (D) having a group capable of reacting with a carboxyl group or an acid anhydride group at only the position of chain end.

    Propylene copolymer, polypropylene composition, use thereof, transition metal compounds, and catalysts for olefin polymerization
    4.
    发明专利
    Propylene copolymer, polypropylene composition, use thereof, transition metal compounds, and catalysts for olefin polymerization 未知

    公开(公告)号：AU2009200068A1

    公开(公告)日：2009-02-05

    申请号：AU2009200068

    申请日：2009-01-07

    Applicant: MITSUI CHEMICALS INC

    Inventor： KANEYOSHI HIROMU ,  HIROTA NARITOSHI ,  INOUE NORIHIDE ,  OKADA KEIJI ,  MORI RYOJI ,  KAWAHARA NOBUO ,  FUNAYA MUNEHITO ,  KASHIWA NORIO ,  TAKAYASU HIROSHI ,  KAWAI KOJI ,  KOJOH SHINICHI ,  IKENAGA SHIGENOBU

    IPC: C08F210/06 ,  C08F4/64 ,  C08F4/6592 ,  C08L23/14

    Abstract: The present invention provides a propylene/1-butene random copolymer (PBR) having excellent flexibility, impact resistance, heat resistance and low-temperature heat-seal properties, a polypropylene composition containg the copolymer, a sheet, film or stretched film comprising the composition and a composite film having a layer of the composition. The propylene/1-butene random copolymer contains 60 to 90 mol% of propylene units and 10 to 40 mol% of 1-butene units and has a triad isotacticity of not less than 85% and not more than 97.5 %, a molecular weight distribution (Mw/Mn) of from 1 to 3, an intrinsic viscosity of from 0.1 to 12 dl/g, a melting point (Tm) of from 40 to 120°C, and satisfies the following relation wherein Tm represents a melting point and M (mol%) represents a content of 1-butene constituent units. The invention, further, provides a transition metal compound useful as an olefin polymerization catalyst and an olefin polymerization catalyst containing the transition metal compound. The transition metal compound is represented by the following formula (2a): wherein each of R 1 and R 3 is hydrogen, R 2 and R 4 are selected from a hydrocarbon group and silicon-containing group, R 5 to R 13 are selected from hydrogen, a hydrocarbon group and silicon-containing group, and adjacent substituent groups R 5 to R 12 may be linked to form a ring. R 14 is an aryl group, and R 13 and R 14 may be linked to form a ring. M is a Group 4 transition metal, Y is a carbon atom, Q is halogen, etc, and j is an integer of 1 to 4.

    5.
    发明专利
    未知

    公开(公告)号：AT420899T

    公开(公告)日：2009-01-15

    申请号：AT03019527

    申请日：2003-08-29

    Applicant: MITSUI CHEMICALS INC

    Inventor： KANEKO HIDEYUKI ,  KOJOH SHIN-ICHI ,  KAWAHARA NOBUO ,  MATSUO SHINGO ,  MATSUGI TOMOAKI ,  SAITO JUNJI ,  MATSUURA SADAHIKO ,  MIYAZAKI KAZUHISA ,  KASHIWA NORIO

    IPC: C08F8/00 ,  C08F10/00 ,  C08F12/12 ,  C08F290/04 ,  C08F299/00 ,  C08G18/62

    Abstract: A novel graft polymer useful in various uses that has a polyolefin backbone having polyolefin segments excellent in moldability can be obtained by homopolymerizing a novel polyolefin macromonomer or polymerizing the novel polyolefin macromonomer in the coexistence of other olefins depending on need, wherein the macromonomer has at the terminal of its polyolefin chain a vinyl group whose ± -position may be substituted, and the macromonomer can be efficiently obtained by a method, for example, successively carrying out i) a step of producing a polyolefin having a hydroxyl group at the terminal of the polyolefin chain and ii) a step of converting the terminal hydroxyl group of the polyolefin chain into an acryloyl group, a methacryloyl group or a styryl group.

    7.
    发明专利
    未知

    公开(公告)号：DE60124829D1

    公开(公告)日：2007-01-11

    申请号：DE60124829

    申请日：2001-09-07

    Applicant: MITSUI CHEMICALS INC

    Inventor： IMUTA JUNICHI ,  KASHIWA NORIO ,  OTA SEIJI ,  MORIYA SATORU ,  NOBORI TADAHITO ,  MIZUTANI KAZUMI

    IPC: C08F210/02 ,  C08F4/659 ,  C08F4/6592 ,  C08F210/00 ,  C08F210/06 ,  C08F210/08 ,  C08F210/14 ,  C08F210/16 ,  C08L23/00

    Abstract: The present invention is intended to provide a polar group-containing olefin copolymer having excellent adhesion properties to metals or polar resins and excellent compatibility therewith, a thermoplastic resin composition containing the copolymer, and uses thereof. The polar group-containing olefin copolymer comprises a constituent unit represented by the following formula (1) and a constituent unit represented by the following formula (4), and optionally a constituent unit represented by the following formula (5), having a molecular weight distribution (Mw/Mn) of not more than 3, and having an intensity ratio of T±² to T±± (T±²/T±±), as determined from a 13 C-NMR spectrum of said copolymer, of not more than 1.0: wherein R 1 is a hydrogen atom or a straight-chain or branched aliphatic hydrocarbon group of 1 to 18 carbon atoms; R 5 is a hydrocarbon group; R 6 is a hetero atom or a group containing a hetero atom; r is 0 or 1; Z is a polymer segment obtained by any one of anionic polymerization, ring-opening polymerization and polycondensation; W is a hydroxyl group or an epoxy group; p is an integer of 1 to 3, q is 0, 1 or 2, and p+q ‰ 3; when p is 2 or 3, each -O-Z may be the same or different, and in this case, if r is 0, -O-Z may be bonded to the same or different atom of R 5 , and if r is 1, -O-Z may be bonded to the same or different atom of R 6 ; when q is 2, each W may be the same or different, and in this case, if r is 0, W may be bonded to the same or different atom of R 5 , and if r is 1, W may be bonded to the same or different atom of R 6 ; in case of p‰¥1 and q‰¥1, if r is 0, W and -O-Z may be bonded to the same or different atom of R 5 , and if r is 1, W and -O-Z may be bonded to the same or different atom of R 6 ; m is 0 or 1; n is an integer of 1 to 3; and when n is 2 or 3, each W may be the same or different, and in this case, if m is 0, W may be bonded to the same or different atom of R 6 , and if m is 1, W may be bonded to the same or different atom of R 7 . The polar group-containing olefin copolymer and the thermoplastic resin composition containing the copolymer are used for films, sheets, modifiers, building/civil engineering materials, automobile exterior trim, electric/electronic parts, coating bases, compatibilizing agents, etc.

    8.
    发明专利
    未知

    公开(公告)号：DE60301042T2

    公开(公告)日：2006-04-20

    申请号：DE60301042

    申请日：2003-10-10

    Applicant: MITSUI CHEMICALS INC

    Inventor： MATSUGI TOMOAKI ,  KAWAHARA NOBUO ,  KANEKO HIDEYUKI ,  MATSUO SHINGO ,  KOJOH SHIN-ICHI ,  KASHIWA NORIO

    IPC: C08F255/00 ,  C08F299/00 ,  C08F8/00 ,  C08F287/00 ,  C08F290/00 ,  C08F291/00 ,  C08F293/00 ,  C08L23/04 ,  C08L23/08 ,  C08L51/06 ,  C08L53/00 ,  C09D151/06 ,  C09D153/00 ,  C09J151/06 ,  C09J153/00

    Abstract: A branched olefin copolymer comprises a branched building block containing polar functional groups and formed by radical polymerization reaction or anion polymerization reaction. A branched olefin copolymer comprises a building block A of formula (1) and a building block B of formula (2). -CH 2-CH(R 1>)- (1) [Image] R 1>H or 1-18C linear or branched aliphatic hydrocarbon; R 2>linear or branched aliphatic or aromatic hydrocarbon; F : heteroatom or heteroatom-containing linking group; Z : polymer segment containing O, N, halo, or aryl and having a molecular weight distribution of 1.0-3.0; W : alcoholic hydroxyl, phenolic hydroxyl, carboxylic acid, carboxylate, acid anhydride, amino, epoxy, siloxy, or mercapto; n : 1-3; m : 0-2. When n is 2 or 3, Z may be the same or different to each other. When m is 2, W may be the same or different to each other. W may be bound to the same or different atom of R 2>to form a cyclic structure. An independent claim is also included for a process for producing the branched olefin copolymer by sequentially conducting a step of synthesizing a polar group-containing olefin copolymer Q containing functional group G, preferably hydroxyl, carboxylic acid, ester, amino, epoxy, silanol, or acid anhydride; a step of converting the functional group G into a group having an ability to initiate radical polymerization; and a step of installing a polymer segment Z in the building block B in the branched olefin copolymer by radical polymerization of a monomer comprising a carbon-carbon double bond-containing compound R containing oxygen, nitrogen, halo or aryl.

    9.
    发明专利
    未知

    公开(公告)号：DE60301042D1

    公开(公告)日：2005-08-25

    申请号：DE60301042

    申请日：2003-10-10

    Applicant: MITSUI CHEMICALS INC

    Inventor： MATSUGI TOMOAKI ,  KAWAHARA NOBUO ,  KANEKO HIDEYUKI ,  MATSUO SHINGO ,  KOJOH SHIN-ICHI ,  KASHIWA NORIO

    IPC: C08F299/00 ,  C08F8/00 ,  C08F255/00 ,  C08F287/00 ,  C08F290/00 ,  C08F291/00 ,  C08F293/00 ,  C08L23/04 ,  C08L23/08 ,  C08L51/06 ,  C08L53/00 ,  C09D151/06 ,  C09D153/00 ,  C09J151/06 ,  C09J153/00

    Abstract: A branched olefin copolymer comprises a branched building block containing polar functional groups and formed by radical polymerization reaction or anion polymerization reaction. A branched olefin copolymer comprises a building block A of formula (1) and a building block B of formula (2). -CH 2-CH(R 1>)- (1) [Image] R 1>H or 1-18C linear or branched aliphatic hydrocarbon; R 2>linear or branched aliphatic or aromatic hydrocarbon; F : heteroatom or heteroatom-containing linking group; Z : polymer segment containing O, N, halo, or aryl and having a molecular weight distribution of 1.0-3.0; W : alcoholic hydroxyl, phenolic hydroxyl, carboxylic acid, carboxylate, acid anhydride, amino, epoxy, siloxy, or mercapto; n : 1-3; m : 0-2. When n is 2 or 3, Z may be the same or different to each other. When m is 2, W may be the same or different to each other. W may be bound to the same or different atom of R 2>to form a cyclic structure. An independent claim is also included for a process for producing the branched olefin copolymer by sequentially conducting a step of synthesizing a polar group-containing olefin copolymer Q containing functional group G, preferably hydroxyl, carboxylic acid, ester, amino, epoxy, silanol, or acid anhydride; a step of converting the functional group G into a group having an ability to initiate radical polymerization; and a step of installing a polymer segment Z in the building block B in the branched olefin copolymer by radical polymerization of a monomer comprising a carbon-carbon double bond-containing compound R containing oxygen, nitrogen, halo or aryl.

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