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    31.
    发明专利
    未知

    公开(公告)号：AT466826T

    公开(公告)日：2010-05-15

    申请号：AT04804421

    申请日：2004-12-30

    Applicant: BASF SE

    Inventor： JOHANN THORSTEN ,  SCHINDLER GOETZ-PETER ,  BRODHAGEN ANDREAS ,  CRONE SVEN ,  BENFER REGINA ,  HILL THOMAS ,  DUDA MARK

    IPC: C07C5/333 ,  C07C5/48 ,  C07C11/167

    Abstract: The disclosure relates to a process for preparing butadiene. The process involves nonoxidatively catalytically dehydrogenating butane to obtain a product gas stream containing butane, 1-butene, 2-butene, butadiene, hydrogen and secondary constituents. The 1-butene and 2-butene of the product gas stream is then oxidatively dehydrogenated to give a second gas stream containing butane,2-butene, butadiene, hydrogen, steam and secondary constituents. Next, the butane,2-butene and butadiene are separated from the second gas stream and the butane and 2-butene are then separated from the butadiene product. The butane and 2-butene are then recycled into the nonoxidative catalytic dehydrogenating zone.

    Reactor from plated stainless steel for the continuous heterogeneously catalyzed partial dehydration of at least one hydrocarbon to be dehydrated, and corresponding method
    32.
    发明专利
    Reactor from plated stainless steel for the continuous heterogeneously catalyzed partial dehydration of at least one hydrocarbon to be dehydrated, and corresponding method 未知

    公开(公告)号：ZA200900538B

    公开(公告)日：2010-04-28

    申请号：ZA200900538

    申请日：2009-01-23

    Applicant: BASF SE

    Inventor： HECHLER CLAUS ,  RUPPEL WILHELM ,  SCHINDLER GOETZ-PETER ,  KLANNER CATHARINA ,  BASSLER HANS-JUERGEN ,  DIETERLE MARTIN ,  KLAPPERT KARL-HEINRICH ,  MUELLER-ENGEL KLAUS JOACHIM

    IPC: B01J20100101 ,  B32B20100101 ,  C07C20100101

    Abstract: Continuous heterogeneously catalyzed partial dehydrogenation of at least one hydrocarbon to be dehydrogenated in the gas phase involves at least one catalyst bed disposed in the reaction chamber and with generation of a product gas comprising the at least one dehydrogenated hydrocarbon, unconverted hydrocarbon to be dehydrogenated and molecular hydrogen and/or steam, is dehydrogenated partially in an oxidative or non-oxidative manner to at least one dehydrogenated hydrocarbon, and at least one product gas stream is withdrawn continuously from the reaction chamber. Process for continuous heterogeneously catalyzed partial dehydrogenation of at least one hydrocarbon to be dehydrogenated in the gas phase involves a reaction chamber enclosed by a shell which is in contact with the reaction chamber and has at least one first orifice for feeding at least one starting gas stream into the reaction chamber and at least one second orifice for withdrawing at least one product gas stream from the reaction chamber, at least one starting gas stream comprising at least one hydrocarbon to be dehydrogenated is fed continuously in the reaction chamber. The at least one hydrocarbon to be dehydrogenated is conducted through at least one catalyst bed disposed in the reaction chamber and with generation of a product gas comprising the at least one dehydrogenated hydrocarbon, unconverted hydrocarbon to be dehydrogenated and molecular hydrogen and/or steam, is dehydrogenated partially in an oxidative or non-oxidative manner to at least one dehydrogenated hydrocarbon, and at least one product gas stream is withdrawn continuously from the reaction chamber. The shell is manufactured from a composite material which, on its side B in contact with the reaction chamber, consists of steel B comprising (wt.%): chromium (18-30), nickel (9-37), silicon (1-4), aluminum (>=0-4), nitrogen (>=0-0.3), carbon (>=0-0.15), manganese (>=0-4), phosphorus (>=0-0.05), sulfur (>=0-0.05), and at least one rare earth metal (>=0-0.1), and iron and impurities resulting from production. The steel B, on its side A facing away from the reaction chamber, is plated either directly or via an intermediate layer of copper, and/or nickel, onto steel A comprising (wt.%): chromium (15-20), nickel (6-18), silicon (>=0-0.8), aluminum (>=0-0.8), nitrogen (>=0-0.3), carbon (>=0-0.15), molybdenum (>=0-4), manganese (>=0-2), titanium (>=0-0.8), niobium (>=0-1.2), vanadium (>=0-0.9), boron (>=0-0.1), phosphorus (>=0-0.05), sulfur (>=0-0.05), iron and impurities resulting from production, or a composition comprising (wt.%) Cr (19-23), Ni (30-35), Co (>=0-1), Si (>=0-1), Al (0.15-0.7), C (>=0-0.12), Mn (>=0-2), Cu (>=0-0.75), Ti (0.15-0.7), Nb (>=0-0.1), P (>=0-0.05), S (>=0-0.05) and iron and impurities resulting from production. An independent claim is included for a shell encloses an interior and has at least one first orifice for feeding at least one gas stream into the interior and at least one second orifice for withdrawing a gas stream fed to the interior beforehand via the at least one first orifice O1 from the interior. The shell is manufactured from a composite material which, on its side B in contact with the reaction chamber, consists of steel B on its side A facing away from the reaction chamber is plated either directly or via an intermediate layer of copper and/or nickel onto steel A.

    34.
    发明专利
    未知

    公开(公告)号：DE502004006964D1

    公开(公告)日：2008-06-05

    申请号：DE502004006964

    申请日：2004-12-30

    Applicant: BASF SE

    Inventor： JOHANN THORSTEN ,  SCHINDLER GOETZ-PETER ,  BRODHAGEN ANDREAS ,  CRONE SVEN ,  DUDA MARK

    IPC: C07C5/333 ,  C07C5/48 ,  C07C11/167

    Abstract: The disclosure involves a process for preparing butadiene from n-butane. In the process, n-butane is first dehydrogenated autothermally under nonoxidative conditions to form a gas stream. The gas stream is then oxidatively dehydrogenated to form a second gas stream. From the second gas stream, a third gas stream containing n-butane, 2-butene and butadiene is obtained. From the third gas stream, a butadiene/butaine product stream is obtained and remaining n-butane and 2-butene is recycled into the first dehydrogenation zone.

    36.
    发明专利
    未知

    公开(公告)号：AT552047T

    公开(公告)日：2012-04-15

    申请号：AT07765633

    申请日：2007-06-26

    Applicant: BASF SE

    Inventor： HECHLER CLAUS ,  RUPPEL WILHELM ,  SCHINDLER GOETZ-PETER ,  HORSTMANN CATHARINA ,  BASSLER HANS-JUERGEN ,  DIETERLE MARTIN ,  KLAPPERT KARL-HEINRICH ,  MUELLER-ENGEL KLAUS JOACHIM

    IPC: B01J8/06 ,  B01J19/02 ,  B32B15/01 ,  C07C5/333 ,  C07C51/215 ,  C22C30/00 ,  C22C38/40

    Abstract: Continuous heterogeneously catalyzed partial dehydrogenation of at least one hydrocarbon to be dehydrogenated in the gas phase involves at least one catalyst bed disposed in the reaction chamber and with generation of a product gas comprising the at least one dehydrogenated hydrocarbon, unconverted hydrocarbon to be dehydrogenated and molecular hydrogen and/or steam, is dehydrogenated partially in an oxidative or non-oxidative manner to at least one dehydrogenated hydrocarbon, and at least one product gas stream is withdrawn continuously from the reaction chamber. Process for continuous heterogeneously catalyzed partial dehydrogenation of at least one hydrocarbon to be dehydrogenated in the gas phase involves a reaction chamber enclosed by a shell which is in contact with the reaction chamber and has at least one first orifice for feeding at least one starting gas stream into the reaction chamber and at least one second orifice for withdrawing at least one product gas stream from the reaction chamber, at least one starting gas stream comprising at least one hydrocarbon to be dehydrogenated is fed continuously in the reaction chamber. The at least one hydrocarbon to be dehydrogenated is conducted through at least one catalyst bed disposed in the reaction chamber and with generation of a product gas comprising the at least one dehydrogenated hydrocarbon, unconverted hydrocarbon to be dehydrogenated and molecular hydrogen and/or steam, is dehydrogenated partially in an oxidative or non-oxidative manner to at least one dehydrogenated hydrocarbon, and at least one product gas stream is withdrawn continuously from the reaction chamber. The shell is manufactured from a composite material which, on its side B in contact with the reaction chamber, consists of steel B comprising (wt.%): chromium (18-30), nickel (9-37), silicon (1-4), aluminum (>=0-4), nitrogen (>=0-0.3), carbon (>=0-0.15), manganese (>=0-4), phosphorus (>=0-0.05), sulfur (>=0-0.05), and at least one rare earth metal (>=0-0.1), and iron and impurities resulting from production. The steel B, on its side A facing away from the reaction chamber, is plated either directly or via an intermediate layer of copper, and/or nickel, onto steel A comprising (wt.%): chromium (15-20), nickel (6-18), silicon (>=0-0.8), aluminum (>=0-0.8), nitrogen (>=0-0.3), carbon (>=0-0.15), molybdenum (>=0-4), manganese (>=0-2), titanium (>=0-0.8), niobium (>=0-1.2), vanadium (>=0-0.9), boron (>=0-0.1), phosphorus (>=0-0.05), sulfur (>=0-0.05), iron and impurities resulting from production, or a composition comprising (wt.%) Cr (19-23), Ni (30-35), Co (>=0-1), Si (>=0-1), Al (0.15-0.7), C (>=0-0.12), Mn (>=0-2), Cu (>=0-0.75), Ti (0.15-0.7), Nb (>=0-0.1), P (>=0-0.05), S (>=0-0.05) and iron and impurities resulting from production. An independent claim is included for a shell encloses an interior and has at least one first orifice for feeding at least one gas stream into the interior and at least one second orifice for withdrawing a gas stream fed to the interior beforehand via the at least one first orifice O1 from the interior. The shell is manufactured from a composite material which, on its side B in contact with the reaction chamber, consists of steel B on its side A facing away from the reaction chamber is plated either directly or via an intermediate layer of copper and/or nickel onto steel A.

    CATALIZADOR CON SOPORTE A BASE DE DIOXIDO DE ZIRCONIO Y EMPLEO PARA DESHIDROGENACIONES.
    38.
    发明专利
    CATALIZADOR CON SOPORTE A BASE DE DIOXIDO DE ZIRCONIO Y EMPLEO PARA DESHIDROGENACIONES. 未知

    公开(公告)号：ES2363218T3

    公开(公告)日：2011-07-27

    申请号：ES03729967

    申请日：2003-05-02

    Applicant: BASF SE

    Inventor： HOFSTADT OTTO ,  HESSE MICHAEL ,  SCHINDLER GOETZ-PETER ,  HARTH KLAUS ,  SIMON FALK

    IPC: B01J21/06 ,  B01J23/62 ,  B01J23/24 ,  B01J23/40 ,  B01J23/63 ,  B01J23/70 ,  B01J35/00 ,  B01J35/10 ,  B01J37/00 ,  C07B61/00 ,  C07C5/327 ,  C07C5/333 ,  C07C11/06

    Abstract: Catalizador, que contiene sobre un soporte del catalizador uno o varios elementos, elegidos entre el grupo que está constituido por los elementos de los grupos VIII y/o VI secundarios y, en caso dado, uno o varios elementos más, elegidos entre el grupo que está constituido por los elementos de los grupos I y II principales, del grupo III secundario, con inclusión de los lantánidos, del grupo III principal, el renio, el zinc y el estaño, siendo preparado el soporte del catalizador por medio de la formación de una mezcla de polvo de dióxido de zirconio con un compuesto orgánico del silicio a título de agente aglutinante, en caso dado con un agente formador de poros, en caso dado con un ácido, con agua así como, en caso dado, con otros aditivos para formar una masa plástica, la homogeneización de la masa, el moldeo de la masa para formar cuerpos moldeados, el secado y la calcinación, caracterizado porque el agente aglutinante se elige entre los compuestos orgánico del silicio monómeros de las formulas generales (I) hasta (VI) (Hal)xSiR4-x (I) (Hal)xSi(OR 1 )4-x (II) (Hal)xSi(NR 1 R 2 )4-x (III) RxSi(OR 1 )4-x (IV) RxSi(NR 1 R 2 )4-X (V) (R 1 O)xSi(NR 1 R 2 )4-x (VI) en las que Hal significan, independientemente entre sí, halógeno (F, Cl, Br o I), R significan, independientemente entre sí, H o un resto alquilo, alquenilo, alquinilo, cicloalquilo, cicloalquenilo, arilalquilo o arilo, en caso dado substituido, R 1 , R 2 significan, independientemente entre sí, H o un resto alquilo, acilo, arilalquilo o arilo, en caso dado substituido, y X significa desde 0 hasta 4.

    39.
    发明专利
    未知

    公开(公告)号：AT461165T

    公开(公告)日：2010-04-15

    申请号：AT03763815

    申请日：2003-07-10

    Applicant: BASF SE

    Inventor： SCHINDLER GOETZ-PETER ,  WALSDORFF CHRISTIAN ,  HARTH KLAUS ,  HIBST HARTMUT

    IPC: B01J23/62 ,  C07C5/333 ,  C07B61/00 ,  C07C11/167

    Abstract: The invention relates to a process for preparing butadiene from n-butane comprising the steps (A) providing an n-butane-containing feed gas stream, (B) feeding the n-butane-containing feed gas stream into a first dehydrogenation zone and nonoxidatively catalytically dehydrogenating n-butane to 1-butene, 2-butene and optionally butadiene to obtain a first product gas stream comprising n-butane, 1-butene and 2-butene, with or without butadiene and secondary components, (C) feeding the first product gas stream comprising n-butane, 1-butene and 2-butene, with or without butadiene and secondary components, into a second dehydrogenation zone and oxidatively dehydrogenating 1-butene and 2-butene to butadiene to give a second product gas stream comprising butadiene, n-butane and steam, with or without secondary components, (D) recovering butadiene from the second product gas stream.

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