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    FERROUS ZEOLITE, METHOD FOR PRODUCING FERROUS ZEOLITES, AND METHOD FOR CATALYTICALLY REDUCING NITROUS OXIDES
    1.
    发明申请
    FERROUS ZEOLITE, METHOD FOR PRODUCING FERROUS ZEOLITES, AND METHOD FOR CATALYTICALLY REDUCING NITROUS OXIDES 审中-公开
    含铁沸石，用于生产含铁沸石和方法的氮氧化物催化还原

    公开(公告)号：WO2011073123A3

    公开(公告)日：2011-10-20

    申请号：PCT/EP2010069476

    申请日：2010-12-13

    Applicant: BASF SE ,  GROSSSCHMIDT DIRK ,  YILMAZ BILGE ,  KLINGLER DIRK ,  ZOELS BERND

    Inventor： GROSSSCHMIDT DIRK ,  YILMAZ BILGE ,  KLINGLER DIRK ,  ZOELS BERND

    IPC: B01J29/76 ,  B01D53/94 ,  B01J29/072 ,  B01J37/02

    CPC classification number: B01J37/0238 ,  B01D53/9427 ,  B01D2251/2062 ,  B01D2255/20738 ,  B01D2255/50 ,  B01J29/072 ,  B01J29/76 ,  B01J29/7615 ,  B01J29/763 ,  B01J29/85 ,  B01J35/0073 ,  B01J35/1014 ,  B01J35/1019 ,  B01J35/1057 ,  B01J37/0234 ,  B01J37/086 ,  B01J2229/186 ,  B01J2229/34 ,  B01J2229/40 ,  Y02C20/10

    Abstract: The present invention relates to a ferrous zeolite, wherein the number of iron centers, relative to the zeolite, is greater than the number of cation positions of the zeolite. The present invention further relates to a ferrous zeolite that can be produced by gas phase reaction with iron pentacarbonyl, comprising a greater specific surface area than analogous ferrous zeolites produced by ion exchange and/or more hydrothermally stable than analogous ferrous zeolites produced by ion exchange. The present invention further relates to a ferrous zeolite of BETA structure that can be produced by gas phase reaction with iron pentacarbonyl, wherein the number of iron clusters greater than 10 nm is less than 15 wt%, relative to the total amount of iron. The present invention further relates to a method for producing ferrous zeolithic material, characterized in that doping with iron takes place by means of a gas phase reaction using iron pentacarbonyl. The present invention further relates to a method for catalytically reducing nitrogen oxides by adding ammoniac and using catalysts comprising said ferrous zeolithic material.

    Abstract translation: 本发明涉及一种含铁沸石，其中铁原子的基于沸石的数量，比沸石的阳离子位置的数目越大。 此外，本发明涉及通过用五羰基铁，其具有比通过离子交换含铁沸石和/或水热比通过离子交换含铁沸石制造的类似的稳定产生模拟较大的比表面积的气相反应产生的含铁Zeoltihen。 此外，本发明betriff结构BETA的含铁沸石，通过用五羰基铁气相反应产生的，与铁簇是大于10纳米，小于15重量％的数量，基于铁的总量是。 此外，本发明涉及一种用于含有铁的沸石材料，其特征在于，所述掺杂经由使用五羰基铁气相反应用铁进行的制备方法。 此外，本发明涉及一种用于在添加氨的催化还原氮氧化物和使用包含所述含铁的沸石材料的催化剂的处理。

    FERROUS ZEOLITE, METHOD FOR PRODUCING FERROUS ZEOLITES, AND METHOD FOR CATALYTICALLY REDUCING NITROUS OXIDES
    3.
    发明专利
    FERROUS ZEOLITE, METHOD FOR PRODUCING FERROUS ZEOLITES, AND METHOD FOR CATALYTICALLY REDUCING NITROUS OXIDES 未知

    公开(公告)号：CA2784860A1

    公开(公告)日：2011-06-23

    申请号：CA2784860

    申请日：2010-12-13

    Applicant: BASF SE

    Inventor： GROSSSCHMIDT DIRK ,  YILMAZ BILGE ,  KLINGLER DIRK ,  ZOELS BERND

    IPC: B01J29/76 ,  B01D53/94 ,  B01J29/072 ,  B01J37/02

    Abstract: The present invention relates to a ferrous zeolite, wherein the number of iron centers, relative to the zeolite, is greater than the number of cation positions of the zeolite. The present invention further relates to a ferrous zeolite that can be produced by gas phase reaction with iron pentacarbonyl, comprising a greater specific surface area than analogous ferrous zeolites produced by ion exchange and/or more hydrothermally stable than analogous ferrous zeolites produced by ion exchange. The present invention further relates to a ferrous zeolite of BETA structure that can be produced by gas phase reaction with iron pentacarbonyl, wherein the number of iron clusters greater than 10 nm is less than 15 wt%, relative to the total amount of iron. The present invention further relates to a method for producing ferrous zeolithic material, characterized in that doping with iron takes place by means of a gas phase reaction using iron pentacarbonyl. The present invention further relates to a method for catalytically reducing nitrogen oxides by adding ammoniac and using catalysts comprising said ferrous zeolithic material.

    Verfahren zur Hydrierung von Butadiin
    4.
    发明专利
    Verfahren zur Hydrierung von Butadiin 未知

    公开(公告)号：DE102009027770B4

    公开(公告)日：2019-05-09

    申请号：DE102009027770

    申请日：2009-07-16

    Applicant: BASF SE

    Inventor： KÖNIGSMANN LUCIA ,  SCHWAB EKKEHARD ,  MAKARCZYK PIOTR ,  EHRHARDT KAI RAINER ,  VICARI MAXIMILIAN ,  HEIDEMANN THOMAS ,  GROSSSCHMIDT DIRK ,  WATERS GERRIT

    IPC: C07C5/08 ,  B01J23/56 ,  C07C7/167 ,  C07C9/10

    Abstract: Verfahren zur Hydrierung von Butadiin zu Butan an einem Katalysator, der mindestens ein Platingruppenmetall auf einem anorganischen Metalloxid als Träger aufweist, wobei die Hydrierung bei einem Druck im Bereich von 1 bis 40 bar und einer Temperatur im Bereich von 0 bis 100 °C durchgeführt wird und 0,05 bis 5 Gew.-%, bezogen auf den gesamten Katalysator, Platingruppenmetall auf dem Träger vorliegt, dadurch gekennzeichnet, dass ein aus der Gaswäsche von Acetylen mit einem organischen Lösungsmittel, ausgewählt aus N-Methylpyrrolidon, Dimethylformamid, Aceton, Furfurol, Acetonitril, Dimethylacetamid oder Gemischen davon erhaltener Strom eingesetzt wird, in dem, bezogen auf Butadiin, bis zu 20 Gew.-% Vinylacetylen und bis zu 10 Gew.-% Acetylen vorliegen können und im Strom 1 bis 10 Gew.-%, bezogen auf den gesamten Strom, an Butadiin enthalten sind, die Hydrierung mit einem Flüssigkreislauf mit einem Gewichtsverhältnis von Recyclestrom zu Zustrom im Bereich von 2 bis 20 betrieben wird und der Katalysatorträger eine Porosität von 0,2 bis 1,0 ml/g aufweist.

    zeólito contendo ferro, processo para a preparação de um material zeolítico contendo ferro, e, uso do material zeolítico contendo ferro
    6.
    发明专利
    zeólito contendo ferro, processo para a preparação de um material zeolítico contendo ferro, e, uso do material zeolítico contendo ferro 未知

    公开(公告)号：BR112012014735A2

    公开(公告)日：2016-04-12

    申请号：BR112012014735

    申请日：2010-12-13

    Applicant: BASF SE

    Inventor： ZOELS BERND ,  YILMAZ BILGE ,  GROSSSCHMIDT DIRK ,  KLINGLER DIRK

    IPC: B01D53/94 ,  B01J29/072 ,  B01J29/76 ,  B01J37/02

    Abstract: zeólito contendo ferro, processo para a preparação de um material zeolítico contendo ferro, e, uso do meterial zeolítico contendo ferro. a presente invenção refere-se a um zeólito ferroso, em que o número de centris de ferro, em relação ao zeólito, é maior do que o npumero de posições de cátion do zeólito. a presente invenção refere-se ainda a um zeólito ferroso, que pode ser produzido através de reação em fase gasossa com ferro pentacarbonila, compreendendo uma área superficial específica maior do que os zeólitos ferrosos análogos, produzidos através de troca iônica e/ou mais hidrotermicamente estáveis do que os zeólitos ferrosos análogos produzidos através de estrutura beta, que pode ser produzido através de reação em fase gagos com ferro pentacarbonila, em que o número de aglomerados de ferro maiores do que 10 nm é inferior a 15%, em peso, em relação à quantidade total de ferro. a presente invenção refere-se ainda a um método para a produção de um material zeolítico ferroso, caracterizado pelo fato de que a dopagem com ferro ocorre por meio de reação de uma fase gasosa, usando ferro pentacarbonila. a presente invenção refere-se ainda a um método para a redução catalítica de óxidos de nitrogênio através da adição de amoníaco e uso de catalisadores compreendendo o referido material zeolítico ferroso.

    Thermal partial oxidation of hydrocarbons in a reactor for producing acetylene and synthesis gas, comprises introducing raw materials into the reactor and mixing in mixing zone, and supplying the mixture by diffuser into burner block
    9.
    发明专利
    Thermal partial oxidation of hydrocarbons in a reactor for producing acetylene and synthesis gas, comprises introducing raw materials into the reactor and mixing in mixing zone, and supplying the mixture by diffuser into burner block 未知

    公开(公告)号：DE102009001045A1

    公开(公告)日：2009-09-10

    申请号：DE102009001045

    申请日：2009-02-20

    Applicant: BASF SE

    Inventor： GROSSSCHMIDT DIRK ,  HOFFMANN ARNE ,  VICARI MAXIMILIAN ,  WEICHERT CHRISTIAN

    IPC: C07C11/24 ,  B01J19/00 ,  B01J19/24 ,  B01J19/26 ,  C07C2/82

    Abstract: The method comprises introducing raw materials needed for thermal partial oxidation into a reactor (1) and mixing in a mixing zone, and supplying the mixture by a diffuser into a burner block (15) provided with channels (2). The mixture flowing through the channels forms a turbulent flow field by turbulence generators arranged in the channels due to the predetermined deflection of flow direction. The turbulence generators are inserted in all channels and are arranged in such a manner that it forms an alternative rotational direction during the flow of the material through the channels. The method comprises introducing raw materials needed for thermal partial oxidation into a reactor (1) and mixing in a mixing zone, and supplying the mixture by a diffuser into a burner block (15) provided with channels (2). The mixture flowing through the channels forms a turbulent flow field by turbulence generators arranged in the channels due to the predetermined deflection of flow direction. The turbulence generators are inserted in all channels and are arranged in such a manner that it forms an alternative rotational direction during the flow of the material through the channels related to neighboring channels. Auxiliary flames (14) used for flame stabilization are generated at a distance of 4-15 times of the channel diameter from the lower edge of the burner block measured in a combustion chamber (4). An independent claim is included for a device for the thermal partial oxidation of hydrocarbons in a reactor for producing acetylene and synthesis gas.

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